Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Log inSign up
Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Blog
Job Board
Q3AS

© 2026 Aqora Quantum S.A.S.

TermsPrivacyLegal Notice

arXiv:1908.06125 · Physical review. B./Physical review. B

Postquench gap dynamics of two-band superconductors

Tianbai Cui, Michael Schütt, Peter P. Orth, Rafael M. Fernandes

Published Oct 23, 2019• 11 citations
arXivHTMLPDF

Abstract

Recent experimental progress in the fields of cold quantum gases and ultrafast optical spectroscopy of quantum materials allows us to controllably induce and probe nonadiabatic dynamics of superconductors and superfluids. The time evolution of the gap function before relaxation with the lattice is determined by the superposition of coherently evolving individual Cooper pairs within the manifold of the Bardeen-Cooper-Schrieffer (BCS) wave function. While dynamics following an abrupt quench of the pairing interaction strength in the single-band BCS model has been exactly solved due to the integrability of the model, the dynamics of postquench multiband superconductors remain under scrutiny. Here, we develop a generalization of the Volkov-Kogan Laplace-space perturbative method that allows us to determine the nonadiabatic gap dynamics of two-band fully gapped superconductors for a wide range of quench amplitudes. Our approach expands the long-time dynamics around the steady-state asymptotic value of the gap, which is self-consistently determined, rather than around the equilibrium value of the gap. We explicitly demonstrate that this method recovers the exact solution of the long-time gap dynamics in the single-band case and perfectly agrees with a numerical solution of the two-band model. We discover that dephasing of Cooper pairs from different bands leads to faster collisionless relaxation of the gap oscillation with a power law of ${t}^{\ensuremath{-}3/2}$ instead of the well-known ${t}^{\ensuremath{-}1/2}$ behavior found in the single-band case. Furthermore, the gap oscillations display beating patterns arising from the existence of two different asymptotic gap values. Our results have important implications to a variety of two-band superconductors driven out of equilibrium, such as iron-based superconductors, ${\mathrm{MgB}}_{2}$, and ${\mathrm{SrTiO}}_{3}$.

DOI
10.1103/physrevb.100.144513

Related papers

Collisionless dynamics of the pairing amplitude in disordered superconductors

Maxim Dzero

I consider relaxation of the pairing amplitude in a disordered Bardeen-Cooper-Schrieffer (BCS) superconductor in the absence of the two-particle collisions. My main assumption is that nonmagnetic and magnetic disorder scattering rates are much smaller than the value of the superconducting pairing gap ${\mathrm{\ensuremath{\Delta}}}_{0}$. I derive a system of nonlinear equations which describe the collisionless relaxation of the pairing amplitude following a quench of the pairing strength. I find that in a superconductor in which scattering on paramagnetic impurities is dominant, the pairing amplitude in a steady state varies periodically with time even for small deviations from equilibrium. It is shown that such a steady state emerges due to scattering on paramagnetic impurities which leads to a decrease in the value of the resonant frequency of the amplitude mode below $2{\mathrm{\ensuremath{\Delta}}}_{0}$.

arXiv:2303.06750•Physical review. B./Physical review. B•Mar 8, 2024•10 citations

Nonequilibrium dynamics from BCS to the bosonic limit

G. Seibold, J. Lorenzana

Within the time-dependent Gutzwiller approximation applied to the negative-$U$ Hubbard model, we investigate the dynamics of a superconductor after an interaction quench for different values of the final interaction from weak to strong coupling. The equilibrium BCS-BEC crossover becomes a sharp transition in the out-of-equilibrium dynamics between weak- and strong-coupling dynamical phases. Two different frequencies (${\mathrm{\ensuremath{\Omega}}}_{J}<{\mathrm{\ensuremath{\Omega}}}_{U}$) dominate the order parameter dynamics. In the weak coupling phase, ${\mathrm{\ensuremath{\Omega}}}_{J}$ follows twice the asymptotic average value of the gap (${\mathrm{\ensuremath{\Omega}}}_{J}\ensuremath{\approx}2{\mathrm{\ensuremath{\Delta}}}_{\ensuremath{\infty}}$) and ${\mathrm{\ensuremath{\Omega}}}_{U}$ is much larger but hardy visible in the anomalous density. At long times the BCS dynamics is recovered but surprisingly differences remain during the transient phase. In the strong coupling phase, the dynamics decouples from the asymptotic value of the order parameter except at exactly half filling and close to the dynamical transition where ${\mathrm{\ensuremath{\Omega}}}_{U}\ensuremath{\approx}2{\mathrm{\ensuremath{\Delta}}}_{\ensuremath{\infty}}$. The out-of-equilibrium transient spectral density and optical conductivity are presented and discussed in relation to pump probe experiments. Both ${\mathrm{\ensuremath{\Omega}}}_{J}$ and ${\mathrm{\ensuremath{\Omega}}}_{U}$ give rise to a complex structure of self-driven slow Rabi oscillations which are visible in the nonequilibrium optical conductivity where also sidebands appear due to the modulation of the double occupancy by superconducting amplitude oscillations. Analogous results apply to CDW and SDW systems. Our results show that in systems with long coherence times, pump-probe experiments allow us to characterize the regime (BCS vs preformed pairs) through very specific out-of-equilibrium fingerprints.

arXiv:2004.02454•Physical review. B./Physical review. B•Oct 5, 2020•12 citations

Novel Non–Equilibrium Dynamics in Superconductors: Induced Superconductivity and Higgs Modes

Nikolaj Bittner

This thesis reports on theoretical investigations of the ultrafast nonequilibrium dynamics in superconductors. In particular, two nonequilibrium scenarios are modeled by combining several analytical and numerical methods: transient superconducting phase transition and collective excitations of a superconducting condensate. In the first part of the thesis the possibility to induce singlet superconducting correlations far from equilibrium is explored by applying time-dependent Lanczos algorithm to the one-dimensional extended Hubbard model. Here, the system is driven into a nonequilibrium state by (i) interaction quench and (ii) quench by pulse. In both cases the buildup of the superconducting correlations is studied in view of several correlation functions. Moreover, a transient Meissner effect, which reflects fingerprints of the induced superconductivity, is observed in calculations of the important for experiments time-dependent optical conductivity. In addition, the differences between nonequilibrium dynamics of the extended Hubbard model initiated by interaction quench and by pulse quench are discussed in detail. The second part is devoted to the excitation of collective modes in a superconductor out of equilibrium. First of all, focus is given to the properties of collective modes close to equilibrium conditions, where a linearized response can be expected. Within the framework of the (Nambu-) matrix kinetic theory in the clean limit a comprehensive gauge-invariant description of the collective modes associated with phase fluctuations of the order parameter is analytically formulated for the generalized case of two- band superconducting systems. Particular emphasis is on the application to the recently discovered noncentrosymmetric superconductors. A detailed analysis of the collective modes includes specification of the gauge mode (common to all superconductors) and the Leggett mode (collective fluctuations of the interband phase difference), and investigation of their subtle interplay in view of validity of the charge conservation law and the participation in the Anderson-Higgs mechanism. Further, the nonequilibrium excitation of the superconducting gaps for the case of two-band superconductors with singlet pairing correlations is investigated in a view of optical pump-probe experiments. For this purpose a semi-numerical method based on the density- matrix theory is formulated. In this case additional amplitude (Higgs) modes were identified, which allow to directly detect the properties of the superconducting condensates as a function of time. Moreover, a new interplay between the phase (Leggett) and amplitude (Higgs) modes is studied in detail. In particular it was found that the nonadiabatic excitation process leads to strong coupling between both modes. Finally, based on calculations of the time-dependent optical conductivity the prediction is made that the coupled Higgs and Leggett modes can be clearly visible in the pump-probe absorption spectra.

•Jan 1, 2017•0 citations

Cooper pair insulators and theory of correlated superconductors

Predrag Nikolić, Zlatko Tešanović

The pseudogap state of cuprate high-temperature superconductors has been often viewed as either a yet unknown competing order or a precursor state to superconductivity. While awaiting the resolution of the pseudogap problem in cuprates, we demonstrate that local pairing fluctuations, vortex liquid dynamics, and other precursor phenomena can emerge quite generally whenever fermionic excitations remain gapped across the superconducting transition, regardless of the gap origin. Our choice of a tractable model is a lattice band insulator with short-range attractive interactions between fermions in the $s$-wave channel. An effective crossover between Bardeen-Cooper-Schrieffer (BCS) and Bose-Einstein condensate (BEC) regimes can be identified in any band insulator above two dimensions, while in two dimensions only the BEC regime exists. The superconducting transition is ``unconventional'' (non-pair-breaking) in the BEC regime, identified by either the bosonic mean field or $\mathit{XY}$ universality class. The insulator adjacent to the superconductor in the BEC regime is a bosonic Mott insulator of Cooper pairs, which may be susceptible to charge density wave ordering. We construct a function of the many-body excitation spectrum whose nonanalytic changes define a sharp distinction between band and Mott insulators. The corresponding ``second-order transition'' can be observed out of equilibrium by driving a Cooper pair laser in the Mott insulator. We explicitly show that the gap for charged bosonic excitations lies below the threshold for Cooper pair breakup in any BEC regime, despite quantum fluctuations. Our discussion ends with a view of possible consequences for cuprates, where antinodal pair dynamics has certain features in common with our simple $s$-wave picture.

arXiv:1008.4369•Physical Review B•Feb 2, 2011•16 citations

Coherent control of the gap dynamics of BCS superconductors in the nonadiabatic regime

Thomas Papenkort, T. Kühn, V. M. Axt

By exciting a BCS superconductor with ultrashort pulses in the frequency range of the superconducting gap a nonadiabatic regime can be reached. In this regime the modulus of the order parameter oscillates in time. Although its average value can be identified with the gap in the absorption spectrum, the oscillation itself remains invisible in pump-probe spectra. In this Brief Report we demonstrate that by employing a coherent control-type scheme of excitation by two phase-locked pump pulses this oscillation can be unveiled in the probe spectrum. We find that the reaction of the superconductor to a second pump pulse depends strongly on its instantaneous state at the time of the impact of the second pulse. Based on numerical calculations performed on the mean-field level it is shown that by varying the delay time between the two pump pulses the transient oscillation of the order parameter can be transformed into an oscillation of its long-time value, which shows up in the absorption spectrum of a subsequent weak probe pulse as an oscillation of the gap when plotted as a function of the delay time.

Physical Review B•Oct 9, 2008•59 citations

Consequences of integrability breaking in quench dynamics of pairing Hamiltonians

Jasen A. Scaramazza, Pietro Smacchia, Emil A. Yuzbashyan

We study the collisionless dynamics of two classes of nonintegrable pairing models. One is a Bardeen-Cooper-Schrieffer model with separable energy-dependent interactions, and the other is a two-dimensional topological superconductor with spin-orbit coupling and a band-splitting external field. The long-time quantum quench dynamics at integrable points of these models are well understood. Namely the squared magnitude of the time-dependent order parameter $\mathrm{\ensuremath{\Delta}}(t)$ can vanish (Phase I), reach a nonzero constant (Phase II), or periodically oscillate as an elliptic function (Phase III). We demonstrate that nonintegrable models, too, exhibit some or all of these nonequilibrium phases. Remarkably, elliptic periodic oscillations persist, even though both their amplitude and functional form change drastically with integrability breaking. Striking new phenomena accompany loss of integrability. First, an extremely long timescale emerges in the relaxation to Phase III, such that short-time numerical simulations risk erroneously classifying the asymptotic state. This timescale diverges near integrable points. Second, an entirely new Phase IV of quasiperiodic oscillations of $|\mathrm{\ensuremath{\Delta}}|$ emerges in the quantum quench phase diagrams of nonintegrable pairing models. As integrability techniques do not apply for the models we study, we develop the concept of asymptotic self-consistency and a linear stability analysis of the asymptotic phases. With the help of these new tools, we determine the phase boundaries, characterize the asymptotic state, and clarify the physical meaning of the quantum quench phase diagrams of BCS superconductors. We also propose an explanation of these diagrams in terms of bifurcation theory.

arXiv:1812.04410•Physical review. B./Physical review. B•Feb 28, 2019•15 citations
Recent experimental progress in the fields of cold quantum gases and ultrafast optical spectroscopy of quantum materials allows us to controllably induce and probe nonadiabatic dynamics of superconductors and superfluids. The time evolution of the gap function before relaxation with the lattice is determined by the superposition of coherently evolving individual Cooper pairs within the manifold of the Bardeen-Cooper-Schrieffer (BCS) wave function. While dynamics following an abrupt quench of the pairing interaction strength in the single-band BCS model has been exactly solved due to the integrability of the model, the dynamics of postquench multiband superconductors remain under scrutiny. Here, we develop a generalization of the Volkov-Kogan Laplace-space perturbative method that allows us to determine the nonadiabatic gap dynamics of two-band fully gapped superconductors for a wide range of quench amplitudes. Our approach expands the long-time dynamics around the steady-state asymptotic value of the gap, which is self-consistently determined, rather than around the equilibrium value of the gap. We explicitly demonstrate that this method recovers the exact solution of the long-time gap dynamics in the single-band case and perfectly agrees with a numerical solution of the two-band model. We discover that dephasing of Cooper pairs from different bands leads to faster collisionless relaxation of the gap oscillation with a power law of t\ensuremath−3/2{t}^{\ensuremath{-}3/2}t\ensuremath−3/2 instead of the well-known t\ensuremath−1/2{t}^{\ensuremath{-}1/2}t\ensuremath−1/2 behavior found in the single-band case. Furthermore, the gap oscillations display beating patterns arising from the existence of two different asymptotic gap values. Our results have important implications to a variety of two-band superconductors driven out of equilibrium, such as iron-based superconductors, MgB2{\mathrm{MgB}}_{2}MgB2​, and SrTiO3{\mathrm{SrTiO}}_{3}SrTiO3​.
I consider relaxation of the pairing amplitude in a disordered Bardeen-Cooper-Schrieffer (BCS) superconductor in the absence of the two-particle collisions. My main assumption is that nonmagnetic and magnetic disorder scattering rates are much smaller than the value of the superconducting pairing gap ${\mathrm{\ensuremath{\Delta}}}_{0}$. I derive a system of nonlinear equations which describe the collisionless relaxation of the pairing amplitude following a quench of the pairing strength. I find that in a superconductor in which scattering on paramagnetic impurities is dominant, the pairing amplitude in a steady state varies periodically with time even for small deviations from equilibrium. It is shown that such a steady state emerges due to scattering on paramagnetic impurities which leads to a decrease in the value of the resonant frequency of the amplitude mode below $2{\mathrm{\ensuremath{\Delta}}}_{0}$.
Within the time-dependent Gutzwiller approximation applied to the negative-UUU Hubbard model, we investigate the dynamics of a superconductor after an interaction quench for different values of the final interaction from weak to strong coupling. The equilibrium BCS-BEC crossover becomes a sharp transition in the out-of-equilibrium dynamics between weak- and strong-coupling dynamical phases. Two different frequencies (${\mathrm{\ensuremath{\Omega}}}_{J}<{\mathrm{\ensuremath{\Omega}}}_{U}$) dominate the order parameter dynamics. In the weak coupling phase, ${\mathrm{\ensuremath{\Omega}}}_{J}$ follows twice the asymptotic average value of the gap (${\mathrm{\ensuremath{\Omega}}}_{J}\ensuremath{\approx}2{\mathrm{\ensuremath{\Delta}}}_{\ensuremath{\infty}}$) and ${\mathrm{\ensuremath{\Omega}}}_{U}$ is much larger but hardy visible in the anomalous density. At long times the BCS dynamics is recovered but surprisingly differences remain during the transient phase. In the strong coupling phase, the dynamics decouples from the asymptotic value of the order parameter except at exactly half filling and close to the dynamical transition where ${\mathrm{\ensuremath{\Omega}}}_{U}\ensuremath{\approx}2{\mathrm{\ensuremath{\Delta}}}_{\ensuremath{\infty}}$. The out-of-equilibrium transient spectral density and optical conductivity are presented and discussed in relation to pump probe experiments. Both ${\mathrm{\ensuremath{\Omega}}}_{J}$ and ${\mathrm{\ensuremath{\Omega}}}_{U}$ give rise to a complex structure of self-driven slow Rabi oscillations which are visible in the nonequilibrium optical conductivity where also sidebands appear due to the modulation of the double occupancy by superconducting amplitude oscillations. Analogous results apply to CDW and SDW systems. Our results show that in systems with long coherence times, pump-probe experiments allow us to characterize the regime (BCS vs preformed pairs) through very specific out-of-equilibrium fingerprints.
This thesis reports on theoretical investigations of the ultrafast nonequilibrium dynamics in superconductors. In particular, two nonequilibrium scenarios are modeled by combining several analytical and numerical methods: transient superconducting phase transition and collective excitations of a superconducting condensate. In the first part of the thesis the possibility to induce singlet superconducting correlations far from equilibrium is explored by applying time-dependent Lanczos algorithm to the one-dimensional extended Hubbard model. Here, the system is driven into a nonequilibrium state by (i) interaction quench and (ii) quench by pulse. In both cases the buildup of the superconducting correlations is studied in view of several correlation functions. Moreover, a transient Meissner effect, which reflects fingerprints of the induced superconductivity, is observed in calculations of the important for experiments time-dependent optical conductivity. In addition, the differences between nonequilibrium dynamics of the extended Hubbard model initiated by interaction quench and by pulse quench are discussed in detail. The second part is devoted to the excitation of collective modes in a superconductor out of equilibrium. First of all, focus is given to the properties of collective modes close to equilibrium conditions, where a linearized response can be expected. Within the framework of the (Nambu-) matrix kinetic theory in the clean limit a comprehensive gauge-invariant description of the collective modes associated with phase fluctuations of the order parameter is analytically formulated for the generalized case of two- band superconducting systems. Particular emphasis is on the application to the recently discovered noncentrosymmetric superconductors. A detailed analysis of the collective modes includes specification of the gauge mode (common to all superconductors) and the Leggett mode (collective fluctuations of the interband phase difference), and investigation of their subtle interplay in view of validity of the charge conservation law and the participation in the Anderson-Higgs mechanism. Further, the nonequilibrium excitation of the superconducting gaps for the case of two-band superconductors with singlet pairing correlations is investigated in a view of optical pump-probe experiments. For this purpose a semi-numerical method based on the density- matrix theory is formulated. In this case additional amplitude (Higgs) modes were identified, which allow to directly detect the properties of the superconducting condensates as a function of time. Moreover, a new interplay between the phase (Leggett) and amplitude (Higgs) modes is studied in detail. In particular it was found that the nonadiabatic excitation process leads to strong coupling between both modes. Finally, based on calculations of the time-dependent optical conductivity the prediction is made that the coupled Higgs and Leggett modes can be clearly visible in the pump-probe absorption spectra.
The pseudogap state of cuprate high-temperature superconductors has been often viewed as either a yet unknown competing order or a precursor state to superconductivity. While awaiting the resolution of the pseudogap problem in cuprates, we demonstrate that local pairing fluctuations, vortex liquid dynamics, and other precursor phenomena can emerge quite generally whenever fermionic excitations remain gapped across the superconducting transition, regardless of the gap origin. Our choice of a tractable model is a lattice band insulator with short-range attractive interactions between fermions in the sss-wave channel. An effective crossover between Bardeen-Cooper-Schrieffer (BCS) and Bose-Einstein condensate (BEC) regimes can be identified in any band insulator above two dimensions, while in two dimensions only the BEC regime exists. The superconducting transition is ``unconventional'' (non-pair-breaking) in the BEC regime, identified by either the bosonic mean field or XY\mathit{XY}XY universality class. The insulator adjacent to the superconductor in the BEC regime is a bosonic Mott insulator of Cooper pairs, which may be susceptible to charge density wave ordering. We construct a function of the many-body excitation spectrum whose nonanalytic changes define a sharp distinction between band and Mott insulators. The corresponding ``second-order transition'' can be observed out of equilibrium by driving a Cooper pair laser in the Mott insulator. We explicitly show that the gap for charged bosonic excitations lies below the threshold for Cooper pair breakup in any BEC regime, despite quantum fluctuations. Our discussion ends with a view of possible consequences for cuprates, where antinodal pair dynamics has certain features in common with our simple sss-wave picture.
By exciting a BCS superconductor with ultrashort pulses in the frequency range of the superconducting gap a nonadiabatic regime can be reached. In this regime the modulus of the order parameter oscillates in time. Although its average value can be identified with the gap in the absorption spectrum, the oscillation itself remains invisible in pump-probe spectra. In this Brief Report we demonstrate that by employing a coherent control-type scheme of excitation by two phase-locked pump pulses this oscillation can be unveiled in the probe spectrum. We find that the reaction of the superconductor to a second pump pulse depends strongly on its instantaneous state at the time of the impact of the second pulse. Based on numerical calculations performed on the mean-field level it is shown that by varying the delay time between the two pump pulses the transient oscillation of the order parameter can be transformed into an oscillation of its long-time value, which shows up in the absorption spectrum of a subsequent weak probe pulse as an oscillation of the gap when plotted as a function of the delay time.
We study the collisionless dynamics of two classes of nonintegrable pairing models. One is a Bardeen-Cooper-Schrieffer model with separable energy-dependent interactions, and the other is a two-dimensional topological superconductor with spin-orbit coupling and a band-splitting external field. The long-time quantum quench dynamics at integrable points of these models are well understood. Namely the squared magnitude of the time-dependent order parameter $\mathrm{\ensuremath{\Delta}}(t)$ can vanish (Phase I), reach a nonzero constant (Phase II), or periodically oscillate as an elliptic function (Phase III). We demonstrate that nonintegrable models, too, exhibit some or all of these nonequilibrium phases. Remarkably, elliptic periodic oscillations persist, even though both their amplitude and functional form change drastically with integrability breaking. Striking new phenomena accompany loss of integrability. First, an extremely long timescale emerges in the relaxation to Phase III, such that short-time numerical simulations risk erroneously classifying the asymptotic state. This timescale diverges near integrable points. Second, an entirely new Phase IV of quasiperiodic oscillations of $|\mathrm{\ensuremath{\Delta}}|$ emerges in the quantum quench phase diagrams of nonintegrable pairing models. As integrability techniques do not apply for the models we study, we develop the concept of asymptotic self-consistency and a linear stability analysis of the asymptotic phases. With the help of these new tools, we determine the phase boundaries, characterize the asymptotic state, and clarify the physical meaning of the quantum quench phase diagrams of BCS superconductors. We also propose an explanation of these diagrams in terms of bifurcation theory.