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arXiv:1309.4707 · Journal of Physics Conference Series

Emergent granularity and pseudogap near the superconductor-insulator transition

Nandini Trivedi, Yen Lee Loh, Karim Bouadim, Mohit Randeria

Published Jul 30, 2012• 19 citations
arXivHTMLPDF

Abstract

In two dimensions there is a direct superconductor-to-insulator quantum phase transition driven by increasing disorder. We elucidate, using a combination of inhomogeneous mean field theory and quantum Monte Carlo techniques, the nature of the phases and the mechanism of the transition. We make several testable predictions specifically for local spectroscopic probes. With increasing disorder, the system forms superconducting blobs on the scale of the coherence length embedded in an insulating matrix. In the superconducting state, the phases on the different blobs are coherent across the system whereas in the insulator long range phase coherence is disrupted by quantum fluctuations. As a consequence of this emergent granularity, we show that the single-particle energy gap in the density of states survives across the transition, but coherence peaks exist only in the superconductor. A characteristic pseudogap persists above the critical disorder and critical temperature, in contrast to conventional theories. Surprisingly, the insulator has a two-particle gap scale that vanishes at the SIT, despite a robust single-particle gap.

DOI
10.1088/1742-6596/376/1/012001

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In two dimensions there is a direct superconductor-to-insulator quantum phase transition driven by increasing disorder. We elucidate, using a combination of inhomogeneous mean field theory and quantum Monte Carlo techniques, the nature of the phases and the mechanism of the transition. We make several testable predictions specifically for local spectroscopic probes. With increasing disorder, the system forms superconducting blobs on the scale of the coherence length embedded in an insulating matrix. In the superconducting state, the phases on the different blobs are coherent across the system whereas in the insulator long range phase coherence is disrupted by quantum fluctuations. As a consequence of this emergent granularity, we show that the single-particle energy gap in the density of states survives across the transition, but coherence peaks exist only in the superconductor. A characteristic pseudogap persists above the critical disorder and critical temperature, in contrast to conventional theories. Surprisingly, the insulator has a two-particle gap scale that vanishes at the SIT, despite a robust single-particle gap.
It is well known that the metal-insulator transition in two dimensions for non-interacting fermions takes place at infinitesimal disorder. In contrast, the superconductor-to-insulator transition takes place at a finite critical disorder (on the order of Vc ~ 2t), where V is the typical width of the distribution of random site energies and t is the hopping scale. In this article we compare the localization/delocalization properties of one and two particles. Whereas the metal-insulator transition is a consequence of single-particle Anderson localization, the superconductor-insulator transition (SIT) is due to pair localization – or, alternatively, fluctuations of the phase conjugate to pair density. The central question we address is how superconductivity emerges from localized single-particle states. We address this question using inhomogeneous mean field theory and quantum Monte Carlo techniques and make several testable predictions for local spectroscopic probes across the SIT. We show that with increasing disorder, the system forms superconducting blobs on the scale of the coherence length embedded in an insulating matrix. In the superconducting state, the phases on the different blobs are coherent across the system whereas in the insulator long-range phase coherence is disrupted by quantum fluctuations. As a consequence of this emergent granularity, we show that the single-particle energy gap in the density of states survives across the transition, but coherence peaks exist only in the superconductor. A characteristic pseudogap persists above the critical disorder and critical temperature, in contrast to conventional theories. Surprisingly, the insulator has a two-particle gap scale that vanishes at the SIT despite a robust single-particle gap.
We show, using a Bogoliubov-de Gennes (BdG) mean field theory, that the local pairing amplitude Δ(r) becomes highly inhomogeneous with increasing disorder in an s-wave superconductor. The probability distribution P(Δ) is peaked about the BCS value at low disorder, but with increasing disorder, progressively develops into a broad distribution with significant build up of weight near Δ≈0. At high disorder, the system is found to form superconducting "islands" separated by a non-superconducting sea. Surprisingly, a finite energy gap persists into the highly disordered state in spite of many sites having negligible pairing amplitude and is understood in detail within the BdG framework. Once the pairing amplitude becomes inhomogeneous, the role of quantum phase fluctuations becomes crucial in driving a superconductor-insulator transition at a critical disorder. The insulator is unusual as it has a finite gap for all disorder strengths in marked contrast to the Anderson insulator in non-interacting systems. We treat the phase fluctuations within a self consistent harmonic approximation and obtain the superfluid stiffness as a function of disorder, which agrees well with our earlier quantum Monte Carlo studies.
The pseudogap state of cuprate high-temperature superconductors has been often viewed as either a yet unknown competing order or a precursor state to superconductivity. While awaiting the resolution of the pseudogap problem in cuprates, we demonstrate that local pairing fluctuations, vortex liquid dynamics, and other precursor phenomena can emerge quite generally whenever fermionic excitations remain gapped across the superconducting transition, regardless of the gap origin. Our choice of a tractable model is a lattice band insulator with short-range attractive interactions between fermions in the sss-wave channel. An effective crossover between Bardeen-Cooper-Schrieffer (BCS) and Bose-Einstein condensate (BEC) regimes can be identified in any band insulator above two dimensions, while in two dimensions only the BEC regime exists. The superconducting transition is ``unconventional'' (non-pair-breaking) in the BEC regime, identified by either the bosonic mean field or XY\mathit{XY}XY universality class. The insulator adjacent to the superconductor in the BEC regime is a bosonic Mott insulator of Cooper pairs, which may be susceptible to charge density wave ordering. We construct a function of the many-body excitation spectrum whose nonanalytic changes define a sharp distinction between band and Mott insulators. The corresponding ``second-order transition'' can be observed out of equilibrium by driving a Cooper pair laser in the Mott insulator. We explicitly show that the gap for charged bosonic excitations lies below the threshold for Cooper pair breakup in any BEC regime, despite quantum fluctuations. Our discussion ends with a view of possible consequences for cuprates, where antinodal pair dynamics has certain features in common with our simple sss-wave picture.
We calculate the dynamical conductivity σðωÞ and the bosonic (pair) spectral function PðωÞ from quantum Monte Carlo simulations across clean and disorder-driven superconductor-insulator transitions (SITs).We identify characteristic energy scales in the superconducting and insulating phases that vanish at the transition due to enhanced quantum fluctuations, despite the persistence of a robust fermionic gap across the SIT.Disorder leads to enhanced absorption in σðωÞ at low frequencies compared to the SIT in a clean system.Disorder also expands the quantum critical region, due to a change in the universality class, with an underlying T ¼ 0 critical point with a universal low-frequency conductivity σ Ã ≃ 0.5ð4e 2 =hÞ.
We study the phase fluctuations in the normal state of generic two-dimensional superconducting systems with sss-wave pairing. The effect of phase fluctuations of the pairing fields can be dealt with perturbatively using disorder averaging, after we treat the local superconducting order parameter as a static disordered background. It is then confirmed that the phase fluctuations above the two-dimensional Berezinskii-Kosterlitz-Thouless transition lead to a significant broadening of the single-particle spectrum, giving birth to the pseudogap phenomenon. Quantitatively, the broadening of spectral weights near the BCS gap is characterized by the ratio of the superconducting coherence length and the spatial correlation length of the superconducting pairing order parameter. Our results are tested on the fermionic attractive-UUU Hubbard model on the square lattice, using the unbiased determinant quantum Monte Carlo method and stochastic analytic continuation.
We study the superconductor-insulator transition (SIT) in ddd-wave superconducting ultrathin films. By means of the kernel polynomial method, the Bogoliubov-de Gennes equations are solved for square lattices with up to 360×360360\times 360360×360 unit cells self-consistently, making it possible to observe fully the nanoscale spatial fluctuations of the superconducting order parameters and discriminate accurately the localized quasiparticle states from the extended ones by the lattice-size scaling of the generalized inverse participation ratio. It is shown that Anderson localization can not entirely inhibit the occurrence of the local superconductivity in strongly-disordered ddd-wave superconductors. Separated by an insulating 'sea' completely, a few isolated superconducting 'islands' with significant enhancement of the local superconducting order parameters can survive across the SIT. The disorder-driven SIT, therefore, is a transition from a ddd-wave superconductor to a Bose insulator which consists of localized Cooper pairs. Unlike an sss-wave superconductor which presents a robust single-particle gap across the SIT, the optical conductivity of a ddd-wave superconductor reveals a gapless insulating phase, where the SIT can be detected by observing the disappearance of the Drude weight with the increasing disorder.