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arXiv:0706.2620

Rhodium Mossbauer Supperadiance Induced by Liquid-Nitrogen Cooling

Cheng, Yao, Xia, Bing, Zhongming Wang

Published Jun 18, 2007• 1 citation
arXivHTMLPDF

Abstract

In the previous report, we have demonstrated cascade branching channels of the multipolar E3 transition of rhodium Mossbauer gamma via the time- and energy-resolved spectroscopy. Moreover, superradiance in the Borrmann channel from inverted nuclei gives gamma entanglement. In this letter, we report further four observations of superradiance and its associated gamma entanglement at the liquid-nitrogen temperature, i.e. (i) speed-up decay, (ii) immediate recovery of the speed-up decay after quenching, (iii) simultaneous suppression of gamma and K lines, and (iv) enhanced multiple ionizations. Anisotropic superradiant channels open by quenching and recover back immediately after quenching. Enhanced K satellites and K hypersatellites induced by cooling are attributed to the inelastic scattering of more than three entangled gammas.

DOI
10.48550/arxiv.0706.2620

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In the previous report, we have demonstrated cascade branching channels of the multipolar E3 transition of rhodium Mossbauer gamma via the time- and energy-resolved spectroscopy. Moreover, superradiance in the Borrmann channel from inverted nuclei gives gamma entanglement. In this letter, we report further four observations of superradiance and its associated gamma entanglement at the liquid-nitrogen temperature, i.e. (i) speed-up decay, (ii) immediate recovery of the speed-up decay after quenching, (iii) simultaneous suppression of gamma and K lines, and (iv) enhanced multiple ionizations. Anisotropic superradiant channels open by quenching and recover back immediately after quenching. Enhanced K satellites and K hypersatellites induced by cooling are attributed to the inelastic scattering of more than three entangled gammas.
Observation of possible stimulated emission of Mossbauer gamma is reported by liquid-nitrogen quenching of rhodium sample from room temperature to 77K in the time-resolved Mossbauer spectroscopy. Recently, we have demonstrated the anomalous emission of three entangled gammas of the E3 Mossbauer transition generated by bremsstrahlung irradiation. In this work, we further report the high-speed decay of excited state. We conjecture that cooling shrinkage, gravitational redshift and crystal lattice collimate entangled gammas in a linear cavity. This opens up a new approach towards gamma lasing, if the stimulated emission occurs at this obtained low excitation density.
We report the resonant propagation of the long-lived Mossbauer gamma in the time-resolved Mossbauer spectroscopy. Recently, three entangled gammas emitted from the E3 rhodium Mossbauer transition has been proposed to interpret the extraordinary observations in the previous report. Further observation reported here is the dynamic beat of these entangled gammas at room temperature and 77K. Apparent beat anisotropy reveals their long-distance resonant propagation, which leads to suppressed Doppler shift of entangled photon transport in the Borrmann channel.
We report experimental observations of the long-lived rhodium Mossbauer emissions by the time- and energy-resolved spectroscopy. The extraordinary observations manifest the open-up of photonic band gap in analogy to the superconducting gap of remarkable symmetry breakings at transition point. These observations are of potential importance for detecting gravitational waves and development of the two-photon gamma laser. Firstly, phase transitions shown by spectral evolution of characteristic emissions reveal the different aggregate exciton orderings at room temperature. Six different phases are identified by spectra profiles emitted from the color centers. Secondly, the cascade branching of the multipolar nuclear transition is discovered being the spontaneous cascade down-conversion to generate entangled gammas. The macroscopic angular distribution of entangled gammas from the polycrystalline sample manifests a global photon-nucleus-photon bound state across the grain boundaries. Thirdly, the gamma-energy distributions depending on exciton phases reveal the photonic band gap typically on the order of several hundred eV.
The effects of crystallinity are of crucial importance in considerations regarding gamma-ray lasers, bringing in new elements of laser theory which could well prove decisive in determining whether lasing can or cannot be achieved. Certain multibeam Borrmann eigenmodes of the radiation field within a perfect crystal containing resonant Mossbauer nuclei exhibit much less photoabsorption and much stronger coupling to the nuclei (provided the nuclear transition is of multipolarity M1 or higher) than do the single plane wave channels of an amorphous system (or equivalently, off-Bragg in the crystal). These modes offer the possibility of achieving lasing with orders of magnitude less population inversion density than would otherwise be the case, provided a nondestructive means is found to achieve a population inversion. The radiation in these modes would emerge from the crystal in a number of well-defined beams, each collimated by Bragg diffraction to an angular divergence of from 10-5to 10-4 rad. The properties of these multibeam modes as they relate to gamma-ray lasers, as well as the effects of crystallinity on the optics of systems which decay by superradiant rather than stimulate demission, are discussed.
We summarize the experimental observations of three case studies on the long-lived rhodium Mossbauer Effect. Extraordinary observations reported in this work manifest the open-up of photonic band gap in analogy to the superconducting gap. Observable gravitational effect is manifested by the superradiance of different sample orientations corresponding to the earth gravity. These observations are of potential importance for detecting gravitational waves and development of the two-photon gamma laser.
The electromagnetic transitions of Mössbauer nuclei provide ideal two-level systems to study the cooperative effects of X-rays with matter. Recently, we have observed the collective Lamb shift (CLS) in nuclear γ-ray superradiance [Röhlsberger, R.; Schlage, K.; Sahoo, B.; Couet, S.; Rüffer, R. Science 2010, 328, 1248–1251]. An ensemble of resonant 57Fe nuclei was embedded in the center of a planar cavity and was collectively excited by synchrotron radiation into a purely superradiant state. The decay of the superradiant state can be almost two orders of magnitude faster than the single-atom nuclear decay and can be accompanied by a CLS of more than 10 times the natural linewidth. Here we review the basic features of cooperative effects that occur in nuclear γ-ray superradiance in comparison with similar effects observed in the optical regime of the electromagnetic spectrum. We show that nuclear resonant scattering of synchrotron radiation opens new ways for systematic studies of cooperative effects in the interaction of X-rays with matter.