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arXiv:1302.0682 · Physical Review A

Stimulated adiabatic passage in a dissipative ensemble of atoms with strong Rydberg-state interactions

David Petrosyan, Klaus Mølmer

Published Mar 21, 2013• 51 citations

Abstract

We study two-photon excitation of Rydberg states of atoms under stimulated adiabatic passage with delayed laser pulses. We find that the combination of strong interaction between the atoms in Rydberg state and the spontaneous decay of the intermediate exited atomic state leads to the Rydberg excitation of precisely one atom within the atomic ensemble. The quantum Zeno effect offers a lucid interpretation of this result: the Rydberg blocked atoms repetitively scattering photons effectively monitor a randomly excited atom, which therefore remains in the Rydberg state. This system can be used for deterministic creation and, possibly, extraction of Rydberg atoms or ions one at a time. The sympathetic monitoring via decay of ancilla particles may find wider applications for state preparation and probing of interactions in dissipative many-body systems.

DOI: 10.1103/physreva.87.033416

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We study two-photon excitation of Rydberg states of atoms under stimulated adiabatic passage with delayed laser pulses. We find that the combination of strong interaction between the atoms in Rydberg state and the spontaneous decay of the intermediate exited atomic state leads to the Rydberg excitation of precisely one atom within the atomic ensemble. The quantum Zeno effect offers a lucid interpretation of this result: the Rydberg blocked atoms repetitively scattering photons effectively monitor a randomly excited atom, which therefore remains in the Rydberg state. This system can be used for deterministic creation and, possibly, extraction of Rydberg atoms or ions one at a time. The sympathetic monitoring via decay of ancilla particles may find wider applications for state preparation and probing of interactions in dissipative many-body systems.

In an atomic ensemble, quantum information is typically carried as single collective excitations. It is very advantageous if the creation of single excitations is efficient and robust. A Rydberg blockade enables deterministic creation of single excitations via a collective Rabi oscillation by precisely controlling the pulse area, being sensitive to many experimental parameters. In this paper, we implement the adiabatic rapid passage technique to the Rydberg excitation process in a mesoscopic atomic ensemble. We make use of a two-photon excitation scheme with an intermediate state off-resonant and sweep the laser frequency of one excitation laser. We find the chirped scheme preserves internal phases of the collective Rydberg excitation and is more robust against variance of laser intensity and frequency detuning.

We propose to apply stimulated adiabatic passage to transfer atoms from their ground state into Rydberg excited states. Atoms a few micrometers apart experience a dipole-dipole interaction among Rydberg states that is strong enough to shift the atomic resonance and inhibit excitation of more than a single atom. We show that the adiabatic passage in the presence of this interaction between two atoms leads to robust creation of maximally entangled states and to two-bit quantum gates. For many atoms, the excitation blockade leads to an effective implementation of collective-spin and Jaynes-Cummings-like Hamiltonians, and we show that the adiabatic passage can be used to generate collective J_{x}=0 eigenstates and Greenberger-Horne-Zeilinger states of tens of atoms.

We propose an efficient method to filter out single atoms from trapped ensembles with unknown numbers of atoms. The method employs stimulated adiabatic passage to reversibly transfer a single atom to the Rydberg state which blocks subsequent Rydberg excitation of all the other atoms within the ensemble. This triggers the excitation of Rydberg-blockaded atoms to short-lived intermediate states and their subsequent decay to untrapped states. Using an auxiliary microwave field to carefully engineer the dissipation, we obtain a nearly deterministic single-atom source. Our method is applicable to small atomic ensembles in individual microtraps and in lattice arrays.

We propose to use adiabatic rapid passage with a chirped laser pulse in the strong dipole blockade regime to deterministically excite only one Rydberg atom from randomly loaded optical dipole traps or optical lattices. The chirped laser excitation is shown to be insensitive to the random number

N

of the atoms in the traps. Our method overcomes the problem of the

\sqrt{N}

dependence of the collective Rabi frequency, which was the main obstacle for deterministic single-atom excitation in the ensembles with unknown

N

, and can be applied for single-atom loading of dipole traps and optical lattices.

We show that with adiabatic passage, one can reliably drive two-photon optical transitions between the ground states and interacting Rydberg states in a pair of atoms. For finite Rydberg interaction strengths a new adiabatic pathway towards the doubly Rydberg excited state is identified when a constant detuning is applied with respect to an intermediate optically excited level. The Rydberg interaction among the excited atoms provides a phase that may be used to implement quantum gate operations on atomic ground state qubits.

We show that with adiabatic passage, one can reliably drive two-photon optical transitions between the ground states and interacting Rydberg states in a pair of atoms. For finite Rydberg-interaction strengths an adiabatic pathway towards the doubly Rydberg excited state is identified when a constant detuning is applied with respect to an intermediate optically excited level. The Rydberg interaction among the excited atoms provides a phase that may be used to implement quantum gate operations on atomic ground-state qubits.