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arXiv:quant-ph/0702220 · International Journal of Modern Physics B

GENERATION OF HIGHER ORDER NONCLASSICAL STATES VIA AN INTENSE ELECTROMAGNETIC FIELD

Anirban Pathak

Published May 20, 2006• 1 citation
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Abstract

Interaction of intense laser beam with an inversion symmetric third order nonlinear medium is modeled as a quartic anharmonic oscillator. A first order operator solution of the model Hamiltonian is used to study the possibilities of generation of higher order nonclassical states. It is found that the higher order squeezed and higher order antibunched states can be produced by this interaction. It is also shown that the higher order nonclassical states may appear separately, i.e. a higher order antibunched state is not essentially higher order squeezed state and vice versa.

DOI
10.1142/s0217979206034029

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Interaction of intense laser beam with an inversion symmetric third order nonlinear medium is modeled as a quartic anharmonic oscillator. A first order operator solution of the model Hamiltonian is used to study the possibilities of generation of higher order nonclassical states. It is found that the higher order squeezed and higher order antibunched states can be produced by this interaction. It is also shown that the higher order nonclassical states may appear separately, i.e. a higher order antibunched state is not essentially higher order squeezed state and vice versa.
Coherent light interacting with a nonlinear nonabsorbing medium of inversion symmetry is modelled as a quartic anharmonic oscillator if the lowest (i.e. third) order of nonlinearity is considered. The equation of motion of the quadrature operators of such an oscillator is solved approximately in a closed analytical form. The corresponding solution is used to investigate the possibility of finding the continuous squeezed states. It is found that the amount of squeezing is increased with the increase of intensity of the applied field. An improvement of the squeezing is also possible if the coupling strength is increased. We report the squeezing effect of the input vacuum field. The possibility of generating continuous squeezing in an absolute sense (i.e. 100%) of the input radiation field is also discussed.
The interaction of coherent light with a nonlinear medium is modeled here by a general quantum anharmonic oscillator. The model is not exactly solvable in a closed analytical form. But we need operator solutions of the equations of motion corresponding to these models in order to study the quantum fluctuations of coherent light in nonlinear media. In the present work we derive approximate operator solutions. From these solutions we observe that there exists an apparent discrepancy between the solutions obtained by different techniques. We compare different solutions and conclude that all correct solutions are equivalent and the apparent discrepancy is due to the use of different ordering of the operators. We use these solutions to investigate the possibilities of observing different optical phenomena in a nonlinear dielectric medium. To be precise, we have studied quantum phase fluctuations of coherent light in a third order inversion symmetric nonlinear medium. Fluctuations in phase space quadrature for the same system are studied and the possibility of generating squeezed state is reported. Fluctuations in photon number are studied and the nonclassical phenomenon of antibunching is predicted. We have generalized the results obtained for third order nonlinear medium and have studied the interaction of an intense laser beam with a general (m-1)-th order nonlinear medium. Aharanov Anandan nonadiabatic geometric phase is also discussed in the context of (m-1)-th order nonlinear medium.
Higher-order nonclassical properties of fields propagating through a codirectional asymmetric nonlinear optical coupler which is prepared by combining a linear waveguide and a nonlinear (quadratic) waveguide operated by second harmonic generation are studied. A completely quantum mechanical description is used here to describe the system. Closed form analytic solutions of Heisenberg's equations of motion for various modes are used to show the existence of higher-order antibunching, higher-order squeezing, and higher-order two-mode and multimode entanglement in the asymmetric nonlinear optical coupler. It is also shown that nonclassical properties of light can transfer from a nonlinear waveguide to a linear waveguide.
We present an analytical framework for the emergence of nonclassical radiation in strongly laser-driven quantum systems, with a focus on high-order harmonic generation (HHG). Starting from a Pauli-Fierz description, we employ a parametric factorization of the coupled light-matter wavefunction that reduces the dynamics to coupled equations for a field-driven electronic state and a quantized light mode. Within this framework, we identify a simple and predictive mechanism for nonclassicality: it originates from the nonlinear dependence of the electronic dipole response on the light-mode coordinate. An approximately constant dipole yields coherent radiation, a linear dependence produces squeezing, and higher-order nonlinearities give rise to Wigner-function negativity. We illustrate this mechanism for atomic and molecular model systems and analyze its scaling in multi-emitter configurations, indicating routes toward high-photon-number nonclassical radiation in HHG. Our results provide a transparent connection between strong-field dynamics and quantum-optical properties of emitted light, offering a basis for engineering nonclassical states in intense laser-matter interactions.
The nonclassical effects of light in the fifth harmonic generation are investigated by quantum mechanically up to the first-order Hamiltonian interaction. The coupled Heisenberg equations of motion involving real and imaginary parts of the quadrature operators are established. The occurrence of amplitude squeezing effects in both quadratures of the radiation field in the fundamental mode is investigated and found to be dependent on the selective phase values of the field amplitude. The photon statistics in the fundamental mode have also been investigated and found to be sub-Poissonian in nature. It is observed that there is no possibility to produce squeezed light in the harmonic mode up to first-order Hamiltonian interaction. Further, we have found that the normal squeezing in the harmonic mode directly depends upon the fifth power of the field amplitude of the initial pump field up to second-order Hamiltonian interaction. This gives a method of converting higher-order squeezing in the fundamental mode into normal squeezing in the harmonic mode and vice versa. The analytic expression of fifth-order squeezing of the fundamental mode in the fifth harmonic generation is established.