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Physical review. B./Physical review. B

Particle conserving approach to ac-dc driven interacting quantum dots with superconducting leads

Julian Siegl, Jordi Picó-Cortés, Milena Grifoni

Published Mar 7, 2023• 5 citations
Publisher

Abstract

The combined action of a dc bias and a microwave drive on the transport characteristic of a superconductor-quantum dot-superconductor junction is investigated. To cope with time dependent nonequilibrium effects and interactions in the quantum dot, we develop a general formalism for the dynamics of the density operator based on a particle conserving approach to superconductivity. Without invoking a broken U(1) symmetry, we identify a dynamical phase connected to the coherent transfer of Cooper pairs across the junction. In the weak-coupling limit, we show that besides quasiparticle transport, proximity induced superconducting correlations manifest in anomalous pair tunneling involving the transfer of a Cooper pair. The resulting generalized master equation in presence of the microwave drive showcases the characteristic bichromatic response due to the combination of the ac Josephson effect and an ac voltage. Analytical expressions for all harmonics in the driving frequency of both the current and the reduced dot operator are given for arbitrary driving strength. For the net dc current, the resulting photon assisted processes give rise to rich current-voltage characteristics. In addition to photon assisted subgap transport, we find regions of total current inversion in the stability diagram. There, the junction acts as a pump with the net dc current flowing against the applied dc bias. The first harmonic of the current, being closely related to the nonlinear dynamic susceptibility of the junction, is discussed at finite applied dc bias.

DOI
10.1103/physrevb.107.115405

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The combined action of a dc bias and a microwave drive on the transport characteristic of a superconductor-quantum dot-superconductor junction is investigated. To cope with time dependent nonequilibrium effects and interactions in the quantum dot, we develop a general formalism for the dynamics of the density operator based on a particle conserving approach to superconductivity. Without invoking a broken U(1) symmetry, we identify a dynamical phase connected to the coherent transfer of Cooper pairs across the junction. In the weak-coupling limit, we show that besides quasiparticle transport, proximity induced superconducting correlations manifest in anomalous pair tunneling involving the transfer of a Cooper pair. The resulting generalized master equation in presence of the microwave drive showcases the characteristic bichromatic response due to the combination of the ac Josephson effect and an ac voltage. Analytical expressions for all harmonics in the driving frequency of both the current and the reduced dot operator are given for arbitrary driving strength. For the net dc current, the resulting photon assisted processes give rise to rich current-voltage characteristics. In addition to photon assisted subgap transport, we find regions of total current inversion in the stability diagram. There, the junction acts as a pump with the net dc current flowing against the applied dc bias. The first harmonic of the current, being closely related to the nonlinear dynamic susceptibility of the junction, is discussed at finite applied dc bias.
The combined action of a DC bias and a microwave drive on the transport characteristic of a superconductor-quantum dot-superconductor junction is investigated. To cope with time dependent non-equilibrium effects and interactions in the quantum dot, we develop a general formalism for the dynamics of the density operator based on a particle conserving approach to superconductivity. Without invoking a broken U (1) symmetry, we identify a dynamical phase connected to the coherent transfer of Cooper pairs across the junction. In the weak coupling limit, we show that besides quasiparticle transport, proximity induced superconducting correlations manifest in anomalous pair tunneling involving the transfer of a Cooper pair. The resulting generalized master equation in presence of the microwave drive showcases the characteristic bichromatic response due to the combination of the AC Josephson effect and an AC voltage. Analytical expressions for all harmonics in the driving frequency of both the current and the reduced dot operator are given for arbitrary driving strength. For the net DC current the resulting photon assisted processes give rise to rich current-voltage characteristics. In addition to photon assisted subgap transport we find regions of total current inversion in the stability diagram. There, the junction acts as a pump with the net DC current flowing against the applied DC bias. The first harmonic of the current, being closely related to the nonlinear dynamic susceptibility of the junction, is discussed at finite applied DC bias.
We investigate nonequilibrium transport through superconducting nanojunctions using a Liouville space approach. The formalism allows us to study finite-gap effects, and to account for both quasiparticle and Cooper-pair tunneling. With focus on the weak-tunneling limit, we study the stationary dc and ac current up to second order (cotunneling) in the hybridization energy. For the particular case of a strongly interacting quantum dot sandwiched between two superconductors, we identify the characteristic virtual processes that yield the Andreev and Josephson current and obtain the dependence on the gate and bias voltage for the dc current, the critical current, and the phase-dependent dissipative current. In particular, the critical current is characterized by regions in the stability diagram in which its sign changes from positive to negative, resulting in a multitude of $0\ensuremath{-}\ensuremath{\pi}$ transitions. The latter signal the interplay between strong interactions and tunneling at finite bias.
Abstract Dynamical processes induced by the external time-dependent fields can provide valuable insight into the characteristic energy scales of a given physical system. We investigate them here in a nanoscopic heterostructure, consisting of the double quantum dot coupled in series to the superconducting and the metallic reservoirs, analyzing its response to (i) abrupt bias voltage applied across the junction, (ii) sudden change of the energy levels, and imposed by (iii) their periodic driving. We explore subgap properties of this setup which are strictly related to the in-gap quasiparticles and discuss their signatures manifested in the time-dependent charge currents. The characteristic multi-mode oscillations, their beating patters and photon-assisted harmonics reveal a rich spectrum of dynamical features that might be important for designing the superconducting qubits.
Dynamical processes induced by the external time-dependent fields can provide valuable insight into the characteristic energy scales of a given physical system. We investigate them here in a nanoscopic heterostructure, consisting of the double quantum dot coupled in series to the superconducting and the metallic reservoirs, analyzing its response to (i) abrupt bias voltage applied across the junction, (ii) sudden change of the energy levels, and imposed by (iii) their periodic driving. We explore subgap properties of this setup which are strictly related to the in-gap quasiparticles and discuss their signatures manifested in the time-dependent charge currents. The characteristic multi-mode oscillations, their beating patters and photon-assisted harmonics reveal a rich spectrum of dynamical features that might be important for designing the superconducting qubits.
Josephson junctions based on quantum dots offer a convenient tunability by means of local gates. Here we analyze a Josephson junction based on a serial double quantum dot in which the two dots are individually gated by phase-shifted microwave tones of equal frequency. We calculate the time-averaged current across the junction and determine how the phase shift between the drives modifies the current-phase relation of the junction. Breaking particle-hole symmetry on the dots is found to give rise to a finite average anomalous Josephson current with phase bias between the superconductors fixed to zero. This microwave gated weak link thus realizes a tunable ``Floquet ${\ensuremath{\varphi}}_{0}$ junction'' with maximum critical current achieved for driving frequencies slightly off resonance with the subgap excitation energy. We provide numerical results supported by an analytical analysis for infinite superconducting gap and weak interdot coupling. We identify an interaction-driven $0\text{\ensuremath{-}}\ensuremath{\pi}$ transition of anomalous Josephson current as a function of driving phase difference. Finally, we show that this junction can be tuned so as to provide for complete rectification of the time-averaged Josephson current-phase relation.
We investigate non-equilibrium transport through interacting superconducting nanojunctions using a Liouville space approach. The formalism allows us to study finite gap effects, and to account for both quasiparticle and Cooper pair tunneling. With focus on the weak tunneling limit, we study the stationary dc and ac current up to second order (cotunneling) in the hybridization energy. We identify the characteristic virtual processes that yield the Andreev and Josephson current and obtain the dependence on the gate and bias voltage for the dc current, the critical current and the phase-dependent dissipative current. In particular, the critical current is characterized by regions in the stability diagram in which its sign changes from positive to negative, resulting in a multitude of 0-πtransitions. The latter signal the interplay between strong interactions and tunneling at finite bias.