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arXiv:0706.2628

Phase Transition of Trapped Nuclear Exciton of Long-lived Rhodium Mossbauer States

Cheng, Yao, Xia, Bing

Published Jun 18, 2007• 2 citations
arXivHTMLPDF

Abstract

We report experimental observations of the long-lived rhodium Mossbauer emissions by the time- and energy-resolved spectroscopy. The extraordinary observations manifest the open-up of photonic band gap in analogy to the superconducting gap of remarkable symmetry breakings at transition point. These observations are of potential importance for detecting gravitational waves and development of the two-photon gamma laser. Firstly, phase transitions shown by spectral evolution of characteristic emissions reveal the different aggregate exciton orderings at room temperature. Six different phases are identified by spectra profiles emitted from the color centers. Secondly, the cascade branching of the multipolar nuclear transition is discovered being the spontaneous cascade down-conversion to generate entangled gammas. The macroscopic angular distribution of entangled gammas from the polycrystalline sample manifests a global photon-nucleus-photon bound state across the grain boundaries. Thirdly, the gamma-energy distributions depending on exciton phases reveal the photonic band gap typically on the order of several hundred eV.

DOI
10.48550/arxiv.0706.2628

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Summary form only given. Recently, it was predicted that laser radiation can be used to manipulate very efficiently nuclear transitions at gamma-ray energies in solids. It results in both drastic qualitative and strong qualitative modifications of the Mossbauer spectra under the action of coherent optical radiation. The solid sample represents a host matrix where high densities of the ions are embedded by doping. The ions should possess both Mossbauer gamma-ray and optical electronic transitions favorable for the desired effects to be observed. Basically one needs Mossbauer-active ions with strong and sharp optical lines. The latter condition is typically satisfied for rare-earth and transition-metal ions in crystalline hosts and, remarkably, the majority of them are also Mossbauer-active.

APS•Mar 1, 2000•0 citations
We report experimental observations of the long-lived rhodium Mossbauer emissions by the time- and energy-resolved spectroscopy. The extraordinary observations manifest the open-up of photonic band gap in analogy to the superconducting gap of remarkable symmetry breakings at transition point. These observations are of potential importance for detecting gravitational waves and development of the two-photon gamma laser. Firstly, phase transitions shown by spectral evolution of characteristic emissions reveal the different aggregate exciton orderings at room temperature. Six different phases are identified by spectra profiles emitted from the color centers. Secondly, the cascade branching of the multipolar nuclear transition is discovered being the spontaneous cascade down-conversion to generate entangled gammas. The macroscopic angular distribution of entangled gammas from the polycrystalline sample manifests a global photon-nucleus-photon bound state across the grain boundaries. Thirdly, the gamma-energy distributions depending on exciton phases reveal the photonic band gap typically on the order of several hundred eV.
We summarize the experimental observations of three case studies on the long-lived rhodium Mossbauer Effect. Extraordinary observations reported in this work manifest the open-up of photonic band gap in analogy to the superconducting gap. Observable gravitational effect is manifested by the superradiance of different sample orientations corresponding to the earth gravity. These observations are of potential importance for detecting gravitational waves and development of the two-photon gamma laser.
In a previous report, we have shown that the rhodium lattice consisting of resonant nuclei is an ideal photonic crystal in nature. Plenty of extraordinary observations are attributed to the collective down conversion of the multipolar nuclear transition; in particular the spontaneous open up of photonic band gap. Emissions of directionality depending on the macroscopic geometry manifest that the standing wave is global in the polycrystalline sample. In this work, further observations of the directional emissions are summarized. By applying an external magnetic field at room temperature, not only the predicted macroscopic nuclear polarization but also its strong directionality are demonstrated. The standing wave lasts for more than hundred hours at room temperature in the single crystal despite its natural half-life of one hour. The so-called nuclear Raman Effect between two M4 transitions of 193mIr and 195mPt and the E3 transition of 103mRh is discovered, which gives the brand new aspects to detect gravitational waves.
We report the resonant propagation of the long-lived Mossbauer gamma in the time-resolved Mossbauer spectroscopy. Recently, three entangled gammas emitted from the E3 rhodium Mossbauer transition has been proposed to interpret the extraordinary observations in the previous report. Further observation reported here is the dynamic beat of these entangled gammas at room temperature and 77K. Apparent beat anisotropy reveals their long-distance resonant propagation, which leads to suppressed Doppler shift of entangled photon transport in the Borrmann channel.
Observation of possible stimulated emission of Mossbauer gamma is reported by liquid-nitrogen quenching of rhodium sample from room temperature to 77K in the time-resolved Mossbauer spectroscopy. Recently, we have demonstrated the anomalous emission of three entangled gammas of the E3 Mossbauer transition generated by bremsstrahlung irradiation. In this work, we further report the high-speed decay of excited state. We conjecture that cooling shrinkage, gravitational redshift and crystal lattice collimate entangled gammas in a linear cavity. This opens up a new approach towards gamma lasing, if the stimulated emission occurs at this obtained low excitation density.
In the previous report, we have demonstrated cascade branching channels of the multipolar E3 transition of rhodium Mossbauer gamma via the time- and energy-resolved spectroscopy. Moreover, superradiance in the Borrmann channel from inverted nuclei gives gamma entanglement. In this letter, we report further four observations of superradiance and its associated gamma entanglement at the liquid-nitrogen temperature, i.e. (i) speed-up decay, (ii) immediate recovery of the speed-up decay after quenching, (iii) simultaneous suppression of gamma and K lines, and (iv) enhanced multiple ionizations. Anisotropic superradiant channels open by quenching and recover back immediately after quenching. Enhanced K satellites and K hypersatellites induced by cooling are attributed to the inelastic scattering of more than three entangled gammas.
Summary form only given. Recently, it was predicted that laser radiation can be used to manipulate very efficiently nuclear transitions at gamma-ray energies in solids. It results in both drastic qualitative and strong qualitative modifications of the Mossbauer spectra under the action of coherent optical radiation. The solid sample represents a host matrix where high densities of the ions are embedded by doping. The ions should possess both Mossbauer gamma-ray and optical electronic transitions favorable for the desired effects to be observed. Basically one needs Mossbauer-active ions with strong and sharp optical lines. The latter condition is typically satisfied for rare-earth and transition-metal ions in crystalline hosts and, remarkably, the majority of them are also Mossbauer-active.