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arXiv:1310.1073 · Physical Review X

Dynamical Conductivity across the Disorder-Tuned Superconductor-Insulator Transition

Mason Swanson, Yen Lee Loh, Mohit Randeria, Nandini Trivedi

Published Apr 9, 2014• 58 citations
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Abstract

We calculate the dynamical conductivity σðωÞ and the bosonic (pair) spectral function PðωÞ from quantum Monte Carlo simulations across clean and disorder-driven superconductor-insulator transitions (SITs).We identify characteristic energy scales in the superconducting and insulating phases that vanish at the transition due to enhanced quantum fluctuations, despite the persistence of a robust fermionic gap across the SIT.Disorder leads to enhanced absorption in σðωÞ at low frequencies compared to the SIT in a clean system.Disorder also expands the quantum critical region, due to a change in the universality class, with an underlying T ¼ 0 critical point with a universal low-frequency conductivity σ Ã ≃ 0.5ð4e 2 =hÞ.

DOI
10.1103/physrevx.4.021007

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We calculate the dynamical conductivity σðωÞ and the bosonic (pair) spectral function PðωÞ from quantum Monte Carlo simulations across clean and disorder-driven superconductor-insulator transitions (SITs).We identify characteristic energy scales in the superconducting and insulating phases that vanish at the transition due to enhanced quantum fluctuations, despite the persistence of a robust fermionic gap across the SIT.Disorder leads to enhanced absorption in σðωÞ at low frequencies compared to the SIT in a clean system.Disorder also expands the quantum critical region, due to a change in the universality class, with an underlying T ¼ 0 critical point with a universal low-frequency conductivity σ Ã ≃ 0.5ð4e 2 =hÞ.
We investigate the disorder-driven superconductor to insulator quantum phase transition (SIT) in an interacting fermion model using determinantal quantum Monte Carlo (QMC) methods. The disordered superconductor is modeled by an attractive Hubbard model with site disorder chosen randomly from a uniform distribution. The superconducting state which exists for small disorder is shown to evolve into an insulating phase beyond a critical disorder. The transition is tracked by the vanishing of (a) the superfluid stiffness, and (b) the charge stiffness or the delta function peak in the optical conductivity at zero frequency. We also show the behavior of the charge, spin, pair, and current correlations in the presence of disorder. Results for the temperature dependence of the dc conductivity, obtained by an approximate analytic continuation technique, are also presented both in the metallic phase above Tc{T}_{c}Tc​ and the insulating phase. We discuss some of the complications in extracting the resistance at the transition point.
It is well known that the metal-insulator transition in two dimensions for non-interacting fermions takes place at infinitesimal disorder. In contrast, the superconductor-to-insulator transition takes place at a finite critical disorder (on the order of Vc ~ 2t), where V is the typical width of the distribution of random site energies and t is the hopping scale. In this article we compare the localization/delocalization properties of one and two particles. Whereas the metal-insulator transition is a consequence of single-particle Anderson localization, the superconductor-insulator transition (SIT) is due to pair localization – or, alternatively, fluctuations of the phase conjugate to pair density. The central question we address is how superconductivity emerges from localized single-particle states. We address this question using inhomogeneous mean field theory and quantum Monte Carlo techniques and make several testable predictions for local spectroscopic probes across the SIT. We show that with increasing disorder, the system forms superconducting blobs on the scale of the coherence length embedded in an insulating matrix. In the superconducting state, the phases on the different blobs are coherent across the system whereas in the insulator long-range phase coherence is disrupted by quantum fluctuations. As a consequence of this emergent granularity, we show that the single-particle energy gap in the density of states survives across the transition, but coherence peaks exist only in the superconductor. A characteristic pseudogap persists above the critical disorder and critical temperature, in contrast to conventional theories. Surprisingly, the insulator has a two-particle gap scale that vanishes at the SIT despite a robust single-particle gap.
In contrast to the case of free fermions which have all states localized in two dimensions, dirty, repulsively-interacting bosons exhibit a zero-temperature localization phase transition between superconducting and insulating states as disorder is increased. The conductivity σ* = g (2 e ) 2 / h at the quantum critical point is a universal critical amplitude analogous to the universal jump in superfluid density at the classical Kosterlitz-Thouless transition. Using numerical Monte Carlo methods we compute the value of g for disorder-tuned transitions with and without long-range Coulomb interactions. We argue that this model is relevant to experiments on superconducting thin films and Josephson junction arrays.
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In this article we study superconductor-insulator transitions within the general framework of an attractive Hubbard model. This is a well-defined model of s-wave superconductivity which permits different tuning parameters (disorder and field). Furthermore, it allows a comparison of various analytical and computational approaches in order to gain a complete understanding of the various effects of amplitude and phase fluctuations. We present a systematic pedagogical approach, aiming to equip the lay reader with enough apparatus to be able to understand the numerical calculations, reproduce some of the simpler results, and be able to tackle future problems related to inhomogeneous phases. We go into considerable detail on mean-field theory (MFT) and the Bogoliubov-de Gennes (BdG) approach, as these are a first line of attack which can capture much of the physics, but we also outline cases where this fails to capture phase fluctuations and more sophisticated Quantum Monte Carlo (QMC) calculations are necessary. We discuss the behavior of many observables, including densities of states, superfluid stiffness, and dynamical conductivity, for the disorder-tuned superconductor-insulator transition. We also discuss SITs tuned by parallel magnetic field, which are quite different due to pairbreaking.
We study the superconductor-insulator transition (SIT) in ddd-wave superconducting ultrathin films. By means of the kernel polynomial method, the Bogoliubov-de Gennes equations are solved for square lattices with up to 360×360360\times 360360×360 unit cells self-consistently, making it possible to observe fully the nanoscale spatial fluctuations of the superconducting order parameters and discriminate accurately the localized quasiparticle states from the extended ones by the lattice-size scaling of the generalized inverse participation ratio. It is shown that Anderson localization can not entirely inhibit the occurrence of the local superconductivity in strongly-disordered ddd-wave superconductors. Separated by an insulating 'sea' completely, a few isolated superconducting 'islands' with significant enhancement of the local superconducting order parameters can survive across the SIT. The disorder-driven SIT, therefore, is a transition from a ddd-wave superconductor to a Bose insulator which consists of localized Cooper pairs. Unlike an sss-wave superconductor which presents a robust single-particle gap across the SIT, the optical conductivity of a ddd-wave superconductor reveals a gapless insulating phase, where the SIT can be detected by observing the disappearance of the Drude weight with the increasing disorder.