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arXiv:2110.10100 · Physical review. B./Physical review. B

Pair-amplitude dynamics in strongly coupled superconductor–quantum dot hybrids

Markus Heckschen, Björn Sothmann

Published Jan 25, 2022• 8 citations
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Abstract

We consider a three-terminal system consisting of a quantum dot strongly coupled to two superconducting reservoirs in the infinite-gap limit and weakly coupled to a normal metal. Using a real-time diagrammatic approach, we calculate the dynamics of the proximity-induced pair amplitude on the quantum dot. We find that after a quench the pair amplitude shows pronounced oscillations with a frequency determined by the coupling to the superconductors. In addition, it decays exponentially on a timescale set by the coupling to the normal metal. Strong oscillations of the pair amplitude occur also when the system is periodically driven both in the adiabatic and fast-driving limit. We relate the dynamics of the pair amplitude to the Josephson and Andreev current through the dot to demonstrate that it is an experimentally accessible quantity.

DOI
10.1103/physrevb.105.045420

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We consider a three-terminal system consisting of a quantum dot strongly coupled to two superconducting reservoirs in the infinite-gap limit and weakly coupled to a normal metal. Using a real-time diagrammatic approach, we calculate the dynamics of the proximity-induced pair amplitude on the quantum dot. We find that after a quench the pair amplitude shows pronounced oscillations with a frequency determined by the coupling to the superconductors. In addition, it decays exponentially on a timescale set by the coupling to the normal metal. Strong oscillations of the pair amplitude occur also when the system is periodically driven both in the adiabatic and fast-driving limit. We relate the dynamics of the pair amplitude to the Josephson and Andreev current through the dot to demonstrate that it is an experimentally accessible quantity.
The proximity effect in hybrid superconducting--normal-metal structures is shown to affect strongly the coherent oscillations of the superconducting order parameter $\mathrm{\ensuremath{\Delta}}$ known as the Higgs modes. The standard Higgs mode at frequency $2\mathrm{\ensuremath{\Delta}}$ is damped exponentially by the quasiparticle leakage from the primary superconductor. Two new Higgs modes with the frequencies depending on both the primary and induced gaps in the hybrid structure are shown to appear due to the coherent electron transfer between the superconductor and the normal metal. Altogether, these three modes determine the long-time asymptotic behavior of the superconducting order parameter disturbed either by the electromagnetic pulse or the quench of the system parameters and thus are of crucial importance for the dynamical properties and restrictions on the operating frequencies for superconducting devices based on the proximity effect used, e.g., in quantum computing, in particular, with topological low-energy excitations.
Dynamical processes induced by the external time-dependent fields can provide valuable insight into the characteristic energy scales of a given physical system. We investigate them here in a nanoscopic heterostructure, consisting of the double quantum dot coupled in series to the superconducting and the metallic reservoirs, analyzing its response to (i) abrupt bias voltage applied across the junction, (ii) sudden change of the energy levels, and imposed by (iii) their periodic driving. We explore subgap properties of this setup which are strictly related to the in-gap quasiparticles and discuss their signatures manifested in the time-dependent charge currents. The characteristic multi-mode oscillations, their beating patters and photon-assisted harmonics reveal a rich spectrum of dynamical features that might be important for designing the superconducting qubits.
Abstract Dynamical processes induced by the external time-dependent fields can provide valuable insight into the characteristic energy scales of a given physical system. We investigate them here in a nanoscopic heterostructure, consisting of the double quantum dot coupled in series to the superconducting and the metallic reservoirs, analyzing its response to (i) abrupt bias voltage applied across the junction, (ii) sudden change of the energy levels, and imposed by (iii) their periodic driving. We explore subgap properties of this setup which are strictly related to the in-gap quasiparticles and discuss their signatures manifested in the time-dependent charge currents. The characteristic multi-mode oscillations, their beating patters and photon-assisted harmonics reveal a rich spectrum of dynamical features that might be important for designing the superconducting qubits.
The combined action of a DC bias and a microwave drive on the transport characteristic of a superconductor-quantum dot-superconductor junction is investigated. To cope with time dependent non-equilibrium effects and interactions in the quantum dot, we develop a general formalism for the dynamics of the density operator based on a particle conserving approach to superconductivity. Without invoking a broken U (1) symmetry, we identify a dynamical phase connected to the coherent transfer of Cooper pairs across the junction. In the weak coupling limit, we show that besides quasiparticle transport, proximity induced superconducting correlations manifest in anomalous pair tunneling involving the transfer of a Cooper pair. The resulting generalized master equation in presence of the microwave drive showcases the characteristic bichromatic response due to the combination of the AC Josephson effect and an AC voltage. Analytical expressions for all harmonics in the driving frequency of both the current and the reduced dot operator are given for arbitrary driving strength. For the net DC current the resulting photon assisted processes give rise to rich current-voltage characteristics. In addition to photon assisted subgap transport we find regions of total current inversion in the stability diagram. There, the junction acts as a pump with the net DC current flowing against the applied DC bias. The first harmonic of the current, being closely related to the nonlinear dynamic susceptibility of the junction, is discussed at finite applied DC bias.
The combined action of a dc bias and a microwave drive on the transport characteristic of a superconductor-quantum dot-superconductor junction is investigated. To cope with time dependent nonequilibrium effects and interactions in the quantum dot, we develop a general formalism for the dynamics of the density operator based on a particle conserving approach to superconductivity. Without invoking a broken U(1) symmetry, we identify a dynamical phase connected to the coherent transfer of Cooper pairs across the junction. In the weak-coupling limit, we show that besides quasiparticle transport, proximity induced superconducting correlations manifest in anomalous pair tunneling involving the transfer of a Cooper pair. The resulting generalized master equation in presence of the microwave drive showcases the characteristic bichromatic response due to the combination of the ac Josephson effect and an ac voltage. Analytical expressions for all harmonics in the driving frequency of both the current and the reduced dot operator are given for arbitrary driving strength. For the net dc current, the resulting photon assisted processes give rise to rich current-voltage characteristics. In addition to photon assisted subgap transport, we find regions of total current inversion in the stability diagram. There, the junction acts as a pump with the net dc current flowing against the applied dc bias. The first harmonic of the current, being closely related to the nonlinear dynamic susceptibility of the junction, is discussed at finite applied dc bias.
We consider a Josephson junction formed by a quantum dot connected to two bulk superconductors in the presence of Coulomb interaction and coupling to both an electromagnetic environment and a finite density of electronic quasiparticles. In the limit of a large superconducting gap we obtain a Born-Markov description of the relevant Andreev bound-states dynamics. We calculate the current-phase relation and we find that the experimentally unavoidable presence of quasiparticles can dramatically modify the 0-π standard transition picture. We show that photon-assisted quasiparticle absorption allows the dynamic switching from the 0 to the π state and vice versa, washing out the 0-π transition predicted by purely thermodynamic arguments. Spectroscopic signatures of Andreev bound-states broadening are investigated by considering microwave irradiation.