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arXiv:1610.04940 · Physical review. B./Physical review. B

Spin blockade and coherent dynamics of high-spin states in a three-electron double quantum dot

Bao-Bao Chen, Bao‐Chuan Wang, Gang Cao, Hai-Ou Li, Ming Xiao, Guang‐Can Guo, H. W. Jiang, Xuedong Hu, Guo‐Ping Guo

Published Jan 10, 2017• 25 citations
arXivHTMLPDF

Abstract

Asymmetry in a three-electron double quantum dot (DQD) allows spin blockade, when spin-3/2 (quadruplet) states and spin-1/2 (doublet) states have different charge configurations. We have observed this DQD spin blockade near the (1,2)-(2,1) charge transition using a pulsed-gate technique and a charge sensor. We, then, use this spin blockade to detect Landau-Zener-St\"uckelberg interference and coherent oscillations between the spin quadruplet and doublet states. Such studies add to our understandings of coherence and control properties of three-spin states in a double dot, which, in turn, would benefit explorations into various qubit encoding schemes in semiconductor nanostructures.

DOI
10.1103/physrevb.95.035408

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Asymmetry in a three-electron double quantum dot (DQD) allows spin blockade, when spin-3/2 (quadruplet) states and spin-1/2 (doublet) states have different charge configurations. We have observed this DQD spin blockade near the (1,2)-(2,1) charge transition using a pulsed-gate technique and a charge sensor. We, then, use this spin blockade to detect Landau-Zener-St"uckelberg interference and coherent oscillations between the spin quadruplet and doublet states. Such studies add to our understandings of coherence and control properties of three-spin states in a double dot, which, in turn, would benefit explorations into various qubit encoding schemes in semiconductor nanostructures.
Landau-Zener-Stuckelberg-Majorana (LZSM) physics has been exploited to coherently manipulate two-electron spin states in a GaAs double quantum dot (DQD) at a singlet (S)-triplet (T+) anti-crossing. The anti-crossing results from the hyperfine interaction with the nuclear spins of the host material [1,2]. However, the fluctuations of the nuclear spin bath result in spin dephasing within T ∗ 2 ∼ 10− 20 ns. As a consequence, the sweep through the anti-crossing would have to be performed on a timescale comparable to T ∗ 2 to achieve LZSM oscillations with 100% visibility. Moreover, the S-T+ anti-crossing is located near the (1, 1)− (2, 0) interdot charge transition, where (nl, nr) denotes the number of electrons in the left and right quantum dot. As a result the singlet state involved in the dynamics is a superpostion of (1, 1) and (2, 0) singlet states. Here we show that it is possible to increase the oscillation visibility while keeping sweep times less than T ∗ 2 using a tailored pulse with a detuning dependent level velocity. The pulse includes a slow level velocity portion that is chosen to coincide with the passage through the S-T+ anti-crossing and two fast level velocity portions. The latter minimize the time spent in regions where spin and charge degrees of freedom are entangled, which renders the qubit susceptible to charge noise. The slow level velocity portion of the pulse results in a stronger effective coupling between the spins states, which increases the oscillations visibility [3,4]. In particular, we were able to obtain a visibility of ∼ 0.5 for LZSM oscillations. This constitutes an important step towards the implementation of a Hadamard gate.
The triple quantum dot energy level spectrum is far more complex than its double quantum dot counterpart. As a result it is a challenge to cleanly manipulate only the two required qubit states without invoking more complex multistate coherent evolution. In this talk I will describe experiments and modeling of lateral triple quantum dot devices where by suitable device gate (i.e. energy level spectrum) tuning and pulse characteristics we were able to characterize and manipulate various three spin qubit species. In particular I will describe measurements where the Landau-Zener –Stuckelberg approach previously demonstrated in double dots is extended to threeinteracting spin states permitting us to demonstrate phenomena such as pairwise exchange control. I will also demonstrate how by tuning the experimental parameters one can controllably switch to coherent oscillations originating from alternative potentially useful qubit states and how to distinguish them.
We present a model of a qubit built of three coherently coupled quantum dots with three spins in a triangular geometry. The qubit states are encoded in the doublet subspace and they are controlled by a gate voltage, which breaks the triangular symmetry of the system. We show how to prepare the qubit and to perform one-qubit operations. A doublet blockade effect in the current will be discussed. The blockade is related to an asymmetry of transfer rates from the electrodes to different doublet states and is used to read out the dynamics of the qubit state. Our research also presents analysis of the Rabi oscillations, decoherence, and leakage processes in the doublets subspace.
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In quantum computing based on semiconductor quantum dots, adding dots (or just electrons) allows a wider search for an optimal qubit-encoding scheme that is both controllable and coherent. This work reports experiments to realize a hybrid charge-spin qubit in a linear triple quantum dot with asymmetric tunnel couplings, in a multielectron charge configuration. This qubit's energy splitting can be tuned conveniently over a wide range, and the authors attain qualitative understanding of the observations in terms of a three-electron system. This should stimulate further exploration of quantum coherent dynamics in the few-electron regime for semiconductor quantum processors.