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arXiv:0905.4498 · Physical Review Letters

Nonequilibrium Dynamics of Weakly and Strongly Paired Superconductors

Victor Gurarie

Published Aug 14, 2009• 87 citations
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Abstract

We study small oscillations of the order parameter in weakly and strongly paired superconductors driven slightly out of equilibrium, in the collisionless approximation. While it was known for quite some time that the amplitude of the oscillations in a weakly paired superconductor decays as t(-1/2), we show that in a superconductor sufficiently strongly paired so that its fermions form bound states usually referred to as molecules, these oscillations decay as t(-3/2). The transition between these two regimes happens when the chemical potential of the superconductor vanishes; thus, the behavior of the oscillations can be used to distinguish weakly and strongly paired superconductors. Finally, we interpret the result in the strongly paired superconductor as the probability of the molecular decay as a function of time.

DOI
10.1103/physrevlett.103.075301

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We study small oscillations of the order parameter in weakly and strongly paired superconductors driven slightly out of equilibrium, in the collisionless approximation. While it was known for quite some time that the amplitude of the oscillations in a weakly paired superconductor decays as t(-1/2), we show that in a superconductor sufficiently strongly paired so that its fermions form bound states usually referred to as molecules, these oscillations decay as t(-3/2). The transition between these two regimes happens when the chemical potential of the superconductor vanishes; thus, the behavior of the oscillations can be used to distinguish weakly and strongly paired superconductors. Finally, we interpret the result in the strongly paired superconductor as the probability of the molecular decay as a function of time.
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We consider a three-terminal system consisting of a quantum dot strongly coupled to two superconducting reservoirs in the infinite-gap limit and weakly coupled to a normal metal. Using a real-time diagrammatic approach, we calculate the dynamics of the proximity-induced pair amplitude on the quantum dot. We find that after a quench the pair amplitude shows pronounced oscillations with a frequency determined by the coupling to the superconductors. In addition, it decays exponentially on a timescale set by the coupling to the normal metal. Strong oscillations of the pair amplitude occur also when the system is periodically driven both in the adiabatic and fast-driving limit. We relate the dynamics of the pair amplitude to the Josephson and Andreev current through the dot to demonstrate that it is an experimentally accessible quantity.
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Recent experimental progress in the fields of cold quantum gases and ultrafast optical spectroscopy of quantum materials allows us to controllably induce and probe nonadiabatic dynamics of superconductors and superfluids. The time evolution of the gap function before relaxation with the lattice is determined by the superposition of coherently evolving individual Cooper pairs within the manifold of the Bardeen-Cooper-Schrieffer (BCS) wave function. While dynamics following an abrupt quench of the pairing interaction strength in the single-band BCS model has been exactly solved due to the integrability of the model, the dynamics of postquench multiband superconductors remain under scrutiny. Here, we develop a generalization of the Volkov-Kogan Laplace-space perturbative method that allows us to determine the nonadiabatic gap dynamics of two-band fully gapped superconductors for a wide range of quench amplitudes. Our approach expands the long-time dynamics around the steady-state asymptotic value of the gap, which is self-consistently determined, rather than around the equilibrium value of the gap. We explicitly demonstrate that this method recovers the exact solution of the long-time gap dynamics in the single-band case and perfectly agrees with a numerical solution of the two-band model. We discover that dephasing of Cooper pairs from different bands leads to faster collisionless relaxation of the gap oscillation with a power law of ${t}^{\ensuremath{-}3/2}$ instead of the well-known ${t}^{\ensuremath{-}1/2}$ behavior found in the single-band case. Furthermore, the gap oscillations display beating patterns arising from the existence of two different asymptotic gap values. Our results have important implications to a variety of two-band superconductors driven out of equilibrium, such as iron-based superconductors, MgB2{\mathrm{MgB}}_{2}MgB2​, and SrTiO3{\mathrm{SrTiO}}_{3}SrTiO3​.
We consider a superconductor in which the density of states at the Fermi level or the pairing interaction is driven periodically with a frequency larger than the superconducting gap in the collisionless regime. We show by numerical and analytical computations that a subset of quasiparticle excitations enter into resonance and perform synchronous Rabi oscillations leading to cyclic population inversion with a frequency that depends on the amplitude of the drive. As a consequence a different ``Rabi-Higgs'' mode emerges. Turning off the drive at different times and modulating the strength allows access to all known dynamical phases of the order parameter: persistent oscillations, oscillations with damping and overdamped dynamics. We discuss physical realizations of the drive and methods to detect the dynamics.
I consider relaxation of the pairing amplitude in a disordered Bardeen-Cooper-Schrieffer (BCS) superconductor in the absence of the two-particle collisions. My main assumption is that nonmagnetic and magnetic disorder scattering rates are much smaller than the value of the superconducting pairing gap ${\mathrm{\ensuremath{\Delta}}}_{0}$. I derive a system of nonlinear equations which describe the collisionless relaxation of the pairing amplitude following a quench of the pairing strength. I find that in a superconductor in which scattering on paramagnetic impurities is dominant, the pairing amplitude in a steady state varies periodically with time even for small deviations from equilibrium. It is shown that such a steady state emerges due to scattering on paramagnetic impurities which leads to a decrease in the value of the resonant frequency of the amplitude mode below $2{\mathrm{\ensuremath{\Delta}}}_{0}$.