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arXiv:0907.4191 · Physical Review Letters

Electrical Measurement of a Two-Electron Spin State in a Double Quantum Dot

Nobuhiko Yokoshi, Hiroshi Imamura, Hideo Kosaka

Published Jul 23, 2009• 9 citations
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Abstract

We propose a scheme for electrical measurement of two-electron spin states in a semiconductor double quantum dot. We calculated the adiabatic charge transfer when surface gates are modulated in time. Because of spin-orbit coupling in the semiconductor, spatial displacement of the electrons causes a total spin rotation. It follows that the expectation value of the transferred charge reflects the relative phase as well as the total spin population of a prepared singlet-triplet superposition state. The precise detection of the charge transfer serves to identify the quantum superposition.

DOI
10.1103/physrevlett.103.046806

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We propose a scheme for electrical measurement of two-electron spin states in a semiconductor double quantum dot. We calculated the adiabatic charge transfer when surface gates are modulated in time. Because of spin-orbit coupling in the semiconductor, spatial displacement of the electrons causes a total spin rotation. It follows that the expectation value of the transferred charge reflects the relative phase as well as the total spin population of a prepared singlet-triplet superposition state. The precise detection of the charge transfer serves to identify the quantum superposition.
A pulsed-gate technique with charge sensing is used to measure the singlet-triplet relaxation time for nearly degenerate spin states in a two-electron double quantum dot. Transitions from the (1,1) charge occupancy state to the (0,2) state, measured as a function of pulse cycle duration and magnetic field, allow the (1,1) singlet-triplet relaxation time $(\ensuremath{\geqslant}70\phantom{\rule{0.3em}{0ex}}\ensuremath{\mu}\mathrm{s})$ and the (0,2) singlet-triplet splitting to be measured. This technique can be readily applied to read out a spin-qubit operating in a singlet-triplet basis.
Exchange-coupled singlet-triplet spin qubits in two gate-defined double quantum dots are considered theoretically. Using charge density operators to describe the double-dot orbital states, we calculate the Coulomb couplings between the qubits and identify optimal bias points for single- and two-qubit operations, as well as convenient idle positions. The same intuitive formulation is used to derive dephasing rates of these qubits due to the fluctuating charge environment, thereby providing the main considerations for a quantum computation architecture that is within current experimental capabilities.
The adiabatic passage of two correlated electrons in three coupled quantum dots is shown to provide a robust and controlled way of distilling, transporting, and detecting spin entanglement, as well as measuring the rate of spin disentanglement. By employing tunable interdot coupling the scheme creates from an unentangled two-electron state, a superposition of spatially separated singlet and triplet states. A single measurement of a dot population (charge) collapses the wave function to either of these states, realizing the entanglement to the charge conversion. The scheme is robust, with the efficiency close to 100%, for a large range of realistic spectral parameters.
A two-level quantum system is the building block of a quantum computer. This pair of quantum states defines the computational unit of a quantum computer, and it is called a quantum bit or qubit in analogy to the bit that is the binary unit of a classical computer. The spin of a single electron naturally defines such a two-level quantum system. A quantum dot can be tuned to the single-electron regime, and an array of singly occupied quantum dots provides a multi-qubit register. This thesis describes the multielectron encoding of a spin qubit using a pair or a trio of quantum dots, and it analyzes the coherence properties and manipulation protocols of this system. The singlet-triplet qubit, coded using the singlet state and the spinless triplet state of a pair of singly occupied quantum dots, can be controlled all electrically when applying voltages to gates close to the quantum dot structure. Rapid, subnanosecond modifications of the double quantum dot's charge configuration have been realized successfully. A small magnetic field gradient across the double quantum dot enables universal qubit control. Two modifications of the normal singlet-triplet encoding are introduced. (1) The six-electron configuration of a double quantum dot encodes a singlet-triplet qubit in the same way as for the two-electron double quantum dot. Two electrons at each quantum dot are irrelevant for the qubit manipulations because they are paired in a singlet state; the remaining two electrons encode the qubit. The qubit's wave function is immune to charge noise at moderate out-of-plane magnetic fields. (2) A singlet-triplet qubit encoded using two quantum dots of different sizes has an orbital state degeneracy of the singlet state and the spinless triplet state at finite out-of-plane magnetic fields. Spin-orbit interactions lift this state degeneracy, while the magnitude of the state coupling is determined by the size difference of the QDs. This setup enables the manipulations of singlet-triplet qubits without the need for magnetic field gradients. Finally, two-qubit gates between singlet-triplet qubits are proposed that use mediated exchange interactions via one quantum state. These operations are well controlled and highly noise insensitive. Orbital interactions alone can control spin qubits coded in a three electron Hilbert space. For example, the exchange-only qubit is encoded using three singly occupied quantum dots. The exchange interactions of two quantum dot pairs need to be modified to manipulate this qubit. The noise sensitivity of the exchange-only qubit is discussed. Alternatively, a three-electron qubit at a double quantum dot can be operated when single electrons are transferred between the quantum dots. Fast, subnanosecond manipulations of the double quantum dot's charge configuration are required to realize single-qubit gates. A novel two-qubit pulse gate for the three-electron double quantum dot qubit is proposed.
We demonstrate one and two photoelectron trapping and the subsequent dynamics associated with interdot transfer in double quantum dots over a time scale much shorter than the typical spin lifetime. Identification of photoelectron trapping is achieved via resonant interdot tunneling of the photoelectrons in the excited states. The interdot transfer enables detection of single photoelectrons in a nondestructive manner. When two photoelectrons are trapped at almost the same time we observed that the interdot resonant tunneling is strongly affected by the Coulomb interaction between the electrons. Finally the influence of the two-electron singlet-triplet state hybridization has been detected using the interdot tunneling of a photoelectron.
The information transfer from a photon to an electron spin in semiconductors is predicted to forward the realization of quantum computation.Gate defined lateral quantum dots is an attractive platform in this sense since the electrical single and two quantum bit (qubit) gate operations have been demonstrated only in this system.However, realization of quantum media conversion is limited up to the single photon to charge conversion due to the large disturbance of electrostatic potentials by the irradiation of light.It is still challenging to achieve high visibility of single-shot photoelectron spin measurements and the detection of angular momentum transfer from a single photon polarization to a single photoelectron spin.This work presents the detection of single photoelectron spins excited by single circularly polarized photons and confirm the optical selection rules associated with the conversion.Double heterostructure GaAs quantum wells (QWs) were prepared to selectively excite electron spins from the discrete heavy and light hole bands.The QWs are also designed to meet the requirement of the coherent transfer scheme.The out of plane electron g-factors were measured from resistively detected electron spin resonance experiments and we determined the well width implying the near zero in-plane electron g-factor.To overcome the disturbance due to light irradiation, a double quantum dot (DQD) was formed on the chosen QW.DQDs are preferable for high visibility detection of spin states using Pauli spin blockade.Additionally, under i Here, I would like to thank them all.