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arXiv:2008.04375 · Physical review. B./Physical review. B

Triplet-blockaded Josephson supercurrent in double quantum dots

Daniël Bouman, Ruben J. J. van Gulik, Gorm O. Steffensen, Dávid Pataki, Péter Boross, Peter Krogstrup, Jesper Nygård, Jens Paaske, András Pályi, Attila Geresdi

Published Dec 21, 2020• 33 citations
arXivHTMLPDF

Abstract

Serial double quantum dots created in semiconductor nanostructures provide a versatile platform for investigating two-electron spin quantum states, which can be tuned by electrostatic gating and an external magnetic field. In this Rapid Communication, we directly measure the supercurrent reversal between adjacent charge states of an InAs nanowire double quantum dot with superconducting leads, in good agreement with theoretical models. In the even charge parity sector, we observe a supercurrent blockade with increasing magnetic field, corresponding to the spin singlet to triplet transition. Our results demonstrate a direct spin to supercurrent conversion, the superconducting equivalent of the Pauli spin blockade. This effect can be exploited in hybrid quantum architectures coupling the quantum states of spin systems and superconducting circuits.

DOI
10.1103/physrevb.102.220505

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Serial double quantum dots created in semiconductor nanostructures provide a versatile platform for investigating two-electron spin quantum states, which can be tuned by electrostatic gating and an external magnetic field. In this Rapid Communication, we directly measure the supercurrent reversal between adjacent charge states of an InAs nanowire double quantum dot with superconducting leads, in good agreement with theoretical models. In the even charge parity sector, we observe a supercurrent blockade with increasing magnetic field, corresponding to the spin singlet to triplet transition. Our results demonstrate a direct spin to supercurrent conversion, the superconducting equivalent of the Pauli spin blockade. This effect can be exploited in hybrid quantum architectures coupling the quantum states of spin systems and superconducting circuits.
We realize a hybrid superconductor-semiconductor transmon device in which the Josephson effect is controlled by a gate-defined quantum dot in an InAs-Al nanowire.Microwave spectroscopy of the transition spectrum of the transmon allows us to probe the ground-state parity of the quantum dot as a function of the gate voltages, the external magnetic flux, and the magnetic field applied parallel to the nanowire.The measured parity phase diagram is in agreement with that predicted by a single-impurity Anderson model with superconducting leads.Through continuous-time monitoring of the circuit, we furthermore resolve the quasiparticle dynamics of the quantum dot Josephson junction across the phase boundaries.Our results can facilitate the realization of semiconductor-based 0-π qubits and Andreev qubits.
We study a double quantum dot, each dot of which is tunnel coupled to superconducting leads. In the Coulomb blockade regime, a spin-dependent Josephson coupling between two superconductors is induced, as well as an antiferromagnetic Heisenberg exchange coupling between the spins on the double dot that can be tuned by the superconducting phase difference. We show that the correlated spin states---singlet or triplets---on the double dot can be probed via the Josephson current in a dc-superconducting quantum interference device setup.
We demonstrate the Josephson effect in a serial double quantum dot defined in a nanowire with epitaxial superconducting leads. The supercurrent stability diagram adopts a honeycomb pattern. We observe sharp discontinuities in the magnitude of the critical current, I_{c}, as a function of dot occupation, related to doublet to singlet ground state transitions. Detuning of the energy levels offers a tuning knob for I_{c}, which attains a maximum at zero detuning. The consistency between experiment and theory indicates that our device is a faithful realization of the two-impurity Anderson model.
A Pauli spin blockade in quantum dot systems occurs when the charge transport is allowed only for some spin states, and it has been an efficient tool in spin-based qubit devices in semiconductors. We theoretically investigate a Pauli spin blockade in a triple quantum dot molecule consisting of three identical quantum dots in a semiconductor in the presence of an external magnetic field through the molecule. When the three-electron state is on resonance with two- or four-electron states, the Aharonov–Bohm oscillation and the Zeeman splitting lead to a periodic spin blockade effect. We focus on the spin blockade at a two- and three-electron resonance and show that we can tune the magnetic field to selectively allow only either a spin-singlet or spin-triplet state to add an additional electron from tunnel-coupled leads. This spin blockade maintains the three quantum dots at the optimal sweet spot against the charge noise, demonstrating its potential as an efficient readout scheme for the qubits in quantum dot systems.
We report a first direct observation of proximity supercurrent in a single InAs self-assembled quantum dot coupled to superconducting electrodes. We utilize large SAQDs with strong dot-lead coupling allowing sufficient overlap of quantized state that charge fluctuation in the dot may exceed one electron. Although the charging energy is larger than the superconductivity gap, Δ, the voltage characteristic measured in the current-driven four-terminal geometry signifies a supercurrent flow though the dot. The observed critical current is of the order of 10 pA, and much smaller than expected from theory. This current also shows the parity effect with the number of electrons in the dot, suggesting that the singlet correlation impedes the Cooper pair tunneling.
We investigate the idea for probing spin states of two coupled quantum dots (CQDs) by the dc Josephson current flowing through them. This theory requires weak coupling between CQDs and electrodes, but allows arbitrary interdot tunnel coupling, intradot and interdot Coulomb interactions. We find that the Coulomb blockade peaks exhibit a nonmonotonous dependence on the Zeeman splitting of CQDs, which can be understood in terms of Andreev bound states. More importantly, the supercurrent in the Coulomb blockade valleys may provide information on the spin states of CQDs: for CQDs with total electron number N=1,3N=1,3N=1,3 (odd), the supercurrent will reverse its sign if the CQD becomes a magnetic molecule; for a CQD with N=2N=2N=2 (even), the supercurrent will decrease sharply around the transition between the spin singlet and triplet ground states of the CQD.