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arXiv:1406.5779 · Physical Review Letters

Scattering in the Ultrastrong Regime: Nonlinear Optics with One Photon

Eduardo Sánchez-Burillo, David Zueco, Juan José García‐Ripoll, Luis Martín-Moreno

Published Dec 31, 2014• 129 citations
arXivHTMLPDF

Abstract

The scattering of a flying photon by a two-level system ultrastrongly coupled to a one-dimensional photonic waveguide is studied numerically. The photonic medium is modeled as an array of coupled cavities and the whole system is analyzed beyond the rotating wave approximation using matrix product states. It is found that the scattering is strongly influenced by the single- and multiphoton dressed bound states present in the system. In the ultrastrong coupling regime a new channel for inelastic scattering appears, where an incident photon deposits energy into the qubit, exciting a photon-bound state, and escaping with a lower frequency. This single-photon nonlinear frequency conversion process can reach up to 50% efficiency. Other remarkable features in the scattering induced by counterrotating terms are a blueshift of the reflection resonance and a Fano resonance due to long-lived excited states.

DOI
10.1103/physrevlett.113.263604

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The scattering of a flying photon by a two-level system ultrastrongly coupled to a one-dimensional photonic waveguide is studied numerically. The photonic medium is modeled as an array of coupled cavities and the whole system is analyzed beyond the rotating wave approximation using matrix product states. It is found that the scattering is strongly influenced by the single- and multiphoton dressed bound states present in the system. In the ultrastrong coupling regime a new channel for inelastic scattering appears, where an incident photon deposits energy into the qubit, exciting a photon-bound state, and escaping with a lower frequency. This single-photon nonlinear frequency conversion process can reach up to 50% efficiency. Other remarkable features in the scattering induced by counterrotating terms are a blueshift of the reflection resonance and a Fano resonance due to long-lived excited states.
Abstract Recent experiments have pushed the studies on atom–photon interactions to the ultrastrong regime, which motivates the exploration of physics beyond the rotation wave approximation. Here we study the single-photon scattering on a system composed of a coupling cavity array with a two-level atom in the center cavity, which, by varying two outside coupling parameters, corresponds to a model from a supercavity (SC) QED to a waveguide QED with counter rotating wave (CRW) interaction. By applying a time-independent scattering theory based on the bound states in the scattering region, we find that the CRW interaction obviously changes the transmission valley even in the weak atom-cavity coupling regime; in particular, the CRW interaction leads to an inelastic scattering process and a Fano-type resonance, which is directly observed in the crossover from the SC-QED case to the waveguide QED case. Predictably, our findings provide the potential of manipulating the CRW effects in realistic systems and pave the way for the numerical study of very general QED systems.
Photon antibunching in the light scattered by single quantum emitters is one of the hallmarks of quantum optics, providing an unequivocal demonstration of the quantized nature of the electromagnetic field. Antibunching can be intuitively understood by the need for a two-level system lying in its lower state after emitting a photon to be re-excited into the upper one before a second emission can take place. Here we show that such a picture breaks down in the ultrastrong light-matter coupling regime, when the coupling strength becomes comparable to the bare emitter frequency. Specialising to the cases of both a natural and a superconducting artificial atom, we thus show that a single emitter coupled to a photonic resonator can emit bunched light. The result presented herein is a clear evidence of how the ultrastrong coupling regime is able to change the nature of individual atoms.
Photon antibunching in the light scattered by single quantum emitters is one of the hallmarks of quantum optics, providing an unequivocal demonstration of the quantized nature of the electromagnetic field. Antibunching can be intuitively understood by the need for a two-level system lying in its lower state after emitting a photon to be re-excited into the upper one before a second emission can take place. Here we show that such a picture breaks down in the ultrastrong light–matter coupling regime, when the coupling strength becomes comparable to the bare emitter frequency. Specializing to the cases of both a natural and an artificial atom, we thus show that a single emitter coupled to a photonic resonator can emit bunched light. The result presented herein is clear evidence of how the ultrastrong coupling regime is able to change the nature of individual atoms.
The propagation of N photons in one dimensional waveguides coupled to M qubits is discussed, both in the strong and ultrastrong qubit-waveguide coupling. Special emphasis is placed on the characterisation of the nonlinear response and its linear limit for the scattered photons as a function of N, M, qubit inter distance and light-matter coupling. The quantum evolution is numerically solved via the matrix product states technique. The time evolutions for both the field and qubits are computed. The nonlinear character (as a function of N/M) depends on the computed observable. While perfect reflection is obtained for N/M≅1, photon-photon correlations are still resolved for ratios N/M=non-zero. Inter-qubit distance enhances the nonlinear response. Moving to the ultrastrong coupling regime, we observe that inelastic processes are robust against the number of qubits and that the qubit-qubit interaction mediated by the photons is qualitatively modified. The theory developed in this work models experiments in circuit QED, photonic crystals and dielectric waveguides.
In this work we study the scattering of pairs of photons by a two-level system ultrastrongly coupled to a one-dimensional waveguide. We describe this problem using a spin-boson model with an Ohmic environment J(ω)=παω1.J(ω)=παω^1.J(ω)=παω1. We show that when coupling strength lays is about α≤1,α\leq 1,α≤1, the dynamics is well approximated by a polaron Hamiltonian, under the approximation of a conserved number of excitations. In this regime, we develop analytical predictions for the single- and two-photon scattering matrix computed with a Green's function method.
The realization of strong nonlinear coupling between single photons has been a long-standing goal in quantum optics and quantum information science, promising wide impact applications, such as all-optical deterministic quantum logic and single-photon frequency conversion. Here, we report an experimental observation of the strong coupling between a single-photon and a two-photon Fock state in an ultrastrongly-coupled circuit-QED system. This strong nonlinear interaction is realized by introducing a detuned flux qubit working as an effective coupler between two modes of a superconducting coplanar waveguide resonator. The ultrastrong light–matter interaction breaks the excitation number conservation, and an external flux bias breaks the parity conservation. The combined effect of the two enables the strong one–two-photon coupling. Quantum Rabi-like avoided crossing is resolved when tuning the two-photon resonance frequency of the first mode across the single-photon resonance frequency of the second mode. Within this new photonic regime, we observe the thresholdless second harmonic generation for a mean photon number below one. Our results represent a key step towards a new regime of quantum nonlinear optics, where individual photons can deterministically and coherently interact with each other in the absence of any stimulating fields. Systems with strong photon-photon interactions enable advanced quantum optical applications as well as the study of highly correlated light-matter states. Here the authors report strong coupling between single- and two-photon states in a superconducting circuit, enabling a new regime of nonlinear quantum optics.