Photon antibunching in the light scattered by single quantum emitters is one of the hallmarks of quantum optics, providing an unequivocal demonstration of the quantized nature of the electromagnetic field. Antibunching can be intuitively understood by the need for a two-level system lying in its lower state after emitting a photon to be re-excited into the upper one before a second emission can take place. Here we show that such a picture breaks down in the ultrastrong light-matter coupling regime, when the coupling strength becomes comparable to the bare emitter frequency. Specialising to the cases of both a natural and a superconducting artificial atom, we thus show that a single emitter coupled to a photonic resonator can emit bunched light. The result presented herein is a clear evidence of how the ultrastrong coupling regime is able to change the nature of individual atoms.
Photon antibunching in the light scattered by single quantum emitters is one of the hallmarks of quantum optics, providing an unequivocal demonstration of the quantized nature of the electromagnetic field. Antibunching can be intuitively understood by the need for a two-level system lying in its lower state after emitting a photon to be re-excited into the upper one before a second emission can take place. Here we show that such a picture breaks down in the ultrastrong light-matter coupling regime, when the coupling strength becomes comparable to the bare emitter frequency. Specialising to the cases of both a natural and a superconducting artificial atom, we thus show that a single emitter coupled to a photonic resonator can emit bunched light. The result presented herein is a clear evidence of how the ultrastrong coupling regime is able to change the nature of individual atoms.
Photon antibunching in the light scattered by single quantum emitters is one of the hallmarks of quantum optics, providing an unequivocal demonstration of the quantized nature of the electromagnetic field. Antibunching can be intuitively understood by the need for a two-level system lying in its lower state after emitting a photon to be re-excited into the upper one before a second emission can take place. Here we show that such a picture breaks down in the ultrastrong light–matter coupling regime, when the coupling strength becomes comparable to the bare emitter frequency. Specializing to the cases of both a natural and an artificial atom, we thus show that a single emitter coupled to a photonic resonator can emit bunched light. The result presented herein is clear evidence of how the ultrastrong coupling regime is able to change the nature of individual atoms.
The scattering of a flying photon by a two-level system ultrastrongly coupled to a one-dimensional photonic waveguide is studied numerically. The photonic medium is modeled as an array of coupled cavities and the whole system is analyzed beyond the rotating wave approximation using matrix product states. It is found that the scattering is strongly influenced by the single- and multiphoton dressed bound states present in the system. In the ultrastrong coupling regime a new channel for inelastic scattering appears, where an incident photon deposits energy into the qubit, exciting a photon-bound state, and escaping with a lower frequency. This single-photon nonlinear frequency conversion process can reach up to 50% efficiency. Other remarkable features in the scattering induced by counterrotating terms are a blueshift of the reflection resonance and a Fano resonance due to long-lived excited states.
Being bosons, photons like to group together, with the behavior of photon bunching described as an attribute of classical light. At the other extreme, photons emitted by a single emitter are expected to antibunch, trickling out of the emitter one at a time. Although bunching and antibunching are well established behaviors of classical and nonclassical light, respectively, the transition between the two has not been observed. It is expected that as the number of emitters is increased, a smooth transition should occur. Using a high-quality cavity into which they can place a variable number of atoms, Hennrich et al. show that they can probe the transition systematically as the number of emitters (atoms in the cavity) is gradually increased. They observe that the antibunching behavior disappears when the average number of atoms in the cavity is one, and they are able to explain the experimental data well if the emitters are assumed to form an independent ensemble. — ISO
In the last decade, the field of Quantum Optics has been enriched with a completely new platform: superconducting quantum circuits, also known as circuit-QED. This platform builds on the original designs of superconducting qubits, that is few-level systems made of superconducting islands and Josephson junctions, but adds to it a new ingredient, microwave photons. In this talk I will review circuit-QED with a focus on two complementary lines of research: ultrastrong light-matter coupling and strongly correlated propagating photons. The first topic deals with novel designs of superconducting qubits, engineering their coupling to the microwave radiation field to reach Rabi frequencies that approach the qubit and photon frequencies. In this regime, known as ”ultrastrong coupling”, the rotating wave approximation from Quantum Optics is no longer valid, the vacuum may spontaneously polarize, producing photons that get bound to the qubit, and novel physics is expected to emerge. I will review recent experiments on this topic, together with various theoretical proposals to tame this ultrastrong coupling. The second topic revolves around the notion of ”propagating” photons in these circuits. Most experiments in circuit-QED so far adopted the typical configuration of artificial atoms (qubits) interacting with artificial cavities (LC resonators). This proved useful in order to reach the strong coupling regime, demonstrating Rabi oscillations and developing a variety of protocols for quantum information, tomograhy, entanglement, etc. However, recent experiments have shown that it is possible to also work with propagating photons, replacing the LC resonators with open transmission lines, and studying the scattering properties of those artificial atoms. In this context we have worked on developing new technology to detect and control these photons, engineering single-photon detectors, quantum metamaterials and photonic crystals, or even new nonlinear media based on coupled cavities.
The prototypical system constituted by a two-level atom interacting with a quantized single-mode electromagnetic field is described by the quantum Rabi model (QRM). The QRM is potentially valid at any light-matter interaction regime, ranging from the weak (where the decay rates exceeds the coupling rate) to the deep strong coupling (where the interaction rate exceeds the bare transition frequencies of the subsystems). However, when reaching the ultrastrong coupling regime, several theoretical issues may prevent the correct description of the observable dynamics of such a system: (i) the standard quantum optics master equation fails to correctly describe the interaction of this system with the reservoirs; (ii) the correct output photon rate is no longer proportional to the intracavity photon number; and (iii) they appear to violate gauge invariance. Here, we study the photon flux emission rate of this system under the incoherent excitation of the two-level atom for any light-matter interaction strength and consider different effective temperatures. The dependence of the emission spectra on the coupling strength is the result of the interplay between energy levels, matrix elements of the observables, and the density of states of the reservoirs. Within this approach, we also study the occurrence of light-matter decoupling in the deep strong-coupling regime and show how all of the obtained results are gauge invariant.
The photon statistics of the light emitted from an atomic ensemble into a single field mode of an optical cavity is investigated as a function of the number of atoms. The light is produced in a Raman transition driven by a pump laser and the cavity vacuum, and a recycling laser is employed to repeat this process continuously. For weak driving, a smooth transition from antibunching to bunching is found for about one intracavity atom. Remarkably, the bunching peak develops within the antibunching dip. The observed behavior is well explained by a model describing an ensemble of independent emitters.