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arXiv:1202.6626 · Physical Review Letters

Adiabatic State Preparation of Interacting Two-Level Systems

Richard Brierley, Celestino Creatore, P. B. Littlewood, P. R. Eastham

Published Jul 23, 2012• 18 citations
arXivHTMLPDF

Abstract

We consider performing adiabatic rapid passage (ARP) using frequency-swept driving pulses to excite a collection of interacting two-level systems. Such a model arises in a wide range of many-body quantum systems, such as cavity QED or quantum dots, where a nonlinear component couples to light. We analyze the one-dimensional case using the Jordan-Wigner transformation, as well as the mean-field limit where the system is described by a Lipkin-Meshkov-Glick Hamiltonian. These limits provide complementary insights into the behavior of many-body systems under ARP, suggesting our results are generally applicable. We demonstrate that ARP can be used for state preparation in the presence of interactions, and identify the dependence of the required pulse shapes on the interaction strength. In general, interactions increase the pulse bandwidth required for successful state transfer, introducing new restrictions on the pulse forms required.

DOI
10.1103/physrevlett.109.043002

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We consider performing adiabatic rapid passage (ARP) using frequency-swept driving pulses to excite a collection of interacting two-level systems. Such a model arises in a wide range of many-body quantum systems, such as cavity QED or quantum dots, where a nonlinear component couples to light. We analyze the one-dimensional case using the Jordan-Wigner transformation, as well as the mean-field limit where the system is described by a Lipkin-Meshkov-Glick Hamiltonian. These limits provide complementary insights into the behavior of many-body systems under ARP, suggesting our results are generally applicable. We demonstrate that ARP can be used for state preparation in the presence of interactions, and identify the dependence of the required pulse shapes on the interaction strength. In general, interactions increase the pulse bandwidth required for successful state transfer, introducing new restrictions on the pulse forms required.
Adiabatic rapid passage (ARP) is a powerful technique for efficient transfer of population between quantum states. In the laboratory, the efficiency of ARP is often limited by noise on either the energies of the states or the frequency of the driving field. We study ARP in the simple setting of a two-level system subject to sinusoidal fluctuations on the energy level separation by numerically solving the optical Bloch equations in the absence of damping. We investigate the dependence of the efficiency of population transfer on the frequency and amplitude of the perturbation and find that it is predominantly affected by resonant coupling when the detuning matches the frequency of the noise. We present intuitive principles for when ARP becomes inefficient within this model, and provide a sufficient condition for the population transfer to be above an arbitrary threshold.
Quantum state preparation through external control is fundamental to established methods in quantum information processing and in studies of dynamics. In this respect, excitons in semiconductor quantum dots are of particular interest, since their coupling to light allows them to be driven into a specified state using the coherent interaction with a tuned optical field, such as an external laser pulse. We propose a protocol, based on adiabatic rapid passage, for the creation of entangled states in an ensemble of pairwise coupled two-level systems, such as an ensemble of coupled quantum dots. We show by quantitative analysis using realistic parameters for semiconductor quantum dots that this method is feasible where other approaches are unavailable. Furthermore, this scheme can be generically transferred to some other physical systems, including circuit QED, nuclear and electron spins in solid-state environments, and photonic coupled cavities.
Abstract We analyze the excitation of two ground state atoms to a double Rydberg state by a two-photon chirped optical pulse in the regime of adiabatic rapid passage (ARP). For intermediate Rydberg–Rydberg interaction strengths relevant for atoms separated by ∼ten μ m, adiabatic excitation can be achieved at experimentally feasible Rabi frequencies and chirp rates of the pulses, resulting in high transfer efficiencies. We also study the adiabatic transfer between ground and Rydberg states as a means to realize a controlled phase gate between atomic qubits.
An exciton in a quantum dot (QD) strongly couples to light, allowing the ultrafast manipulation of the quantum states on the order of femtoseconds [1]. Since a QD exciton can be regarded as a two-level system, the excitonic state can be manipulated coherently via Rabi oscillations depending on the electric field of the excitation pulse and the resonant frequency of the QD exciton. However, uniformly manipulating the exciton ensemble in a large number of QDs using ultrashort pulses is quite difficult due to the inhomogeneous distributions of the excitonic resonant frequency and the laser intensity for each QD. Adiabatic rapid passage (ARP) has been demonstrated to overcome this problem because it provides a quantum manipulation technique robust over the inhomogeneities [2], [3] by using chirped pulses (CP) instead of using Fourier transform-limited pulses (TLP). While ARP has been studied extensively in two-level systems with inhomogeneous linewidths up to GHz, it has not been rarely applied to two-level systems with THz inhomogeneous linewidths such as QDs. In this work, we experimentally demonstrate the ultrafast coherent transfer of the exciton population via ARP in two kinds of QD samples; 150-layer stacked InAs QDs and 50-layer stacked InAs QDs embedded in a resonator (Fig. 1(a)).
Adiabatic rapid passage (ARP) is extensively used to achieve efficient transfer or inversion of populations in quantum systems. Landau and Zener accurately estimated the transfer probability of ARP for a closed system and showed that this probability improved with higher drive amplitude. Recently, we found that, in open quantum systems, applying a strong drive can give rise to significant drive-induced dissipation (DID). Here, we investigate the effect of DID on the performance of ARP that is implemented using a linearly chirped pulse on a two-level system. From the Landau-Zener formula, the population transfer was known to be enhanced with increasing drive amplitude. However, here we show that, beyond a threshold value of the drive amplitude, the transfer probability is reduced because of the detrimental effect of DID. We show that the competition between the two processes results in an optimal behavior of the population transfer. We also propose a phenomenological model that helps explain such nonmonotonic behavior of the transfer. Using this model, we estimate the optimum time at which the maximum population transfer occurs. We extend the analysis for rectangular as well as Gaussian pulse profiles and conclude that a Gaussian pulse outperforms a rectangular pulse.
We study the evolution of an exciton confined in a quantum dot adiabatically controlled by a frequency-swept (chirped) laser pulse in the presence of carrier-phonon coupling. We focus on the dynamics induced by a linearly polarized beam and analyze the decoherence due to phonon-assisted biexciton generation. We show that if the biexciton state is shifted down by a few meV, as is typically the case, then the resulting decoherence is strong even at low temperatures. As a result, efficient state preparation is restricted to a small parameter area corresponding to low temperatures, positive chirps, and moderate pulse areas.