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arXiv:2212.05737 · Physical review. B./Physical review. B

Phase fluctuations in two-dimensional superconductors and pseudogap phenomenon

Xu-Cheng Wang, Yang Qi

Published Jun 1, 2023• 16 citations
arXivHTMLPDF

Abstract

We study the phase fluctuations in the normal state of generic two-dimensional superconducting systems with $s$-wave pairing. The effect of phase fluctuations of the pairing fields can be dealt with perturbatively using disorder averaging, after we treat the local superconducting order parameter as a static disordered background. It is then confirmed that the phase fluctuations above the two-dimensional Berezinskii-Kosterlitz-Thouless transition lead to a significant broadening of the single-particle spectrum, giving birth to the pseudogap phenomenon. Quantitatively, the broadening of spectral weights near the BCS gap is characterized by the ratio of the superconducting coherence length and the spatial correlation length of the superconducting pairing order parameter. Our results are tested on the fermionic attractive-$U$ Hubbard model on the square lattice, using the unbiased determinant quantum Monte Carlo method and stochastic analytic continuation.

DOI
10.1103/physrevb.107.224502

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We study the phase fluctuations in the normal state of generic two-dimensional superconducting systems with sss-wave pairing. The effect of phase fluctuations of the pairing fields can be dealt with perturbatively using disorder averaging, after we treat the local superconducting order parameter as a static disordered background. It is then confirmed that the phase fluctuations above the two-dimensional Berezinskii-Kosterlitz-Thouless transition lead to a significant broadening of the single-particle spectrum, giving birth to the pseudogap phenomenon. Quantitatively, the broadening of spectral weights near the BCS gap is characterized by the ratio of the superconducting coherence length and the spatial correlation length of the superconducting pairing order parameter. Our results are tested on the fermionic attractive-UUU Hubbard model on the square lattice, using the unbiased determinant quantum Monte Carlo method and stochastic analytic continuation.
The effect of random on-site disorder on s-wave (BCS) superconductors described by a two dimensional negative-U Hubbard model is studied using Bogoliubov-de Gennes (BdG) method. The mean field pairing amplitudes become spatially inhomogeneous at large values of disorder where the system breaks up into superconducting islands with large pairing amplitudes, separated by insulating strips. The amplitude fluctuations are correctly accounted for via BdG calculations, however it misses phase fluctuations which are inherent to low dimensions. The phase fluctuations affect superconducting properties strongly, and the effect is more pronounced in the limit of large disorder. We provide a close estimate of the actual transition temperature, Tcby incorporating phase fluctuations about the inhomogeneous BdG state. This is obtained by relating the jump in renormalized Ds(obtained from a self consistent Harmonic approximation on a phase-only Hamiltonian) at the Kosterlitz-Thouless (KT) transition and the KT transition temperature, TKTobtained from Ds(T) = (2/π)TKTas temperature tends to TKTfrom below. This yields opening of a large region sandwiched between [Formula: see text] (obtained by the vanishing of [Formula: see text]) and TKTwhere there is no phase coherence between the pairs, however amplitude correlations continue to exist, reminiscent of a pseudogap phase in high-Tcsuperconductors which is marked by short ranged preformed pairs without any definite phase relation between them. Further, the appearance of the superconducting islands from a homogeneous phase indicates the evolution of a system consisting of large and overlapping pairs to one that contains short and tightly bound pairs - a scenario termed as BCS-BEC crossover. We have investigated in details the crossover phenomenon as a function of disorder and confirmed it's existence at small values of electron concentration, however, absent at larger densities.
This paper addresses the transition from the normal to the superfluid state in strongly correlated two dimensional fermionic superconductors and Fermi gases. We arrive at the Berezinskii-Kosterlitz-Thouless (BKT) temperature TBKTT_{\text{BKT}}TBKT​ as a function of \emph{attractive} pairing strength by associating it with the onset of quasi-condensation in the normal phase. Our approach builds on a criterion for determining the BKT transition temperature for atomic gases which is based on a well established Quantum Monte Carlo analysis of the phase space density. This latter quantity, when derived from BCS-BEC crossover theory for fermions, leads to non-monotonic behavior for TBKTT_{\text{BKT}}TBKT​ as a function of the attractive interaction or inverse scattering length. In Fermi gases, this implies a robust superconducting dome followed by a long tail from the flat BEC asymptote, rather similar to what is observed experimentally. For lattice systems we find that TBKTT_{\text{BKT}}TBKT​ has an absolute maximum of the order of 0.1EF0.1 E_F0.1EF​. We discuss how our results compare with those derived from the Nelson Kosterlitz criterion based on the mean field superfluid density and the approach to the transition from below. While there is agreement in the strict mean-field BCS regime at weak coupling, we find that at moderate pairing strength bosonic excitations cause a substantial increase in TBKTT_\text{BKT}TBKT​ followed by an often dramatic decrease before the system enters the BEC regime.
The two-dimensional attractive Hubbard model is studied in the weak-to-intermediate-coupling regime by employing a nonperturbative approach. It is shown that this approach is in quantitative agreement with Monte Carlo calculations for both single-particle and two-particle quantities. Both the density of states and the single-particle spectral weight show a pseudogap at the Fermi energy below some characteristic temperature T∗,{T}^{*},T∗, also in good agreement with quantum Monte Carlo calculations. The pseudogap is caused by critical pairing fluctuations in the low-temperature renormalized classical regime $(\ensuremath{\Elzxh}\ensuremath{\omega}<{k}_{B}T)$ of the two-dimensional system. With increasing temperature the spectral weight fills in the pseudogap instead of closing it, and the pseudogap appears earlier in the density of states than in the spectral function. Small temperature changes around T∗{T}^{*}T∗ can modify the spectral weight over frequency scales much larger than temperature. Several qualitative results for the s-wave case should remain true for d-wave superconductors.
We investigate single-particle excitations and strong-coupling effects in a twodimensional Fermi gas. Including pairing fluctuations within a Gaussian fluctuation theory, we calculate the density of states ρ ( ω ) near the Berezinskii-Kosterlitz-Thouless (BKT) transition temperature T BKT . Near T BKT , we show that superfluid fluctuations induce a pseudogap in ρ (ω). The pseudogap structure is very similar to the BCS superfluid density of states, although the superfluid order parameter is absent in the present two-dimensional case. Since a twodimensional 40 K Fermi gas has recently been realized, our results would contribute to the understanding of single-particle properties near the BKT instability.
We theoretically investigate strong-coupling properties of a two-dimensional Fermi gas in the normal phase. Including pairing fluctuations within the framework of a self-consistent T -matrix approximation, we calculate the single-particle density of states (DOS) near the observed Berezinskii-Kosterlitz-Thouless phase transition temperature T BKT . We show that the pseudogap phenomenon associated with strong pairing fluctuations appears as an almost fully gapped single-particle density of states in the strong-coupling regime, indicating that amplitude fluctuations of the order parameter are almost absent and the system is dominated by phase fluctuations of the order parameter, as expected in a two-dimensional system near T BKT . On the other hand, although pairing fluctuations are enhanced by the low-dimensionality of the system, they are found to be still not strong enough to open such a full gap in the intermediate coupling (crossover) regime. In this regime, a dip structure is only seen in DOS around ω = 0, indicating that amplitude of the superfluid order parameter is also fluctuating, in addition to phase fluctuations. In theoretically determining T BKT in a two-dimensional Fermi gas, it is frequently assumed that, while phase fluctuations exist, the amplitude of the superfluid order parameter is fixed. However, our results indicate the necessity of including both amplitude and phase fluctuations of the order parameter in evaluating T BKT in the crossover region. Since the BKT phase transition has recently been reported in a two-dimensional 6 Li Fermi gas, our results would be useful for the theoretical study of this observed novel Fermi superfluid and effects of strong low-dimensional pairing fluctuations.
Abstract This paper addresses the transition from the normal to the superfluid state in strongly correlated two dimensional fermionic superconductors and Fermi gases. We arrive at the Berezinskii–Kosterlitz–Thouless (BKT) temperature T BKT as a function of attractive pairing strength by associating it with the onset of ‘quasi-condensation’ in the normal phase. Our approach builds on a criterion for determining the BKT transition temperature for atomic gases which is based on a well established quantum Monte Carlo analysis of the phase space density. This latter quantity, when derived from BCS–BEC crossover theory for fermions, leads to non-monotonic behavior for T BKT as a function of the attractive interaction or inverse scattering length. In Fermi gases, this implies a robust superconducting dome followed by a long tail from the flat BEC asymptote, rather similar to what is observed experimentally. For lattice systems we find that T BKT has an absolute maximum of the order of 0.1E F. We discuss how our results compare with those derived from the Nelson–Kosterlitz criterion based on the mean field superfluid density and the approach to the transition from below. While there is agreement in the strict mean-field BCS regime at weak coupling, we find that at moderate pairing strength bosonic excitations cause a substantial increase in T BKT followed by an often dramatic decrease before the system enters the BEC regime.