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Bulletin of the American Physical Society

Interplay of charge and spin coherence in Landau-Zener interferometry in double quantum dots

Hugo Ribeiro

Published Mar 18, 2013• 0 citations
OpenAlex

Abstract

Landau-Zener-Stuckelberg-Majorana (LZSM) physics has been exploited to coherently manipulate two-electron spin states in a GaAs double quantum dot (DQD) at a singlet (S)-triplet (T+) anti-crossing. The anti-crossing results from the hyperfine interaction with the nuclear spins of the host material [1,2]. However, the fluctuations of the nuclear spin bath result in spin dephasing within T ∗ 2 ∼ 10− 20 ns. As a consequence, the sweep through the anti-crossing would have to be performed on a timescale comparable to T ∗ 2 to achieve LZSM oscillations with 100% visibility. Moreover, the S-T+ anti-crossing is located near the (1, 1)− (2, 0) interdot charge transition, where (nl, nr) denotes the number of electrons in the left and right quantum dot. As a result the singlet state involved in the dynamics is a superpostion of (1, 1) and (2, 0) singlet states. Here we show that it is possible to increase the oscillation visibility while keeping sweep times less than T ∗ 2 using a tailored pulse with a detuning dependent level velocity. The pulse includes a slow level velocity portion that is chosen to coincide with the passage through the S-T+ anti-crossing and two fast level velocity portions. The latter minimize the time spent in regions where spin and charge degrees of freedom are entangled, which renders the qubit susceptible to charge noise. The slow level velocity portion of the pulse results in a stronger effective coupling between the spins states, which increases the oscillations visibility [3,4]. In particular, we were able to obtain a visibility of ∼ 0.5 for LZSM oscillations. This constitutes an important step towards the implementation of a Hadamard gate.

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Landau-Zener-Stuckelberg-Majorana (LZSM) physics has been exploited to coherently manipulate two-electron spin states in a GaAs double quantum dot (DQD) at a singlet (S)-triplet (T+) anti-crossing. The anti-crossing results from the hyperfine interaction with the nuclear spins of the host material [1,2]. However, the fluctuations of the nuclear spin bath result in spin dephasing within T ∗ 2 ∼ 10− 20 ns. As a consequence, the sweep through the anti-crossing would have to be performed on a timescale comparable to T ∗ 2 to achieve LZSM oscillations with 100% visibility. Moreover, the S-T+ anti-crossing is located near the (1, 1)− (2, 0) interdot charge transition, where (nl, nr) denotes the number of electrons in the left and right quantum dot. As a result the singlet state involved in the dynamics is a superpostion of (1, 1) and (2, 0) singlet states. Here we show that it is possible to increase the oscillation visibility while keeping sweep times less than T ∗ 2 using a tailored pulse with a detuning dependent level velocity. The pulse includes a slow level velocity portion that is chosen to coincide with the passage through the S-T+ anti-crossing and two fast level velocity portions. The latter minimize the time spent in regions where spin and charge degrees of freedom are entangled, which renders the qubit susceptible to charge noise. The slow level velocity portion of the pulse results in a stronger effective coupling between the spins states, which increases the oscillations visibility [3,4]. In particular, we were able to obtain a visibility of ∼ 0.5 for LZSM oscillations. This constitutes an important step towards the implementation of a Hadamard gate.
We study finite-time Landau-Zener transitions at a singlet-triplet level crossing in a GaAs double quantum dot, both experimentally and theoretically. Sweeps across the anticrossing in the high driving speed limit result in oscillations with a small visibility. Here we demonstrate how to increase the oscillation visibility while keeping sweep times shorter than T(2)(*) using a tailored pulse with a detuning dependent level velocity. Our results show an improvement of a factor of ~2.9 for the oscillation visibility. In particular, we were able to obtain a visibility of ~0.5 for Stückelberg oscillations, which demonstrates the creation of an equally weighted superposition of the qubit states.
We show that universal quantum control of a two-electron singlet-triplet spin qubit can be achieved using Landau-Zener-St\uckelberg interferometry. Going beyond normal Landau-Zener dynamics with infinitely long constant velocity sweeps across an energy level anti-crossing, we focus on a physical system consisting of a two-electron double quantum dot, where the spin states can be admixtures of charge states and the level velocity can be tuned in a time-dependent fashion. Our results indicate that charge coherence must be treated on an equal footing with spin coherence. In particular, we predict the presence of finite-time effects, which result in population transfer even in cases of an incomplete sweep through the anti-crossing. The competing requirements of adiabaticity and coherence are reconciled using specially designed pulses with a tunable level velocity. As a relevant example, we demonstrate that a Hadamard gate can be implemented for a realistic set of conditions in a GaAs double quantum dot device.
Landau-Zener (LZ) transition has received renewed interest as an alternative approach to control single-qubit states. An LZ transition occurs when a system passes through an avoided crossing that arises from quantum mechanical coupling of two levels, taking the system to a coherent superposition of the two states. Then, multiple LZ transitions induce interference known as Landau-Zener-Stückelberg (LZS) interference whose amplitude strongly depends on the velocity or adiabaticity of the passage. Here, we study the roles of LZ transitions and LZS interference in coherent charge oscillations of a one-electron semiconductor double quantum dot by time-domain experiments using standard rectangular voltage pulses. By employing density matrix simulations, we show that, in the standard setup using rectangular pulses, even a small distortion of the pulse can give rise to LZ transitions and hence LZS interference, which significantly enhances the measured oscillation amplitude. We further show experimentally that the nature of the coherent charge oscillations changes from Rabi-type to LZS oscillations with increasing pulse distortion. Our results thus demonstrate that it is essential to take into account LZS interference for both precise control of charge qubits and correct interpretation of measurement results.
We theoretically model a nuclear-state preparation scheme that increases the coherence time of a two-spin qubit in a double quantum dot. The two-electron system is tuned repeatedly across a singlet-triplet level anticrossing with alternating slow and rapid sweeps of an external bias voltage. Using a Landau-Zener-Stückelberg model, we find that in addition to a small nuclear polarization that weakly affects the electron spin coherence, the slow sweeps are only partially adiabatic and lead to a weak nuclear spin measurement and a nuclear-state narrowing which prolongs the electron spin coherence. This resolves some open problems brought up by a recent experiment [D. J. Reilly, Science 321, 817 (2008).10.1126/science.1159221]. Based on our description of the weak measurement, we simulate a system with up to n=200 nuclear spins per dot. Scaling in n indicates a stronger effect for larger n.
Single-spin state evolution induced by the Landau-Zener-St\"uckelberg-Majorana (LZSM) interference in a Zeeman-spit four-level system in a periodically driven double quantum dot is studied theoretically by the Floquet stroboscopic method. An interplay between spin-conserving and spin-flip tunneling processes with the electric dipole spin resonance (EDSR) that is induced in an individual dot and enhanced by the LZSM multiple level crossings with the neighboring quantum dot is investigated as a function of the microwave (MW) frequency, driving amplitude, interdot detuning, and magnetic field. A number of special points in the parameter space are identified, out of which all three features are merged. Under this triple-crossing resonance condition, the interdot tunneling is combined with a fast spin evolution in each dot at the EDSR frequency. Harmonics of the EDSR are revealed in the spin-dependent tunneling maps versus variable magnetic field and MW frequency. The results are applicable for both electron and hole systems with strong spin-orbit interaction and may be useful for developing new time-efficient schemes of the spin control and readout in qubit devices.
We study the dynamics of a pulse-gated semiconductor double-quantum-dot qubit. In our experiments, the qubit coherence times are relatively long, but the visibility of the quantum oscillations is low. We show that these observations are consistent with a theory that incorporates decoherence arising from charge noise that gives rise to detuning fluctuations of the double dot. Because effects from charge noise are largest near the singlet-triplet avoided level crossing, the visibility of the oscillations is low when the singlet-triplet avoided level crossing occurs in the vicinity of the charge degeneracy point crossed during the manipulation, but there is only modest dephasing at the large detuning value at which the quantum phase accumulates. This theory agrees well with experimental data and predicts that the visibility can be increased greatly by appropriate tuning of the interdot tunneling rate.