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arXiv:1705.08913 · Physical review. B./Physical review. B

Bound states of fractionalized excitations in a modulated Kitaev spin liquid

Hugo Théveniaut, Matthias Vojta C

Published Aug 1, 2017• 7 citations
arXivHTMLPDF

Abstract

Fractionalization is a hallmark of spin-liquid behavior; it typically leads to response functions consisting of continua instead of sharp modes. However, microscopic processes can enable the formation of short-distance bound states of fractionalized excitations, despite asymptotic deconfinement. Here we study such bound-state formation for the ${\mathbb{Z}}_{2}$ spin liquid realized in Kitaev's honeycomb compass model, supplemented by a kekul\'e distortion of the lattice. Bound states between flux pairs and Majorana fermions form in the Majorana band gaps. We calculate the dynamic spin susceptibility and show that bound states lead to sharp modes in the magnetic response of the spin liquid, with the momentum dependence of the corresponding spectral weight encoding the internal symmetry of the bound state. As a byproduct, we also show that isolated fluxes may produce Majorana bound states at exactly zero energy. Generalizations and implications of the results are discussed.

DOI
10.1103/physrevb.96.054401

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Fractionalization is a hallmark of spin-liquid behavior; it typically leads to response functions consisting of continua instead of sharp modes. However, microscopic processes can enable the formation of short-distance bound states of fractionalized excitations, despite asymptotic deconfinement. Here we study such bound-state formation for the Z2{\mathbb{Z}}_{2}Z2​ spin liquid realized in Kitaev's honeycomb compass model, supplemented by a kekul'e distortion of the lattice. Bound states between flux pairs and Majorana fermions form in the Majorana band gaps. We calculate the dynamic spin susceptibility and show that bound states lead to sharp modes in the magnetic response of the spin liquid, with the momentum dependence of the corresponding spectral weight encoding the internal symmetry of the bound state. As a byproduct, we also show that isolated fluxes may produce Majorana bound states at exactly zero energy. Generalizations and implications of the results are discussed.
The Kitaev model on a honeycomb lattice with bond-dependent Ising interactions offers an exactly solvable model of a quantum spin liquid (QSL) with fractionalized excitations: gapped Z2{Z}_{2}Z2​ fluxes and gapless linearly dispersing Majorana fermions in the isotropic limit (Kx=Ky=Kz{K}_{x}={K}_{y}={K}_{z}Kx​=Ky​=Kz​). We explore the phase diagram along two axes, an external magnetic field hhh, applied out of plane of the honeycomb, and anisotropic interactions Kz{K}_{z}Kz​ larger than the other two (${K}_{x}={K}_{y}\ensuremath{\equiv}K$). For ${K}_{z}/K\ensuremath{\gg}2$ and h=0h=0h=0, the matter Majorana fermions have the largest gap, and the system is described by a gapped Z2{Z}_{2}Z2​ toric code. One of the central questions we address is whether the fractionalized excitations in the different phases have sharp signatures that can be detected in experiments. We show that while the response to single-spin excitations is broad, the spectral function corresponding to two-spin excitations across a bond has sharp signatures that can be attributed to specific anyons. In the toric code regime, the $\ensuremath{\epsilon}=e\ifmmode\times\else\texttimes\fi{}m$ fermion, formed from the bosonic Ising electric (eee) and magnetic (mmm) charges, disperses along a specific one-dimensional direction that provides a fingerprint of fractionalization. At lower Kz{K}_{z}Kz​ in the center of the Abelian phase, in a regime we dub the primordial fractionalized regime, the field generates a hybridization between the $\ensuremath{\epsilon}$ fermion and the Majorana matter fermion, resulting in a $\ensuremath{\psi}$ fermion which too has a distinct quasi-one-dimensional dispersion. All the other phases in the field-anisotropy plane are naturally obtained from this primordial soup. These highly constrained fractonlike dispersions can be observable by inelastic light and neutron scattering, thereby providing ``smoking gun'' signatures of fractionalization in the QSL phase. Our analysis is based on calculations of susceptibilities, topological entanglement entropy, and excitation dynamics, obtained using exact diagonalization and density matrix renormalization group, and supported by perturbation theory.
We provide a complete and exact theoretical study of the dynamical structure factor of a twodimensional quantum spin liquid in gapless and gapped phases, as realized in Kitaev's honeycomb model.We show that there are direct signatures-qualitative and quantitative-of the Majorana fermions and gauge fluxes emerging in this model.These include counterintuitive manifestations of quantum number fractionalization, such as a neutron scattering response with a gap even in the presence of gapless excitations, and a sharp component despite the fractionalization of electron spin.Our analysis identifies new varieties of the venerable x-ray edge problem and explores connections to the physics of quantum quenches.
The Kitaev honeycomb model has attracted significant interest due to its quantum spin liquid ground state, fractionalized Majorana excitations, and topological properties. Motivated by these features, we introduce a quasi-one-dimensional Kitaev-like spin chain derived from a truncated honeycomb geometry. The resulting Majorana band structure contains both dispersive and flat bands, with a gap closing at a critical anisotropy that separates trivial and chiral topological phases. Under open boundary conditions, the topological regime hosts zero-energy edge modes protected by chiral symmetry, placing the system in the BDI symmetry class with a quantized winding number. In the excited spectrum, localized plaquette modes emerge near zero energy and can be tuned by introducing domains of negative plaquettes. The dynamical spin correlation function reveals broad continua associated with fractionalized excitations, together with characteristic low-energy spectral weight from edge Majorana modes. These features distinguish the present system from conventional Heisenberg spin chains and provide experimentally relevant fingerprints of chiral topological order. Our model thus establishes a conceptual bridge between the two-dimensional Kitaev spin liquid and Kitaev's one-dimensional quantum wire.
Motivated by the appearance of Majorana fermions in a broad range of correlated and topological electronic systems, we develop a general method to compute the dynamical response of interacting Majorana fermions in the random-phase approximation (RPA). This can be applied self-consistently on top of Majorana mean-field theory backgrounds, thereby in particular providing a powerful tool to analyze behavior in the vicinity of (various heavily studied) exactly soluble models. Prime examples are quantum spin liquids (QSL) with emergent Majorana excitations, with the celebrated exact solution of Kitaev. We employ the RPA to study in considerable detail phase structure and dynamics of the extended Kitaev honeycomb K J Γ model, with and without an applied field. First, we benchmark our method with Kitaev's exactly soluble model, finding a remarkable agreement. The interactions between Majorana fermions even turn out to mimic the effect of local Z 2 flux excitations, which we explain analytically. Second, we show how small non-Kitaev couplings J and Γ induce Majorana bound states, resulting in sharp features in the dynamical structure factor in the presence of fractionalization: such “spinon excitons” naturally appear, and can coexist and interact with the broad Majorana continuum. Third, for increasing couplings or field, our theory predicts instabilities of the Kitaev QSL (KQSL) triggered by the condensation of the sharp modes. From the high-symmetry momenta of the condensation we can deduce which magnetically ordered phases surround the KQSL, in good agreement with previous finite-size numerics. We discuss implications for experiments and the broad range of applicability of our method to other QSL and Majorana systems.
We propose a mechanism to explain the emergence of an intermediate gapless spin liquid phase in the antiferromagnetic Kitaev model in an externally applied magnetic field, sandwiched between the well-known gapped chiral spin liquid and the gapped partially polarized phase. We propose that, in moderate fields, π-fluxes nucleate in the ground state and trap Majorana zero modes. As these fluxes proliferate with increasing field, the Majorana zero modes overlap creating an emergent Z2{{\mathbb{Z}}}_{2}Z2​ quantum Majorana metallic state with a “Fermi surface” at zero energy. We further show that the Majorana spectral function captures the dynamical spin and dimer correlations obtained by the infinite Projected Entangled Pair States method, thereby validating our variational approach. The authors study the formation and characteristics of a Majorana metallic quantum spin liquid state in Kitaev’s honeycomb model under a moderate external magnetic field. This state represents a novel class of gapless quantum spin liquids stabilized by magnetic field.
Kitaev's model of spins interacting on a honeycomb lattice describes a quantum spin liquid, where an emergent static Z2{\mathbb{Z}}_{2}Z2​ gauge field is coupled to Majorana fermions. In the presence of an external magnetic field and for a range of interaction strengths, the system behaves as a gapped, non-Abelian quantum spin liquid. In this phase, the vortex excitations of the emergent Z2{\mathbb{Z}}_{2}Z2​ gauge field have Majorana zero modes bound to them. Motivated by recent experimental progress in measuring and characterizing real materials that could exhibit spin-liquid behavior, we analytically calculate the dynamical spin structure factor in the non-Abelian phase of the Kitaev's honeycomb model. In particular, we treat the case of quenched disorder in the vortex configurations. Our calculations reveal a peak in the low-energy dynamical structure factor that is a signature of the spin-liquid behavior. We map the effective Hamiltonian to that of a chiral ppp-wave superconductor by using the Jordan-Wigner transformation. Subsequently, we analytically calculate the wave functions of the Majorana zero modes, the energy splitting for finite separation of the vortices and, finally, the dynamical structure factor in presence of quenched disorder.