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arXiv:1103.2032 · Physical Review A

Raman-assisted Rabi resonances in two-mode cavity QED

P. Grünwald, S. K. Singh, W. Vogel

Published Jun 8, 2011• 20 citations
arXivHTMLPDF

Abstract

The dynamics of a vibronic system in a lossy two-mode cavity is studied, with the first mode being resonant to the electronic transition and the second one being nearly resonant due to Raman transitions. We derive analytical solutions for the dynamics of this system. For a properly chosen detuning of the second mode from the exact Raman resonance, we obtain conditions that are closely related to the phenomenon of Rabi resonance as it is well known in laser physics. Such resonances can be observed in the spontaneous emission spectra, where the spectrum of the second mode in the case of weak Raman coupling is enhanced substantially.

DOI
10.1103/physreva.83.063806

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The dynamics of a vibronic system in a lossy two-mode cavity is studied, with the first mode being resonant to the electronic transition and the second one being nearly resonant due to Raman transitions. We derive analytical solutions for the dynamics of this system. For a properly chosen detuning of the second mode from the exact Raman resonance, we obtain conditions that are closely related to the phenomenon of Rabi resonance as it is well known in laser physics. Such resonances can be observed in the spontaneous emission spectra, where the spectrum of the second mode in the case of weak Raman coupling is enhanced substantially.
We study the classically driven two-level system with its center-of-mass motion vibrating in a harmonic trap and coupled to the photons in a two-mode cavity. The first mode is resonant to the driving field and an electronic transition. The second mode is off-resonant, forming a vibrational-assisted Raman transition. Using an exact numerical method, we investigate the quantum dynamics of the light emitted by the atom and the cavity modes. We analyze and compare the corresponding atomic and intracavity photon spectra for a range of the driving laser field and the cavity coupling strengths. The results provide better understanding of the effects of the laser field and atom-cavity coupling strengths on quantum interference effects and photon blockade, particularly the Mollow's triplet and the Autler-Townes splitting in the good and bad cavity limits.
Within the framework of exact quantum electrodynamics in dispersing and absorbing media, we have studied the emission from an initially in the upper state prepared emitter in a high-quality cavity in the case when there are two cavity modes that resonantly interact with the emitter. In the case when one of the modes is in resonance with the emitter transition and the other mode is tuned to the frequency equal to the Rabi splitting of the first mode, the effect of Rabi resonance is observed. In particular, the second mode exhibits a substantial increase of the one-photon Fock state efficiency and enhancement of the emission spectrum in comparison to the exact resonant case.
We study nonlinear dynamics in the fundamental cavity QED system, consisting of a point-like collection of two-level atoms moving through a single-mode cavity, with a spatially inhomogenous field. In the semiclassical, strong-coupling and rotating-wave approximations, the model is shown to be integrable with atoms moving at exact resonance through a cavity with an arbitrary spatial profile of the mode along the propagation axis. The general exact semiclassical solution is derived in an explicit form, in terms of Jacobian elliptic functions. Numerical simulation confirms that perturbations, which are produced by a modulation of the coupling between moving atoms and a cavity mode, provide, our of resonance, a mechanism responsible for Hamiltonian chaos. Taking into account the interatomic quantum correlations, we go beyond the semiclassical model and derive a dynamical system, which is able to describe vacuum Rabi oscillation with moving atoms. At resonance, this system is again shown to be integrable with a general semiquantum solution found. Out of resonance, it can demonstrate chaotic vacuum Rabi oscillations, which may be considered as a new kind of reversible spontaneous emission.
We study a classically driven two-level system in a harmonic trap and a lossy two-mode cavity, with the first mode being resonant to the driving field and an electronic transition, and the second mode being off-resonant, forming a vibrational-assisted Raman transition. Using an exact numerical method, we compute the steady state as well as the time evolution of the photon statistics. We further investigate the photon correlations of both the cavity modes and identify the laser parameters and coupling strength that give the nonclassical sub-Poissonian property. The work is useful for coherent control of photon statistics and photon correlations in the trapped two-level system.
We measure the transmission spectrum of an optical cavity filled with two-level atoms. For small intensities, the coupling between atoms and a single mode of the cavity splits the spectrum into two normal modes: the vacuum Rabi peaks. We gradually decouple the system in two ways and study the evolution of the vacuum Rabi peaks. First we lower the atom-cavity coupling frequency through its intensity dependence, showing that the peaks shift, deform, exhibit frequency hysteresis, and eventually merge into a single peak that approaches the empty cavity resonance. Second we detune the atoms and the cavity mode and observe an avoided crossing. The normal modes of the coupled system transform into the two resonances of the uncoupled system. We map out the transition region and find good agreement with theoretical predictions.
Recently, cavity quantum electrodynamic (QED) effects in semiconductor microcavities have been of considerable interest since, in the weak-coupling regime they play an important role in selectively increasing spontaneous emission into the lasing mode of vertical-cavity surface-emitting lasers (VCSEL’s) [1,2], enabling low-threshold, high speed, and high efficiency. In a strong-coupling regime, the normal modes of the coupled system are superpositions of the exciton and cavity modes. Hence the impulsively excited system will evolve in time with the energy oscillating between the exciton and cavity modes. This is known as a vacuum-Rabi oscillation (VRO), with a frequency of Ω=d¯⋅E¯/@@h, where d¯ is the transition dipole moment of atoms and E¯ the vacuum-field strength. Of course, VRO are observable only when the cavity lifetime and exciton dephasing time are long enough compared to VRO period. Recently, Weisbuch et al. [3] have reported an observation of the normal-mode vacuum Rabi splitting in 2-D-exciton/planar-DBR microcavities. The observed splittings were as large as 6 meV in reflection and transmission spectra, implying 690-fs vacuum Rabi oscillations.