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arXiv:1008.3212 · Physical Review B

Collective modes in multiband superfluids and superconductors: Multiple dynamical classes

Yukihiro Ota, Masahiko Machida, Tomio Koyama, Hideo Aoki

Published Feb 23, 2011• 40 citations
arXivHTMLPDF

Abstract

One important way to characterize the states having a gauge symmetry spontaneously broken over multibands is to look at their collective excitation modes. We find that a three-band system has multiple Leggett modes with significantly different masses, which can be classified into different dynamical classes according to whether multiple interband Josephson currents add or cancel. This provides a way to dynamically characterize multiband superconductivity while the pairing symmetry is a static property.

DOI
10.1103/physrevb.83.060507

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One important way to characterize the states having a gauge symmetry spontaneously broken over multibands is to look at their collective excitation modes. We find that a three-band system has multiple Leggett modes with significantly different masses, which can be classified into different dynamical classes according to whether multiple interband Josephson currents add or cancel. This provides a way to dynamically characterize multiband superconductivity while the pairing symmetry is a static property.
Motivated by the recent development of terahertz pump-probe experiments, we investigate the short-time dynamics in superconductors with multiple attractive pairing channels. Studying a single-band square lattice model with a spin-spin interaction as an example, we find the signatures of collective excitations of the pairing symmetries (known as Bardasis-Schrieffer modes) as well as the order parameter amplitude (Higgs mode) in the short-time dynamics of the spectral gap and quasiparticle distribution after an excitation by a pump pulse. We show that the polarization and intensity of the pulse can be used to control the symmetry of the nonequilibrium state as well as frequencies and relative intensities of the contributions of different collective modes. We find particularly strong signatures of the Bardasis-Schrieffer mode in the dynamics of the quasiparticle distribution function. Our work shows the potential of modern ultrafast experiments to address the collective excitations in unconventional superconductors and highlights the importance of subdominant interactions for the nonequilibrium dynamics in these systems.
We consider multiband BCS superconductors that exhibit time-reversal symmetry and uniform pairing, and analyze their dynamic density and spin structure factors using linear-response theory within the mean-field BCS-BEC crossover framework at zero temperature. Our results for the multi-orbital Hubbard model satisfy the associated f-sum rules in several limits. In particular, in the strong-coupling limit, they coincide with those of a weakly-interacting Bose gas of Cooper pairs, where the low-energy collective Goldstone modes serve as Bogoliubov phonons. We further reveal that the quantum-geometric origin of the low-energy structure factors, along with related observables such as the superfluid-weight tensor and the effective-mass tensor of Cooper pairs, can be traced all the way back to the effective-mass theorem for Bloch bands in this limit. As an illustration, we investigate the pyrochlore-Hubbard model numerically and demonstrate that the Goldstone modes are the only relevant collective degrees of freedom in the flat-band regime.
Beyond the frozen-pairing contribution, the superfluid weight of a multiband superconductor contains a correction from the self-consistent relaxation of the pairing amplitudes under a phase twist. We show that this correction has a quantum-geometric origin, not in the space of Bloch states but in the space of collective pairing fields. For an attractive multiband Hubbard model at the mean-field level, the thermodynamic Hessian governing the pairing response coincides with the static Gaussian pair-fluctuation kernel at zero momentum at every temperature below TcT_cTc​. Since gauge invariance relates a phase twist to a finite center-of-mass momentum of the pair field, the superfluid weight is set by the small-momentum curvature of the eigenvalue branch that evolves from the Goldstone mode, and the relaxation correction is a stiffness-weighted quantum metric of the corresponding soft eigenvector on the manifold of pairing configurations. The same construction yields the Ginzburg-Landau gradient coefficient with the identical geometric correction, hence the coherence-length tensor, and, with the low-frequency dynamics of the kernel, the pair-mass tensor. Lieb-lattice calculations verify the equivalence of the thermodynamic, fluctuation-kernel, and soft-mode formulations and the independence of the superfluid weight from the orbital embedding.
Abstract The Leggett collective excitations for a two-band Fermi gas with s-wave pairing and Josephson interband coupling in the BCS-BEC crossover at finite temperatures are investigated within the Gaussian pair fluctuation approach. Eigenfrequencies and damping factors for Leggett modes are determined in a nonperturbative way, using the analytic continuation of the fluctuation propagator through a branch cut in the complex frequency plane, as in Kurkjian et al (2019 Phys. Rev. Lett. 122 093403). The treatment is performed beyond the low-energy expansion, which is necessary when the collective excitation energy reaches the pair-breaking continuum edge. The results are applied in particular to cold atomic gases at the orbital Feshbach resonance and in a regime far from BEC, which can be relevant for future experiments.
The anti-ferromagnetic Lieb-Mattis model is investigated in detail. Symmetry breaking, low-lying excitation spectrum and macroscopic quantity like Berry phase are calculated for this model. Superconductivity is studied with respect to the collective modes of negative U Hubbard model and the BCS superconductor. The Integer Quantum Hall is looked into by various ways such as by using the center of mass and orbital center coordinates. The importance of domain wall in a Quantum Hall system is stressed.These systems are particularly chosen as they are prototypical/ archetypal fermionic and spin quantum condensed matter systems. iii
This thesis reports on theoretical investigations of the ultrafast nonequilibrium dynamics in superconductors. In particular, two nonequilibrium scenarios are modeled by combining several analytical and numerical methods: transient superconducting phase transition and collective excitations of a superconducting condensate. In the first part of the thesis the possibility to induce singlet superconducting correlations far from equilibrium is explored by applying time-dependent Lanczos algorithm to the one-dimensional extended Hubbard model. Here, the system is driven into a nonequilibrium state by (i) interaction quench and (ii) quench by pulse. In both cases the buildup of the superconducting correlations is studied in view of several correlation functions. Moreover, a transient Meissner effect, which reflects fingerprints of the induced superconductivity, is observed in calculations of the important for experiments time-dependent optical conductivity. In addition, the differences between nonequilibrium dynamics of the extended Hubbard model initiated by interaction quench and by pulse quench are discussed in detail. The second part is devoted to the excitation of collective modes in a superconductor out of equilibrium. First of all, focus is given to the properties of collective modes close to equilibrium conditions, where a linearized response can be expected. Within the framework of the (Nambu-) matrix kinetic theory in the clean limit a comprehensive gauge-invariant description of the collective modes associated with phase fluctuations of the order parameter is analytically formulated for the generalized case of two- band superconducting systems. Particular emphasis is on the application to the recently discovered noncentrosymmetric superconductors. A detailed analysis of the collective modes includes specification of the gauge mode (common to all superconductors) and the Leggett mode (collective fluctuations of the interband phase difference), and investigation of their subtle interplay in view of validity of the charge conservation law and the participation in the Anderson-Higgs mechanism. Further, the nonequilibrium excitation of the superconducting gaps for the case of two-band superconductors with singlet pairing correlations is investigated in a view of optical pump-probe experiments. For this purpose a semi-numerical method based on the density- matrix theory is formulated. In this case additional amplitude (Higgs) modes were identified, which allow to directly detect the properties of the superconducting condensates as a function of time. Moreover, a new interplay between the phase (Leggett) and amplitude (Higgs) modes is studied in detail. In particular it was found that the nonadiabatic excitation process leads to strong coupling between both modes. Finally, based on calculations of the time-dependent optical conductivity the prediction is made that the coupled Higgs and Leggett modes can be clearly visible in the pump-probe absorption spectra.