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Achieving quantum computation with quantum dot spin qubits

Sebastian Mehl, David Peter Divincenzo

Published Jan 1, 2014• 0 citations
OpenAlex

Abstract

A two-level quantum system is the building block of a quantum computer. This pair of quantum states defines the computational unit of a quantum computer, and it is called a quantum bit or qubit in analogy to the bit that is the binary unit of a classical computer. The spin of a single electron naturally defines such a two-level quantum system. A quantum dot can be tuned to the single-electron regime, and an array of singly occupied quantum dots provides a multi-qubit register. This thesis describes the multielectron encoding of a spin qubit using a pair or a trio of quantum dots, and it analyzes the coherence properties and manipulation protocols of this system. The singlet-triplet qubit, coded using the singlet state and the spinless triplet state of a pair of singly occupied quantum dots, can be controlled all electrically when applying voltages to gates close to the quantum dot structure. Rapid, subnanosecond modifications of the double quantum dot's charge configuration have been realized successfully. A small magnetic field gradient across the double quantum dot enables universal qubit control. Two modifications of the normal singlet-triplet encoding are introduced. (1) The six-electron configuration of a double quantum dot encodes a singlet-triplet qubit in the same way as for the two-electron double quantum dot. Two electrons at each quantum dot are irrelevant for the qubit manipulations because they are paired in a singlet state; the remaining two electrons encode the qubit. The qubit's wave function is immune to charge noise at moderate out-of-plane magnetic fields. (2) A singlet-triplet qubit encoded using two quantum dots of different sizes has an orbital state degeneracy of the singlet state and the spinless triplet state at finite out-of-plane magnetic fields. Spin-orbit interactions lift this state degeneracy, while the magnitude of the state coupling is determined by the size difference of the QDs. This setup enables the manipulations of singlet-triplet qubits without the need for magnetic field gradients. Finally, two-qubit gates between singlet-triplet qubits are proposed that use mediated exchange interactions via one quantum state. These operations are well controlled and highly noise insensitive. Orbital interactions alone can control spin qubits coded in a three electron Hilbert space. For example, the exchange-only qubit is encoded using three singly occupied quantum dots. The exchange interactions of two quantum dot pairs need to be modified to manipulate this qubit. The noise sensitivity of the exchange-only qubit is discussed. Alternatively, a three-electron qubit at a double quantum dot can be operated when single electrons are transferred between the quantum dots. Fast, subnanosecond manipulations of the double quantum dot's charge configuration are required to realize single-qubit gates. A novel two-qubit pulse gate for the three-electron double quantum dot qubit is proposed.

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A two-level quantum system is the building block of a quantum computer. This pair of quantum states defines the computational unit of a quantum computer, and it is called a quantum bit or qubit in analogy to the bit that is the binary unit of a classical computer. The spin of a single electron naturally defines such a two-level quantum system. A quantum dot can be tuned to the single-electron regime, and an array of singly occupied quantum dots provides a multi-qubit register. This thesis describes the multielectron encoding of a spin qubit using a pair or a trio of quantum dots, and it analyzes the coherence properties and manipulation protocols of this system. The singlet-triplet qubit, coded using the singlet state and the spinless triplet state of a pair of singly occupied quantum dots, can be controlled all electrically when applying voltages to gates close to the quantum dot structure. Rapid, subnanosecond modifications of the double quantum dot's charge configuration have been realized successfully. A small magnetic field gradient across the double quantum dot enables universal qubit control. Two modifications of the normal singlet-triplet encoding are introduced. (1) The six-electron configuration of a double quantum dot encodes a singlet-triplet qubit in the same way as for the two-electron double quantum dot. Two electrons at each quantum dot are irrelevant for the qubit manipulations because they are paired in a singlet state; the remaining two electrons encode the qubit. The qubit's wave function is immune to charge noise at moderate out-of-plane magnetic fields. (2) A singlet-triplet qubit encoded using two quantum dots of different sizes has an orbital state degeneracy of the singlet state and the spinless triplet state at finite out-of-plane magnetic fields. Spin-orbit interactions lift this state degeneracy, while the magnitude of the state coupling is determined by the size difference of the QDs. This setup enables the manipulations of singlet-triplet qubits without the need for magnetic field gradients. Finally, two-qubit gates between singlet-triplet qubits are proposed that use mediated exchange interactions via one quantum state. These operations are well controlled and highly noise insensitive. Orbital interactions alone can control spin qubits coded in a three electron Hilbert space. For example, the exchange-only qubit is encoded using three singly occupied quantum dots. The exchange interactions of two quantum dot pairs need to be modified to manipulate this qubit. The noise sensitivity of the exchange-only qubit is discussed. Alternatively, a three-electron qubit at a double quantum dot can be operated when single electrons are transferred between the quantum dots. Fast, subnanosecond manipulations of the double quantum dot's charge configuration are required to realize single-qubit gates. A novel two-qubit pulse gate for the three-electron double quantum dot qubit is proposed.
This thesis addresses the concept of quantum computing with semiconductor quantum dots. The basic unit of a quantum computer is a quantum mechanical two-level system, the so-called quantum bit (qubit). The qubit can be defined as the spin of an electron confined in a quantum dot or as a two-dimensional subspace of the Hilbert space for several spins. Some semiconductors have several minima in their conduction band, socalled valleys. A two-dimensional valley degree of freedom can also be considered as a qubit. In this thesis, quantum registers storing spin as well as valley qubits are described theoretically. Virtual hopping yields an exchange interaction between neighboring quantum dots, which reduces the energy of antisymmetric spin-valley states according to the Pauli principle. Considering the spin and the valley degrees of freedom of two electrons in neighboring quantum dots as qubits, the exchange interaction is a four-qubit interaction. In this thesis, it will be shown that it is, nevertheless, possible to generate a universal two-qubit gate for spin qubits or for valley qubits by combining the exchange interaction and individual single-qubit gates. The exchange interaction in this two-electron double quantum dot directly provides a universal two-qubit gate for one spin and one valley qubit as well. For this, the qubits are defined as suitable subspaces, spanned by the singlet and one triplet state of the spin and the valley states, respectively, Using those gates, arbitrary quantum operations can be performed for single-spin and single-valley qubits in the same quantum register, where in one double quantum dot the quantum states are restricted to the singlet-triplet subspace. While in this register single-spin and single-valley rotations are required, these gates are dispensable in a quantum register storing spin and valley singlet-triplet qubits. The single-qubit operations, in this case, can be provided by the exchange interaction and a gradient in the energy splitting of spin and valley states when the spin qubit is stored in a double quantum dot with spin degrees of freedom only and when the spin states in the double quantum dot which stores the valley qubit are polarized. For providing the two-qubit gate, the spin and the valley qubits need to be stored in the same double quantum dot. The crucial task for this register is to interchange the spin of a spin-only and a spin-valley quantum dot in order to switch between the single-qubit and the two-qubit operation mode. This interchanging of the spin can be achieved by a valley-depending virtual hopping between the quantum dots. Furthermore, echo sequences for a so-called exchange-only qubit are considered. An exchange-only qubit is defined as a subspace in a system of three electron spins in a triple quantum dot. An inhomogeneous magnetic field, which may be caused by nuclear spins in the semiconductor, can lead to decoherence and leakage, i.e., the state might leave the qubit subspace. Suppressing this effect by an echo sequence which consists of pulses interchanging neighboring spin states, so-called SWAP gates, was proposed. Controllability over these quantum operations is provided via the exchange interaction. In this thesis, the performance of different such sequences is investigated. The analysis shows that optimization strategies developed for single spin echoes can be adapted for the three spin system. The echo sequences can be different in their order of applied SWAP gates interchanging the spins in the first and second dots or in the second and third dots. The noise suppression performance depends slightly on this order of SWAP gates. For two spins in a double quantum dot a scheme for quantum state tomography is presented. The corresponding measurement operators are constructed from a set of mutually unbiased bases of the four-dimensional two-qubit Hilbert space. These measurements are represented by short sequences of no more than three elementary quantum gates and projective measurements by the well-established spin-to-charge conversion.
Coherent control of quantum operations has previously been demonstrated in singlet-triplet qubits which store information in the relative spin of two electrons occupying two same size quantum dots positioned side by side. Here the authors propose to use two quantum dots differing both in size and out-of-plane magnetic field. This is called an inverted singlet-triplet qubit because the existence of a singlet-triplet inversion differs from other qubits. A comparative advantage is that the strongly confined quantum dot can be used for qubit initialization and readout while the weakly confined one is preferable for qubit manipulations. The authors show that full control could be implemented with electrostatic operations even in the presence of realistic noise.
Semiconductor-based spin qubits embedded into a superconducting microwave cavity constitute a fast-progressing and promising platform for realizing fast and fault-tolerant qubit control with long-range two-qubit coupling. The flopping-mode spin qubit consists of a single electron in a double quantum dot; it combines a charge qubit with a spin qubit. With its strong and tunable cavity coupling, the flopping-mode qubit is proven to be well suited for low-power qubit control and cavity-mediated long-range quantum gates. The singlet-triplet (ST) and exchange-only (EO) qubits are multielectron realizations that go without broadband control and are protected from some types of noise, but are challenging to couple to each other and to microwave cavities. We combine the flopping-mode concept with the ST and EO qubits and propose two new flopping-mode qubits that consist of three (four) quantum dots, occupied by two (three) electrons near the ( 1 , 0 , 1 ) ↔ ( 0 , 1 , 1 ) [ ( 1 , 0 , 1 , 1 ) ↔ ( 0 , 1 , 1 , 1 ) ] charge transition. The two-electron system augments the ST 0 spin qubit with a charge qubit that interacts transversally and longitudinally with a cavity. Both couplings are highly tunable, and the longitudinal coupling distinguishes the flopping-mode ST qubit from the regular flopping-mode qubit. The longitudinal coupling allows for nondissipative universal control similar to superconducting transmon qubits. The EO flopping-mode qubit comprises four dots occupied by three electrons and opens a new possibility to perform two-qubit gates for EO qubits that are challenging to perform directly with the exchange coupling. We use input-output theory to provide means of extracting the coupling strengths from cavity transmission data.
Exchange-coupled singlet-triplet spin qubits in two gate-defined double quantum dots are considered theoretically. Using charge density operators to describe the double-dot orbital states, we calculate the Coulomb couplings between the qubits and identify optimal bias points for single- and two-qubit operations, as well as convenient idle positions. The same intuitive formulation is used to derive dephasing rates of these qubits due to the fluctuating charge environment, thereby providing the main considerations for a quantum computation architecture that is within current experimental capabilities.
We study the two-qubit controlled-NOT gate operating on qubits encoded in the spin state of a pair of electrons in a double quantum dot. We assume that the electrons can tunnel between the two quantum dots encoding a single qubit, while tunneling between the quantum dots that belong to different qubits is forbidden. Therefore, the two qubits interact exclusively through the direct Coulomb repulsion of the electrons. We find that entangling two-qubit gates can be performed by the electrical biasing of quantum dots and/or tuning of the tunneling matrix elements between the quantum dots within the qubits. The entangling interaction can be controlled by tuning the bias through the resonance between the singly occupied and doubly occupied singlet ground states of a double quantum dot.