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arXiv:1407.6960 · Physical Review A

Phase diagram of dipolar bosons in two dimensions with tilted polarization

A. Macia, Jordi Boronat, Ferran Mazzanti

Published Dec 1, 2014• 32 citations
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Abstract

We analyze the ground state of a system of dipolar bosons moving in the $XY$ plane and such that their dipolar moments are all aligned in a fixed direction in space. We focus on the general case where the polarization field forms a generic angle $\ensuremath{\alpha}$ with respect to the $Z$ axis. We use the path-integral ground-state method to analyze the static properties of the system as both $\ensuremath{\alpha}$ and the density $n$ vary over a wide range where the system is stable. We use the maximum of the static structure function as an order parameter to characterize the different phases and the transition lines among them. We find that, in addition to a superfluid gas and a solid phase, the system reaches a stripe phase at large tilting angles that is entirely induced by the anisotropic character of the interaction. We also show that the quantum phase transition from the gas to the stripe phase is of second order and report approximate values for the critical exponents.

DOI
10.1103/physreva.90.061601

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We analyze the ground state of a system of dipolar bosons moving in the XYXYXY plane and such that their dipolar moments are all aligned in a fixed direction in space. We focus on the general case where the polarization field forms a generic angle \ensuremathα\ensuremath{\alpha}\ensuremathα with respect to the ZZZ axis. We use the path-integral ground-state method to analyze the static properties of the system as both \ensuremathα\ensuremath{\alpha}\ensuremathα and the density nnn vary over a wide range where the system is stable. We use the maximum of the static structure function as an order parameter to characterize the different phases and the transition lines among them. We find that, in addition to a superfluid gas and a solid phase, the system reaches a stripe phase at large tilting angles that is entirely induced by the anisotropic character of the interaction. We also show that the quantum phase transition from the gas to the stripe phase is of second order and report approximate values for the critical exponents.
We present calculations of the ground state and excitations of an anisotropic dipolar Bose gas in two dimensions, realized by a nonperpendicular polarization with respect to the system plane. For sufficiently high density, an increase of the polarization angle leads to a density instability of the gas phase in the direction where the anisotropic interaction is strongest. Using a dynamic many-body theory, we calculate the dynamic structure function in the gas phase which shows the anisotropic dispersion of the excitations. We find that the energy of roton excitations in the strongly interacting direction decreases with increasing polarization angle and almost vanishes close to the instability. Exact path integral ground state Monte Carlo simulations show that this instability is indeed a quantum phase transition to a stripe phase, characterized by long-range order in the strongly interacting direction.
We study the superfluid properties of a system of fully polarized dipolar bosons moving in the XY plane. We focus on the general case where the polarization field forms an arbitrary angle α with respect to the Z axis, while the system is still stable. We use the diffusion Monte Carlo and the path integral ground state methods to evaluate the one-body density matrix and the superfluid fractions in the region of the phase diagram where the system forms stripes. Despite its oscillatory behavior, the presence of a finite large-distance asymptotic value in the s-wave component of the one-body density matrix indicates the existence of a Bose condensate. The superfluid fraction along the stripes direction is always close to 1, while in the Y direction decreases to a small value that is nevertheless different from zero. These two facts confirm that the stripe phase of the dipolar Bose system is a clear candidate for an intrinsic supersolid without the presence of defects as described by the Andreev-Lifshitz mechanism.
Motivated by recent experiments with ultracold magnetic atoms trapped in optical lattices where the orientation of atomic dipoles can be fully controlled by external fields, we study, by means of quantum Monte Carlo, the ground-state properties of dipolar bosons trapped in a two-dimensional lattice with density-induced hopping and where the dipoles are tilted along the xzxzxz plane. We present ground-state phase diagrams of the above system at different tilt angles. We find that as the dipolar interaction increases, the superfluid phase at half-filling factor is destroyed in favor of either a checkerboard or stripe solid phase for tilt angle $\ensuremath{\theta}\ensuremath{\lesssim}{30}^{\ensuremath{\circ}}$ or $\ensuremath{\theta}\ensuremath{\gtrsim}{30}^{\ensuremath{\circ}}$, respectively. More interesting physics happens at tilt angles $\ensuremath{\theta}\ensuremath{\gtrsim}{58}^{\ensuremath{\circ}}$, where we find that as the dipolar interaction strength increases, solid phases first appear at filling factor lower than 0.5. Moreover, unlike what is observed at lower tilt angles, we find that at half filling, a stripe supersolid intervenes between the superfluid and stripe solid phase.
The recent advances in creating nearly degenerate quantum dipolar gases in optical lattices are opening the doors for the exploration of equilibrium physics of quantum systems with anisotropic and long-range dipolar interactions. In this paper we study the zero- and finite-temperature phase diagrams of a system of hard-core dipolar bosons at half-filling, trapped in a two-dimensional square optical lattice. The dipoles are aligned parallel to one another and tilted out of the optical lattice plane by means of an external electric field. At zero-temperature, the system is a superfluid (SF) at all tilt angles θ provided that the strength of dipolar interaction is below a critical value . Upon increasing the interaction strength while keeping θ fixed, the SF phase is destabilized in favor of a checkerboard or a stripe solid (SS) depending on the tilt angle. We explore the nature of the phase transition between the two solid phases, identifying a region of metastable emulsion states intervening between the two solid lobes. Additionally, we study the stability of these quantum phases against thermal fluctuations and find that the SS is the most robust, making it the best candidate for experimental observation.
Recent experimental advances in creating stable dipolar systems, including polar molecules with large electric dipole moments, have led to vigorous theoretical activities. Here we discuss our work on homogeneous 2D dipolar bosons with dipoles oriented at an angle to the direction perpendicular to the confining 2D plane, i.e. for non-zero tilt angles. Using Bogoliubov-de Gennes equations, we obtain T=0 excitation spectrum of the dipolar Bose gas, and explore instabilities at varying tilt angle, density and dipolar coupling. We map out a phase diagram a function of tilt angle, dipole strength and density. We find the development of maxon-roton behavior leading to roton instabilities at large densities for small tilt angles, and at low densities for large tilt angles. The behavior is anisotropic in k-space; accordingly the roton instabilities occur in the k y direction, suggestive of inhomogeneity and stripe phase, with density mode becoming soft in the y direction. Our results compare favorably with existing Quantum Monte Carlo calculations for non-zero tilt angles.
The energy of ultra-dilute quantum many-body systems is known to exhibit a universal dependence on the gas parameter x=n a_0^d x = n a 0 d , with n n the density, d d the dimensionality of the space ( d=1,2,3 d = 1 , 2 , 3 ) and a_0 a 0 the s s -wave scattering length. The universal regime typically extends up to x\approx 0.001 x ≈ 0.001 , while at larger values specific details of the interaction start to be relevant and different model potentials lead to different results. Dipolar systems are peculiar in this regard since the anisotropy of the interaction makes a_0 a 0 depend on the polarization angle \alpha α , so different combinations of n and \alpha α can lead to the same value of the gas parameter x. In this work we analyze the scaling properties of dipolar bosons in two dimensions as a function of the density and polarization dependent scattering length up to very large gas parameter values. Using Quantum Monte Carlo (QMC) methods we study the energy and the main structural and coherence properties of the ground state of a gas of dipolar bosons by varying the density and scattering length for a fixed gas parameter. We find that the dipolar interaction shows relevant scaling laws up to unusually large values of x x that hold almost to the boundaries in the phase diagram where a transition to a stripe phase takes place.