The propagation of N photons in one dimensional waveguides coupled to M qubits is discussed, both in the strong and ultrastrong qubit-waveguide coupling. Special emphasis is placed on the characterisation of the nonlinear response and its linear limit for the scattered photons as a function of N, M, qubit inter distance and light-matter coupling. The quantum evolution is numerically solved via the matrix product states technique. The time evolutions for both the field and qubits are computed. The nonlinear character (as a function of N/M) depends on the computed observable. While perfect reflection is obtained for N/M≅1, photon-photon correlations are still resolved for ratios N/M=non-zero. Inter-qubit distance enhances the nonlinear response. Moving to the ultrastrong coupling regime, we observe that inelastic processes are robust against the number of qubits and that the qubit-qubit interaction mediated by the photons is qualitatively modified. The theory developed in this work models experiments in circuit QED, photonic crystals and dielectric waveguides.
The propagation of N photons in one dimensional waveguides coupled to M qubits is discussed, both in the strong and ultrastrong qubit-waveguide coupling. Special emphasis is placed on the characterisation of the nonlinear response and its linear limit for the scattered photons as a function of N, M, qubit inter distance and light-matter coupling. The quantum evolution is numerically solved via the matrix product states technique. The time evolutions for both the field and qubits are computed. The nonlinear character (as a function of N/M) depends on the computed observable. While perfect reflection is obtained for N/M≅1, photon-photon correlations are still resolved for ratios N/M=non-zero. Inter-qubit distance enhances the nonlinear response. Moving to the ultrastrong coupling regime, we observe that inelastic processes are robust against the number of qubits and that the qubit-qubit interaction mediated by the photons is qualitatively modified. The theory developed in this work models experiments in circuit QED, photonic crystals and dielectric waveguides.
Strong coupling between light and matter has been demonstrated both in classical cavity quantum electrodynamics (QED) systems and in more recent circuit-QED experiments. This enables the generation of strong nonlinear photon-photon interactions at the single-photon level, which is of great interest for the observation of quantum nonlinear optical phenomena, the control of light quanta in quantum information protocols such as quantum networking, as well as the study of strongly correlated quantum many-body systems using light. Recently, strong coupling has also been realized in a variety of one-dimensional (1D) waveguide- QED experimental systems, which in turn makes them promising candidates for quantum information processing. Compared to cavity-QED systems, there are two new features in waveguide-QED: the existence of a continuum of states and the restricted 1D phase space, which together bring in new physical effects, such as the bound-state effects. This thesis consists of two parts: 1) understanding the fundamental interaction between local quantum objects, such as two-level systems and four-level systems, and photons confined in the waveguide; 2) exploring its implications in quantum information processing, in particular photonic quantum computation and quantum key distribution. First, we demonstrate that by coupling a two-level system (TLS) or three/fourlevel system to a 1D continuum, strongly-correlated photons can be generated inside the waveguide. Photon-photon bound states, which decay exponentially as a function of the relative coordinates of photons, appear in multiphoton scattering processes. As a result, photon bunching and antibunching can be observed in the photon-photon correlation function, and nonclassical light source can be generated on demand. In the case of an N-type four-level system, we show that the effective photon-photon interaction mediated by the four-level system, gives rise to a variety of nonlinear optical phenomena, including photon blockade, photon-induced tunneling, and creation of single-photon states and photon pairs with a high degree of spectral entanglement, all in the absence of a cavity. However, to enable greater quantum networking potential using waveguide- QED, it is important to study systems having more than just one TLS/qubit. We develop a numerical Green function method to study cooperative effects in a system of two qubits coupled to a 1D waveguide. Quantum beats emerge in photon-photon correlations, and persist to much longer time scales because of non-Markovian processes. In addition, this system can be used to generate a high-degree of long-distance entanglement when one of the two qubits is driven by an on-resonance laser, further paving the way toward waveguide-QED-based quantum networks. Furthermore, based on our study of light-matter interactions in waveguide- QED, we investigate its implications in quantum information processing. First, we study quantum key distribution using the sub-Possonian single photon source obtained by scattering a coherent state off a two-level system. The rate for key generation is found to be twice as large as for other sources. Second, we propose a new scheme for scalable quantum computation using flying qubits--propagating photons in a one-dimensional waveguide--interacting with matter qubits. Photonphoton interactions are mediated by the coupling to a three- or four-level system, based on which photon-photon -phase gates (Controlled-NOT) can be implemented for universal quantum computation. We show that high gate fidelity is possible given recent dramatic experimental progress in superconducting circuits and photonic-crystal waveguides. The proposed system can be an important building block for future on-chip quantum networks.
The study of waveguide-QED systems, where a continuum of quantum field modes is coupled to qubits or two-level systems, has improved our ability to manipulate quantum light-matter interactions on chip. In the typical theoretical approaches to waveguide QED, there are a few necessary approximations, e.g., considering the system in the weak excitation regime, or treating the waveguide as a bath. However, these inherent approximations can break down with short pulse excitation. Here, we investigate the few-photon quantum nonlinear response of chiral qubits, when excited with one and two-photon Fock states. Our theory uses a numerically exact approach, based on Matrix Product States, avoiding the limitations of the usual waveguide-QED approximations. Using a chiral-emitter waveguide system, we show explicitly the breakdown of the weak excitation approximation, and study the single and two-photon nonlinear responses. We demonstrate the impact on the qubit population, and discuss how the phase change can be examined from the photon quantum correlation functions, seeing a radical departure from scattering theory solutions.
Quantum nonlinear optics seeks to harness strong photon-photon interactions for scalable quantum technologies, although dissipative losses still pose a major barrier to near-unity conversion efficiency. Here, we bridge non-Hermitian physics with the quantum nonlinear domain by exploiting perfect absorption to identify and optimize few-photon nonlinear processes. We theoretically investigate two circuit QED systems, operating in the light-matter ultrastrong coupling regime. The first (i) enables simultaneous two-atom excitations by single photons, while the second (ii) realizes the strong coupling between a single-photon and a two-photon Fock states. We demonstrate that, since the strong optical nonlinearities cause quantum spectral features to emerge already at the level of linear response theory, the perfect absorption condition in ∣S11∣ enables near-deterministic single-photon down-conversion into (i) a qubit-qubit-correlated pair and (ii) a two-photon pair. We show that the conversion efficiency can be systematically optimized through experimentally accessible parameters, both linked to the emergence of Hermitian subspaces within the effective non-Hermitian Hamiltonians. These findings position non-Hermitian engineering as a broadly applicable route to optimizing quantum devices at the single-photon level, even beyond circuit-QED platforms.
The scattering of a flying photon by a two-level system ultrastrongly coupled to a one-dimensional photonic waveguide is studied numerically. The photonic medium is modeled as an array of coupled cavities and the whole system is analyzed beyond the rotating wave approximation using matrix product states. It is found that the scattering is strongly influenced by the single- and multiphoton dressed bound states present in the system. In the ultrastrong coupling regime a new channel for inelastic scattering appears, where an incident photon deposits energy into the qubit, exciting a photon-bound state, and escaping with a lower frequency. This single-photon nonlinear frequency conversion process can reach up to 50% efficiency. Other remarkable features in the scattering induced by counterrotating terms are a blueshift of the reflection resonance and a Fano resonance due to long-lived excited states.
Harnessing the interaction between light and matter at the quantum level has been a central theme in atomic physics and quantum optics, with applications from quantum computation to quantum metrology. Combining complex interactions with photonic synthetic materials provides an opportunity to investigate novel quantum phases and phenomena, establishing interesting connections to condensed matter physics. Here we explore many-body phenomena with a single artificial atom coupled to the many discrete modes of a photonic crystal. This experiment reaches the ultrastrong light-matter coupling regime using the circuit quantum electrodynamics paradigm, by galvanically coupling a highly nonlinear fluxonium qubit to a tight-binding lattice of microwave resonators. In this regime, the transport of a single photon becomes a many-body problem, owing to the strong participation of multi-photon bound states arising from interactions that break particle number conservation. Exploiting the effective photon-photon interactions mediated by the qubit, the transport of multiple photons leads to complex multimode dynamics that can be employed for generating a continuous reservoir of strongly-correlated photons, an important resource for quantum networks. This work opens exciting prospects for exploring nonlinear quantum optics at the single-photon level and stabilizing entangled many-body phases of light.
Waveguide quantum electrodynamics (waveguide QED) describes the interaction between an electromagnetic field confined to a one-dimensional waveguide with atom-like quantum emitters close by. The characteristics of these kinds of systems are the possibility for strong and even ultrastrong interactions between the photonic and atom-like systems, and practically infinite range interactions between the emitters. These properties are valuable for a wide range of quantum optical applications, like quantum communication, quantum networks and quantum metrology. In this thesis we focus on two challenges in quantum optics, namely the generation and scattering of multiphoton states. In the first part of this thesis we demonstrate how waveguide QED systems can be exploited for the generation of multiphoton states, in particular of single-mode Fock states and superpositions thereof as well as multi-mode photonic states with metrological applications. The basic setup for this goal is an ensemble of quantum emitters coupled to a waveguide. In the so-called atomic mirror configuration symmetric Dicke states (or a superposition thereof) decay superradiantly to the ground state and emit the desired multiphoton state, which can be efficiently collected at the ends of the waveguide. We propose various protocols for the preparation of these Dicke states in waveguide QED systems and characterize the emitted photonic state. It turns out that in the low excitation regime, that is, if the number of photons is much lower than the ensemble size, the photonic state is emitted into a single mode. This single-mode structure is fundamental to current proposals for applications in quantum metrology with optical interferometers. Outside the low excitation regime, a multi-mode photonic state is generated, for which the metrological capabilities were unknown. We were able to show that these states still lead to quantum-enhanced optical interferometry. In the second part of this thesis we demonstrate how the scattering of multiphoton states on a single quantum emitter coupled to the waveguide can be used for testing the limits of the light-matter interaction strength. In particular, we investigate systems in the so-called ultrastrong coupling regime, where the coupling strength between the photonic and atom-like system is of the order of the emitter's transition energy. In this regime, many methods and approximations used in quantum optics, especially the Rotating Wave Approximation, break down and one needs to develop new analytical and numerical methods to study these systems. One approach is the so-called polaron Transformation. We show how this transformation can be applied for predicting the scattering amplitude of few photons scattering on the emitter. The comparison of these results with numerical simulations using matrix product states shows a good agreement for moderate coupling strengths. Both parts together show that waveguide QED systems are promising candidates for the generation of multiphoton states as well as for the investigation of fundamental limits probed through the scattering of multiphoton states. The latter also finds application in the implementation of photon-photon nonlinearities induced by the interaction with the quantum emitters. Apart from these and many other theoretical predictions, waveguide QED systems are also undergoing rapid progress in experiments. Therefore, we expect these kinds of systems to bring forth several advances in the field of quantum optics.