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Journal of Modern Optics

The collective Lamb shift in nuclear γ-ray superradiance

Ralf Röhlsberger

Published Aug 12, 2010• 4 citations
Publisher

Abstract

The electromagnetic transitions of Mössbauer nuclei provide ideal two-level systems to study the cooperative effects of X-rays with matter. Recently, we have observed the collective Lamb shift (CLS) in nuclear γ-ray superradiance [Röhlsberger, R.; Schlage, K.; Sahoo, B.; Couet, S.; Rüffer, R. Science 2010, 328, 1248–1251]. An ensemble of resonant 57Fe nuclei was embedded in the center of a planar cavity and was collectively excited by synchrotron radiation into a purely superradiant state. The decay of the superradiant state can be almost two orders of magnitude faster than the single-atom nuclear decay and can be accompanied by a CLS of more than 10 times the natural linewidth. Here we review the basic features of cooperative effects that occur in nuclear γ-ray superradiance in comparison with similar effects observed in the optical regime of the electromagnetic spectrum. We show that nuclear resonant scattering of synchrotron radiation opens new ways for systematic studies of cooperative effects in the interaction of X-rays with matter.

DOI
10.1080/09500340.2010.506248

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The electromagnetic transitions of Mössbauer nuclei provide ideal two-level systems to study the cooperative effects of X-rays with matter. Recently, we have observed the collective Lamb shift (CLS) in nuclear γ-ray superradiance [Röhlsberger, R.; Schlage, K.; Sahoo, B.; Couet, S.; Rüffer, R. Science 2010, 328, 1248–1251]. An ensemble of resonant 57Fe nuclei was embedded in the center of a planar cavity and was collectively excited by synchrotron radiation into a purely superradiant state. The decay of the superradiant state can be almost two orders of magnitude faster than the single-atom nuclear decay and can be accompanied by a CLS of more than 10 times the natural linewidth. Here we review the basic features of cooperative effects that occur in nuclear γ-ray superradiance in comparison with similar effects observed in the optical regime of the electromagnetic spectrum. We show that nuclear resonant scattering of synchrotron radiation opens new ways for systematic studies of cooperative effects in the interaction of X-rays with matter.
Abstract The narrow nuclear resonances of Mössbauer isotopes constitute almost ideal two‐level systems to study cooperative effects in the interaction of x‐rays with matter. Embedding an ensemble of resonant Mössbauer nuclei into a planar cavity facilitates the excitation of superradiant oscillatory eigenmodes via pulses of synchrotron radiation. These modes exhibit a large collective Lamb shift that can be controlled via the excitation conditions and the cavity geometry. Cooperative emission in connection with the radiative coupling of two resonant ensembles in a cavity leads to electromagnetically induced transparency (EIT). This contribution gives a review on cooperative effects in nuclear resonant scattering of synchrotron radiation. Special emphasis is given to the basic principles of recent experiments that led to the observation of the collective Lamb shift and EIT with nuclear resonances in the regime of hard x‐rays.
Superradiance, the cooperative spontaneous emission of photons from an ensemble of identical atoms, provides valuable insights into the many-body physics of photons and atoms. We show that an ensemble of resonant atoms embedded in the center of a planar cavity can be collectively excited by synchrotron radiation into a purely superradiant state. The collective coupling of the atoms via the radiation field leads to a substantial radiative shift of the transition energy, the collective Lamb shift. We simultaneously measured the temporal evolution of the superradiant decay and the collective Lamb shift of resonant 57Fe nuclei excited with 14.4-kilo-electron volt synchrotron radiation. Our experimental technique provides a simple method for spectroscopic analysis of the superradiant emission.
This thesis is dedicated to the study of collective effects of nuclei in single xray photon superradiance. To this end we investigate aspects of superradiance in both nuclear forward scattering and in thin-film cavities with an embedded 57Fe nuclear layer. A general theoretical framework is developed to investigate a single-photon cooperative emission from a cloud of resonant systems, atoms or nuclei, in the presence of magnetic hyperfine splitting. In the limit of a thick sample, we present our results for two means to coherently control the collective single x-ray photon emission in nuclear forward scattering. In the limit of a thin sample in a thin-film cavity with embedded resonant nuclei, we find out that unlike the magnetic hyperfine splitting of a single atom or nucleus, interesting collective effects may occur which modify the hyperfine level structure. In addition, for a certain parameter regime a spectrum reminiscent of electromagnetically induced transparency (EIT) can be achieved. Based on this EIT-like effect, a theoretical control mechanism for stopping x-ray pulses in the thin-film x-ray cavity is put forward. Finally, we show theoretically that for the case of two nuclear ensembles in the thin-film cavity, pseudo-Rabi splitting due to the strong coupling between the two layers should occur. The latter findings are confirmed by preliminary experimental data.
Superradiance is one of the many fascinating phenomena predicted by quantum electrodynamics that have first been experimentally demonstrated in atomic systems and more recently in condensed matter systems like quantum dots, superconducting q-bits, cyclotron transitions and plasma oscillations in quantum wells (QWs). It occurs when a dense collection of N identical two-level emitters are phased via the exchange of photons, giving rise to enhanced light-matter interaction, hence to a faster emission rate. Of great interest is the regime where the ensemble interacts with one photon only and therefore all of the atoms, but one, are in the ground state. In this case the quantum superposition of all possible configurations produces a symmetric state that decays radiatively with a rate N times larger than that of the individual oscillators. This phenomenon, called single photon superradiance, results from the exchange of real photons among the N emitters. Yet, to single photon superradiance is also associated another collective effect that renormalizes the emission frequency, known as cooperative Lamb shift. In this work, we show that single photon superradiance and cooperative Lamb shift can be engineered in a semiconductor device by coupling spatially separated plasma resonances arising from the collective motion of confined electrons in QWs. These resonances hold a giant dipole along the growth direction z and have no mutual Coulomb coupling. They thus behave as a collection of macro-atoms on different positions along the z axis. Our device is therefore a test bench to simulate the low excitation regime of quantum electrodynamics.
In an ensemble of identical atoms, cooperative effects like sub- and superradiance may alter the decay rates and the energies of specific transitions may be shifted from the single-atom value by the so-called collective Lamb shift. While such effects in ensembles of two-level systems are by now well understood, realistic multilevel systems are more difficult to handle. In this work we show that in a system of atoms under the action of an external magnetic field, the collective contribution to the level shifts can amount to sizable quantitative and qualitative deviations from the single-atom Zeeman splitting picture. We develop a formalism to describe single-photon superradiance in multilevel systems and identify three-parameter regimes, two of which present measurable deviations in the radiation spectrum compared to the case of single-atom magnetic-field-induced splitting.
Superradiant burst often arises from photon-mediated interactions within an excited ensemble of emitters, where collective emission leads to a sharp increase in photon intensity. Here, we focus on a nuclear ensemble with cooperative excitations and propose, for the first time, the generation of superradiant burst of x-ray photons. We establish the required excitation conditions to observe x-ray superradiant bursts, offering guidance for the experiments utilizing state-of-the-art x-ray sources. Building on this, we investigate the dynamics of the x-ray superradiant burst and reveal novel nonlinear relationships between the time required to reach the peak intensity and the excitation number, as well as between the peak intensity and the excitation number. Additionally, we introduce a dimensionless parameter that serves as an indicator of the system, reflecting how strongly the burst can occur in a given configuration. Our work provides fresh insights into the understanding of collective emission in many-body x-ray-nuclei systems within the nonlinear regime, opening new avenues for x-ray quantum optics.