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arXiv:quant-ph/0611031

Possible Stimulated Emission of Entangled Rhodium Mossbauer Gammas

Cheng Yao, Wang, Zhongming

Published Nov 2, 2006• 1 citation
arXivHTMLPDF

Abstract

Observation of possible stimulated emission of Mossbauer gamma is reported by liquid-nitrogen quenching of rhodium sample from room temperature to 77K in the time-resolved Mossbauer spectroscopy. Recently, we have demonstrated the anomalous emission of three entangled gammas of the E3 Mossbauer transition generated by bremsstrahlung irradiation. In this work, we further report the high-speed decay of excited state. We conjecture that cooling shrinkage, gravitational redshift and crystal lattice collimate entangled gammas in a linear cavity. This opens up a new approach towards gamma lasing, if the stimulated emission occurs at this obtained low excitation density.

DOI
10.48550/arxiv.quant-ph/0611031

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Summary form only given. Recently, it was predicted that laser radiation can be used to manipulate very efficiently nuclear transitions at gamma-ray energies in solids. It results in both drastic qualitative and strong qualitative modifications of the Mossbauer spectra under the action of coherent optical radiation. The solid sample represents a host matrix where high densities of the ions are embedded by doping. The ions should possess both Mossbauer gamma-ray and optical electronic transitions favorable for the desired effects to be observed. Basically one needs Mossbauer-active ions with strong and sharp optical lines. The latter condition is typically satisfied for rare-earth and transition-metal ions in crystalline hosts and, remarkably, the majority of them are also Mossbauer-active.

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Observation of possible stimulated emission of Mossbauer gamma is reported by liquid-nitrogen quenching of rhodium sample from room temperature to 77K in the time-resolved Mossbauer spectroscopy. Recently, we have demonstrated the anomalous emission of three entangled gammas of the E3 Mossbauer transition generated by bremsstrahlung irradiation. In this work, we further report the high-speed decay of excited state. We conjecture that cooling shrinkage, gravitational redshift and crystal lattice collimate entangled gammas in a linear cavity. This opens up a new approach towards gamma lasing, if the stimulated emission occurs at this obtained low excitation density.
We report the resonant propagation of the long-lived Mossbauer gamma in the time-resolved Mossbauer spectroscopy. Recently, three entangled gammas emitted from the E3 rhodium Mossbauer transition has been proposed to interpret the extraordinary observations in the previous report. Further observation reported here is the dynamic beat of these entangled gammas at room temperature and 77K. Apparent beat anisotropy reveals their long-distance resonant propagation, which leads to suppressed Doppler shift of entangled photon transport in the Borrmann channel.
In the previous report, we have demonstrated cascade branching channels of the multipolar E3 transition of rhodium Mossbauer gamma via the time- and energy-resolved spectroscopy. Moreover, superradiance in the Borrmann channel from inverted nuclei gives gamma entanglement. In this letter, we report further four observations of superradiance and its associated gamma entanglement at the liquid-nitrogen temperature, i.e. (i) speed-up decay, (ii) immediate recovery of the speed-up decay after quenching, (iii) simultaneous suppression of gamma and K lines, and (iv) enhanced multiple ionizations. Anisotropic superradiant channels open by quenching and recover back immediately after quenching. Enhanced K satellites and K hypersatellites induced by cooling are attributed to the inelastic scattering of more than three entangled gammas.
We report experimental observations of the long-lived rhodium Mossbauer emissions by the time- and energy-resolved spectroscopy. The extraordinary observations manifest the open-up of photonic band gap in analogy to the superconducting gap of remarkable symmetry breakings at transition point. These observations are of potential importance for detecting gravitational waves and development of the two-photon gamma laser. Firstly, phase transitions shown by spectral evolution of characteristic emissions reveal the different aggregate exciton orderings at room temperature. Six different phases are identified by spectra profiles emitted from the color centers. Secondly, the cascade branching of the multipolar nuclear transition is discovered being the spontaneous cascade down-conversion to generate entangled gammas. The macroscopic angular distribution of entangled gammas from the polycrystalline sample manifests a global photon-nucleus-photon bound state across the grain boundaries. Thirdly, the gamma-energy distributions depending on exciton phases reveal the photonic band gap typically on the order of several hundred eV.
We summarize the experimental observations of three case studies on the long-lived rhodium Mossbauer Effect. Extraordinary observations reported in this work manifest the open-up of photonic band gap in analogy to the superconducting gap. Observable gravitational effect is manifested by the superradiance of different sample orientations corresponding to the earth gravity. These observations are of potential importance for detecting gravitational waves and development of the two-photon gamma laser.
The purpose of this paper is to describe a method for observing stimulated emission of gamma radiation. Stimulated emission of gamma radiation has never been observed. Stimulated emission of gamma radiation will be essential for developing gamma-ray lasers. The method uses the ‘π phase-shift induced transparency’ of gamma radiation, previously called the ‘gamma echo’. The gamma-echo technique is based on a modification of the time-differential Mössbauer spectroscopic method, i.e. the source is moved ‘instantaneously’ during the lifetime of the excited state. Then a resonant absorber becomes transparent to the resonant gamma radiation. There is a type of ‘self-stimulated’ emission in which the radiation ‘absorbed’, before the phase shift, is stimulated to emit after the phase shift. To observe stimulated emission of the resonant gamma radiation, one performs the same gamma-echo experiment except the resonant absorber is replaced by another source. This secondary source is chosen to be in resonance with the original source. Under these conditions there will be no stimulated emission, in the secondary source, before the π phase shift because the incident radiation is absorbed. However, after the phase shift, the secondary source becomes transparent to the incident radiation. If one uses a matched pair of Co57 sources and the secondary source is 2mCi, there will be about 3 nuclei in the secondary source, in the first excited state of Fe57, that are available to be stimulated during the 97.8ns lifetime of the primary source radiation.
Summary form only given. Recently, it was predicted that laser radiation can be used to manipulate very efficiently nuclear transitions at gamma-ray energies in solids. It results in both drastic qualitative and strong qualitative modifications of the Mossbauer spectra under the action of coherent optical radiation. The solid sample represents a host matrix where high densities of the ions are embedded by doping. The ions should possess both Mossbauer gamma-ray and optical electronic transitions favorable for the desired effects to be observed. Basically one needs Mossbauer-active ions with strong and sharp optical lines. The latter condition is typically satisfied for rare-earth and transition-metal ions in crystalline hosts and, remarkably, the majority of them are also Mossbauer-active.