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arXiv:1503.07512 · Physica Scripta

Adiabatic rapid passage two-photon excitation of a Rydberg atom

Elena Kuznetsova, Gengyuan Liu, Svetlana Malinovskaya

Published Apr 1, 2014• 12 citations
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Abstract

We considered the two-photon adiabatic rapid passage excitation of a single atom from the ground to a Rydberg state. Three schemes were analyzed: both pump and Stokes fields chirped and pulsed, only the pump field chirped, and only the pump field pulsed and chirped while the Stokes field is continuous wave (CW). In all three cases high transfer efficiencies > 99% were achieved for the experimentally realizable Rabi frequencies and the pulse durations of the fields.

DOI
10.1088/0031-8949/2014/t160/014024

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We considered the two-photon adiabatic rapid passage excitation of a single atom from the ground to a Rydberg state. Three schemes were analyzed: both pump and Stokes fields chirped and pulsed, only the pump field chirped, and only the pump field pulsed and chirped while the Stokes field is continuous wave (CW). In all three cases high transfer efficiencies > 99% were achieved for the experimentally realizable Rabi frequencies and the pulse durations of the fields.
Abstract We analyze the excitation of two ground state atoms to a double Rydberg state by a two-photon chirped optical pulse in the regime of adiabatic rapid passage (ARP). For intermediate Rydberg–Rydberg interaction strengths relevant for atoms separated by ∼ten μ m, adiabatic excitation can be achieved at experimentally feasible Rabi frequencies and chirp rates of the pulses, resulting in high transfer efficiencies. We also study the adiabatic transfer between ground and Rydberg states as a means to realize a controlled phase gate between atomic qubits.
In an atomic ensemble, quantum information is typically carried as single collective excitations. It is very advantageous if the creation of single excitations is efficient and robust. A Rydberg blockade enables deterministic creation of single excitations via a collective Rabi oscillation by precisely controlling the pulse area, being sensitive to many experimental parameters. In this paper, we implement the adiabatic rapid passage technique to the Rydberg excitation process in a mesoscopic atomic ensemble. We make use of a two-photon excitation scheme with an intermediate state off-resonant and sweep the laser frequency of one excitation laser. We find the chirped scheme preserves internal phases of the collective Rydberg excitation and is more robust against variance of laser intensity and frequency detuning.
The population of atoms in Rydberg states is efficiently transferred with a change in principal quantum number nnn of up to ten via multiphoton adiabatic rapid passage through a single multiphoton resonance using a frequency-chirped microwave pulse. A quantum-mechanical picture of multiphoton adiabatic rapid passage in a one-dimensional atom using a Floquet approach provides a good description of most, but not all, of the observed phenomena.
We have considered a coherent population transfer to a higher excited singlet state ( S2 ) of molecules with anomalous fluorescence in molecular assemblies (e.g., a dense medium). A direct excitation to S2 requires light in the UV region. Because of this, the transition is conveniently realized by a two-step (two-photon) process: S0→S1→S2 , where transitions S0→S1 and S1→S2 correspond to the optical region. We have shown that efficient stimulated Raman adiabatic passage (STIRAP) in the ladder configuration can be realized in this case, using suitably chirped pulses, to compensate a change of the two-photon transition frequency in time, induced by the pulses themselves, due to near dipole-dipole interactions. We have provided a reduced state formulation of the optical control process. Chirping the “pump” pulse that excites transition S0→S1 is nonequivalent to chirping the “Stokes” pulse that excites transition S1→S2 , with respect to the population of the intermediate state ( S1 ) in the pulse nonadiabatic regime. We have also shown that with suitably chirped pulses, efficient STIRAP still persists even for a rather large decay of the intermediate state.
We generalize Stark-chirped rapid adiabatic passage to the case of a multilevel atom.The atom is assumed to have two ground state levels g and f and an excited level e.The adiabatic passage is carried out by resonantly driving the g-e and f -e transitions with time-dependent pump and Stokes fields in the presence of strong far-off-resonant Stark field.Our formalism determines the states that participate in population transfer and is applicable to systems with arbitrary numbers of degenerate states in each level and arbitrary couplings of the g-e and f -e transitions.We give an application to adiabatic passage in Rb atom.
Efficient population transfer by adiabatically chirping through a multiphoton resonance in microwave driven and kicked Rydberg atoms has recently been reported both experimentally and theoretically. Here we report on our simulations in which we have exploited this mechanism to vibrationally excite a diatomic molecule up to |ν = 4, J from the ground state by chirping through a four-photon resonance condition. This is an efficient means of population transfer, which is an alternative to the ladder climbing scheme requiring chirping through a sequence of states in the correct order. We discuss and compare one-dimensional quantum and classical models where there is no rotational degree of freedom. This comparison suggests that for the lowest laser intensity we consider, the process is classically forbidden and the transition occurs through tunnelling. We show that for larger peak intensities, the transfer can be looked upon as a classical transition in phase space, similar to that observed in the atomic case. We extend our simulations to fully three-dimensional quantum calculations and investigate the effect of coupling between different rotational pathways. We finally discuss the effect of thermal averaging over the initial J-states using a temperature for which the first few rotational levels inside the ν = 0 manifold are populated.