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arXiv:1609.05304 · Physical review. B./Physical review. B

Low-energy dynamical response of an Anderson insulator with local attraction

Dmitri A. Ivanov, M. V. Feigel’man

Published Jan 30, 2017• 4 citations
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Abstract

The low-frequency dynamical response of an Anderson insulator is dominated by so-called Mott resonances: hybridization of pairs of states close in energy but separated spatially. We study the effect of interaction on Mott resonances in the model of spinful fermions (electrons) with local attraction. This model is known to exhibit a so-called pseudogap: a suppression of the low-energy, single-particle excitations. Correspondingly, the low-energy dynamical response is also reduced. However, this reduction has mostly quantitative character. In particular, the Mott formula for frequency-dependent conductivity preserves its functional asymptotic behavior at low frequencies, but with a small numerical prefactor. This result can be explained in terms of Mott resonances for electron pairs instead of single electrons.

DOI
10.1103/physrevb.95.045147

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The low-frequency dynamical response of an Anderson insulator is dominated by so-called Mott resonances: hybridization of pairs of states close in energy but separated spatially. We study the effect of interaction on Mott resonances in the model of spinful fermions (electrons) with local attraction. This model is known to exhibit a so-called pseudogap: a suppression of the low-energy, single-particle excitations. Correspondingly, the low-energy dynamical response is also reduced. However, this reduction has mostly quantitative character. In particular, the Mott formula for frequency-dependent conductivity preserves its functional asymptotic behavior at low frequencies, but with a small numerical prefactor. This result can be explained in terms of Mott resonances for electron pairs instead of single electrons.
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The pseudogap phase is considered to be a new state of matter in the phase string model of the doped Mott insulator, which is composed of two distinct regimes known as the upper and lower pseudogap phases, respectively. The former corresponds to the formation of spin-singlet pairing, the magnetic characterizations of which have been recently studied [Phys. Rev. B 72, 104520 (2005)]. The latter, as a low-temperature regime of the pseudogap phase, is systematically explored in this work, which is characterized by the formation of the Cooper pair amplitude and described by a generalized Ginzburg-Landau theory. Elementary excitation in this phase is a charge-neutral object carrying spin-1∕21∕21∕2 and locking with a supercurrent vortex, known as a spinon-vortex composite. Such a lower pseudogap phase can be regarded as a vortex liquid state due to the presence of free spinon vortices. Here thermally excited spinon vortices destroy the phase coherence and are responsible for the nontrivial Nernst effect and diamagnetism. The transport entropy and core energy associated with a spinon vortex are determined by the spin degrees of freedom. Such a spontaneous vortex liquid phase can be also considered as a spin liquid with a finite correlation length and gaped S=1∕2S=1∕2S=1∕2 excitations, where a resonancelike nonpropagating spin mode emerges at the antiferromagnetic wavevector $(\ensuremath{\pi},\ensuremath{\pi})$ with a doping-dependent characteristic energy. The superconducting phase is closely related to the lower pseudogap phase by a topological transition with spinon vortices and antivortices forming bound pairs and the emergence of fermionic quasiparticles as holon-spinon-vortex bound objects. A quantitative phase diagram in the parameter space of doping, temperature, and magnetic field is determined. Comparisons with experiments are also made.
We present a formalism for strongly correlated electron systems which consists in a local approximation of the dynamical three-leg interaction vertex. This vertex is self-consistently computed using a quantum impurity model with dynamical interactions in the charge and spin channels, similar to dynamical mean field theory approaches. The electronic self-energy and the polarization are both frequency and momentum dependent. The method interpolates between the spin-fluctuation or GW approximations at weak coupling and the atomic limit at strong coupling. We apply the formalism to the Hubbard model on a two-dimensional square lattice and show that as interactions are increased towards the Mott insulating state, the local vertex acquires a strong frequency dependence, driving the system to a Mott transition, while at low enough temperatures the momentum dependence of the self-energy is enhanced due to large spin fluctuations. Upon doping, we find a Fermi arc in the one-particle spectral function, which is one signature of the pseudogap state.
We apply the recently developed slave fermion approach to study the doped Mott insulator in the one-band Hubbard and Hubbard-Heisenberg models. Our results produce several subtle features in the electron spectra and confirm the key role of antiferromagnetic (AFM) correlations in the appearance of the pseudogap. Upon hole doping, the electron spectra exhibit a single peak near the Fermi energy in the local approximation of the Hubbard model where AFM correlations are not included. When AFM correlations are included through an explicit mean-field Heisenberg interaction, a second peak emerges at slightly lower energy and pushes the other peak to higher energy, so that a pseudogap emerges between the two peaks at small doping. Both peaks grow rapidly with increasing doping and eventually merge together, where the pseudogap no longer exists. Detailed analyses of the spectral evolution with doping and the strength of the Heisenberg interaction confirm that the lower-energy peak comes from a polaronic mechanism due to the holon-spinon interaction in the AFM-correlated background and the higher-energy peak arises from the holon hybridization to form the electron quasiparticles. Thus, the pseudogap arises from the interplay of the polaronic and hybridization mechanisms. Our results are in good agreement with previous numerical calculations using the dynamical mean-field theory and its cluster extensions, but give a clearer picture of the underlying physics. Our work provides a promising perspective for clarifying the nature of doped Mott insulators and may serve as a starting point for more elaborate investigations in the future.