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arXiv:2206.12990 · Physical review. B./Physical review. B

Anyon dynamics in field-driven phases of the anisotropic Kitaev model

Shi Feng, Adhip Agarwala, Subhro Bhattacharjee, Nandini Trivedi

Published Jul 27, 2023• 18 citations
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Abstract

The Kitaev model on a honeycomb lattice with bond-dependent Ising interactions offers an exactly solvable model of a quantum spin liquid (QSL) with fractionalized excitations: gapped ${Z}_{2}$ fluxes and gapless linearly dispersing Majorana fermions in the isotropic limit (${K}_{x}={K}_{y}={K}_{z}$). We explore the phase diagram along two axes, an external magnetic field $h$, applied out of plane of the honeycomb, and anisotropic interactions ${K}_{z}$ larger than the other two (${K}_{x}={K}_{y}\ensuremath{\equiv}K$). For ${K}_{z}/K\ensuremath{\gg}2$ and $h=0$, the matter Majorana fermions have the largest gap, and the system is described by a gapped ${Z}_{2}$ toric code. One of the central questions we address is whether the fractionalized excitations in the different phases have sharp signatures that can be detected in experiments. We show that while the response to single-spin excitations is broad, the spectral function corresponding to two-spin excitations across a bond has sharp signatures that can be attributed to specific anyons. In the toric code regime, the $\ensuremath{\epsilon}=e\ifmmode\times\else\texttimes\fi{}m$ fermion, formed from the bosonic Ising electric ($e$) and magnetic ($m$) charges, disperses along a specific one-dimensional direction that provides a fingerprint of fractionalization. At lower ${K}_{z}$ in the center of the Abelian phase, in a regime we dub the primordial fractionalized regime, the field generates a hybridization between the $\ensuremath{\epsilon}$ fermion and the Majorana matter fermion, resulting in a $\ensuremath{\psi}$ fermion which too has a distinct quasi-one-dimensional dispersion. All the other phases in the field-anisotropy plane are naturally obtained from this primordial soup. These highly constrained fractonlike dispersions can be observable by inelastic light and neutron scattering, thereby providing ``smoking gun'' signatures of fractionalization in the QSL phase. Our analysis is based on calculations of susceptibilities, topological entanglement entropy, and excitation dynamics, obtained using exact diagonalization and density matrix renormalization group, and supported by perturbation theory.

DOI
10.1103/physrevb.108.035149

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The Kitaev model on a honeycomb lattice with bond-dependent Ising interactions offers an exactly solvable model of a quantum spin liquid (QSL) with fractionalized excitations: gapped Z2{Z}_{2}Z2​ fluxes and gapless linearly dispersing Majorana fermions in the isotropic limit (Kx=Ky=Kz{K}_{x}={K}_{y}={K}_{z}Kx​=Ky​=Kz​). We explore the phase diagram along two axes, an external magnetic field hhh, applied out of plane of the honeycomb, and anisotropic interactions Kz{K}_{z}Kz​ larger than the other two (Kx=Ky\ensuremath≡K{K}_{x}={K}_{y}\ensuremath{\equiv}KKx​=Ky​\ensuremath≡K). For Kz/K\ensuremath≫2{K}_{z}/K\ensuremath{\gg}2Kz​/K\ensuremath≫2 and h=0h=0h=0, the matter Majorana fermions have the largest gap, and the system is described by a gapped Z2{Z}_{2}Z2​ toric code. One of the central questions we address is whether the fractionalized excitations in the different phases have sharp signatures that can be detected in experiments. We show that while the response to single-spin excitations is broad, the spectral function corresponding to two-spin excitations across a bond has sharp signatures that can be attributed to specific anyons. In the toric code regime, the \ensuremathϵ=e\ifmmode×\else\texttimes\fim\ensuremath{\epsilon}=e\ifmmode\times\else\texttimes\fi{}m\ensuremathϵ=e\ifmmode×\else\texttimes\fim fermion, formed from the bosonic Ising electric (eee) and magnetic (mmm) charges, disperses along a specific one-dimensional direction that provides a fingerprint of fractionalization. At lower Kz{K}_{z}Kz​ in the center of the Abelian phase, in a regime we dub the primordial fractionalized regime, the field generates a hybridization between the \ensuremathϵ\ensuremath{\epsilon}\ensuremathϵ fermion and the Majorana matter fermion, resulting in a \ensuremathψ\ensuremath{\psi}\ensuremathψ fermion which too has a distinct quasi-one-dimensional dispersion. All the other phases in the field-anisotropy plane are naturally obtained from this primordial soup. These highly constrained fractonlike dispersions can be observable by inelastic light and neutron scattering, thereby providing ``smoking gun'' signatures of fractionalization in the QSL phase. Our analysis is based on calculations of susceptibilities, topological entanglement entropy, and excitation dynamics, obtained using exact diagonalization and density matrix renormalization group, and supported by perturbation theory.
Quantum spin liquids (QSLs) host a variety of fractionalized particles. In Kitaev's paradigmatic honeycomb model a spin-fractionalizes intoflux due to emergentgauge field and matter Majorana fermions. Although these excitations have well-defined dynamics in the integrable limit, their direct experimental identification is notoriously challenging: realistic materials inevitably host additional symmetry-allowed interactions that break integrability and hybridize gauge and matter sectors, while magnetic fields, which are often required to suppress competing order and stabilize a putative QSL regime, further entangle the responses of different fractionalized quasiparticles and may even drive the system into field-induced spin-liquid phases that are not adiabatically connected to the integrable limit. A prominent example is the quantum Majorana metal, in which the distinct dynamics of fractionalized Majorana fermions can become directly visible in scattering. This review highlights recent progress on these related questions: in which field-stabilized QSL regimes and nearby emergent phases, and under what conditions, can the response of a specific fractionalized quasiparticle be isolated and positively understood, thereby clarifying the existence and the experimental scope of putative spin liquids? We review the progress on these questions across Abelian, non-Abelian, and emergent quantum phases under magnetic field that are not perturbatively connected to the integrable limit. We connect these field-induced dynamical phenomena to concrete experimental observables, relevant for neutron scattering, resonant inelastic x-ray scattering, and pump-probe spectroscopy, techniques that are capable of identifying the nature of different magnetic-field-induced phases and resolving specific types of fractionalized particles, including Majoranas andfluxes.
The authors investigate dynamical signatures of fractionalization in the Kitaev honeycomb model under an out-of-plane magnetic field using advanced tensor network methods. By analyzing spin-spin and dimer-dimer correlations through the infinite Projected Entangled Pair States (iPEPS) simulations, they demonstrate distinct spectral features separating Majorana fermions from Z₂ flux excitations in the chiral spin liquid phase. Crucially, they identify the controversial intermediate phase as a gapless Majorana metal driven by strong flux fluctuations, characterized by logarithmic divergence in the low-energy density of states. This resolves a longstanding debate about the regime in question.
In the Kitaev honeycomb model, a weak magnetic field gaps the gapless Majorana cone, driving the system into a gapped non-Abelian phase with Ising topological order. The edge supports a single chiral Majorana mode with chiral central charge c−=1/2c_- = 1/2c−​=1/2, yielding a half-quantized thermal Hall conductance κxy/T=π2kB2/6h\kappa_{xy}/T = \pi^2 k_B^2/6hκxy​/T=π2kB2​/6h. We rigorously investigate whether observing this half-quantized value uniquely identifies the non-Abelian Ising anyon sector, or whether Abelian topological orders or extrinsic mechanisms can produce the same signature. By combining the edge-bulk correspondence with the classification of strictly two-dimensional bosonic topological orders, we show that a chiral central charge c−=1/2c_-=1/2c−​=1/2 (mod 8) is the unique fingerprint of the Ising non-Abelian anyon theory among minimal bosonic topological orders. Abelian bosonic orders necessarily have integer c−c_-c−​, with the minimal nonzero value being c−=1c_-=1c−​=1. Thus, a robustly half-quantized κxy/T\kappa_{xy}/Tκxy​/T uniquely distinguishes the Majorana sector from Abelian alternatives, provided the system is a genuine 2D bosonic spin system free of invertible E8E_8E8​ stacking or phonon contamination. ## 1. Introduction The Kitaev honeycomb model is an exactly solvable model of a quantum spin liquid, characterized by fractionalized excitations known as anyons. In the absence of a magnetic field, the model hosts a gapless Majorana cone. A weak magnetic field in the [111] direction gaps this cone and induces a non-Abelian phase with Ising topological order. This phase supports a single chiral Majorana edge mode, which contributes to a quantized thermal Hall conductance. The central question addressed in this preprint is whether the observation of a half-quantized thermal Hall conductance, corresponding to a chiral central charge c−=1/2c_- = 1/2c−​=1/2, uniquely identifies the non-Abelian Ising anyon sector, or if Abelian topological orders can mimic this signature. ## 2. Background The thermal Hall conductance $\kappa_{x
A prominent feature of quantum spin liquids is fractionalization of the spin degree of freedom. Fractionalized excitations have their own dynamics in different energy scales, and hence, affect finite-temperature (TTT) properties in a peculiar manner even in the paramagnetic state harboring the quantum spin liquid state. We here present a comprehensive theoretical study of the spin dynamics in a wide TTT range for the Kitaev model on a honeycomb lattice, whose ground state is a quantum spin liquid. In this model, the fractionalization occurs to break up quantum spins into itinerant matter fermions and localized Z2{Z}_{2}Z2​ fluxes, which results in two crossovers at very different TTT scales. Extending the previous study for the isotropic coupling case [J. Yoshitake, J. Nasu, and Y. Motome, Phys. Rev. Lett. 117, 157203 (2016)], we calculate the dynamical spin structure factor $S(\mathbf{q},\ensuremath{\omega})$, the NMR relaxation rate 1/T11/{T}_{1}1/T1​, and the magnetic susceptibility $\ensuremath{\chi}$ while changing the anisotropy in the exchange coupling constants, by using the dynamical mean-field theory based on a Majorana fermion representation. We describe the details of the methodology including the continuous-time quantum Monte Carlo method for computing dynamical spin correlations and the maximum entropy method for analytic continuation. We confirm that the combined method provides accurate results in a wide TTT range including the region where the spins are fractionalized. We find that also in the anisotropic cases the system exhibits peculiar behaviors below the high-TTT crossover whose temperature is comparable to the average of the exchange constants: $S(\mathbf{q},\ensuremath{\omega})$ shows an inelastic response at the energy scale of the averaged exchange constant, 1/T11/{T}_{1}1/T1​ continues to grow even though the equal-time spin correlations are saturated and almost TTT independent, and $\ensuremath{\chi}$ deviates from the Curie-Weiss behavior. In particular, when the exchange interaction in one direction is stronger than the other two, the dynamical quantities exhibit qualitatively different TTT dependences from the isotropic case at low TTT, reflecting the opposite parity between the flux-free ground state and the flux-excited state, and a larger energy cost for flipping a spin in the strong interaction direction. On the other hand, when the exchange anisotropy is in the opposite way, the results are qualitatively similar to those in the isotropic case. All these behaviors manifest the spin fractionalization in the paramagnetic region. Among them, the dichotomy between the static and dynamical spin correlations is unusual behavior hardly seen in conventional magnets. We discuss the relation between the dichotomy and the spatial configuration of the Z2{Z}_{2}Z2​ gauge fields. Our results could stimulate further experimental and theoretical analyses of candidate materials for the Kitaev quantum spin liquids.
We determine the phase diagrams of anisotropic Kitaev-Heisenberg models on the honeycomb lattice using parton mean-field theories based on different Majorana fermion representations of the S=1/2 spin operators. First, we use a two-dimensional Jordan-Wigner transformation (JWT) involving a semi-infinite snake string operator. To ensure that the fermionized Hamiltonian remains local, we consider the limit of extreme Ising exchange anisotropy in the Heisenberg sector. Second, we use the conventional Kitaev representation in terms of four Majorana fermions subject to local constraints, which we enforce through Lagrange multipliers. For both representations, we self-consistently decouple the interaction terms in the bond and magnetization channels and determine the phase diagrams as a function of the anisotropy of the Kitaev couplings and the relative strength of the Ising exchange. While both mean-field theories produce identical phase boundaries for the topological phase transition between the gapless and gapped Kitaev quantum spin liquids, the JWT fails to correctly describe the magnetic instability and finite-temperature behavior. Our results show that the magnetic phase transition is first order at low temperatures but becomes continuous above a certain temperature. At this energy scale, we also observe a finite-temperature crossover on the quantum-spin-liquid side, from a fractionalized paramagnet at low temperatures, in which gapped flux excitations are frozen out, to a conventional paramagnet at high temperatures. Published by the American Physical Society 2024
A Kitaev quantum spin liquid involves fractionalized quasiparticles called itinerant Majorana fermions and localized gauge fluxes. The topological character with chiral excitations under a magnetic field is currently in an active debate. For a candidate spin liquid $\ensuremath{\alpha}\text{\ensuremath{-}}{\mathrm{RuCl}}_{3}$, we report low-energy spin excitations through nuclear magnetic and quadrupole resonance measurements down to temperatures three orders of magnitude lower than the exchange energy. In a field-driven disordered state, we found the evolution of two kinds of gapped spin excitations with distinct field dependences. The result is indicative of a field-induced hybridization between fractionalized quasiparticles, as inferred by the perturbation theory for the Kitaev model. The detailed field dependence of spin dynamics across the quantum critical region shows the emergence of a gapless intermediate phase between the gapped zigzag order phase and spin-disordered phases.