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arXiv:quant-ph/0505186 · Journal of Modern Optics

EIT and diffusion of atomic coherence

Irina V. Novikova, Yanhong Xiao, David F. Phillips, Ronald Lee Walsworth

Published Nov 10, 2005• 33 citations
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Abstract

We study experimentally the effect of diffusion of Rb atoms on electromagnetically induced transparency (EIT) in a buffer gas vapour cell. In particular, we find that diffusion of atomic coherence in and out of the laser beam plays a crucial role in determining the EIT resonance lineshape and the stored light lifetime.
DOI
10.1080/09500340500275637

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In a recent paper [Y. Xiao et al., Phys. Rev. Lett. 96, 043601 (2006)] we characterized diffusion-induced Ramsey narrowing as a general phenomenon, in which diffusion of coherence in-and-out of an interaction region such as a laser beam induces spectral narrowing of the associated resonance lineshape. Here we provide a detailed presentation of the repeated interaction model of diffusion-induced Ramsey narrowing, with particular focus on its application to Electromagnetically Induced Transparency (EIT) of atomic vapor in a buffer gas cell. We compare this model both to experimental data and numerical calculations.
Electromagnetically induced transparency (EIT) due to Zeeman coherences in the Rb buffer gas cell is studied for different laser beam profiles, laser beam radii and intensities from 0.1 to 10 mW cm −2 . EIT line shapes can be approximated by the Lorentzian for wide Gaussian laser beam (6.5 mm in diameter) if laser intensity is weak and for a Π laser beam profile of the same diameter. Line shapes of EIT become non-Lorentzian for the Gaussian laser beam if it is narrow (1.3 mm in diameter) or if it has a higher intensity. EIT amplitudes and linewidths, for both laser beam profiles of the same diameter, have very similar behaviour regarding laser intensity and Rb cell temperature. EIT amplitudes are maximal at a certain laser beam intensity and this intensity is higher for narrower laser beams. The EIT linewidth estimated at zero laser intensity is about 50 nT or 0.7 kHz, which refers to 1.5 ms relaxation times of Zeeman coherences in 87 Rb atoms in our buffer gas cell. Blocking of the centre of the wide Gaussian laser beam in front of the photo detector yields Lorentzian profiles with a much better contrast to the linewidth ratio for EIT at higher intensities, above ∼2 mW cm −2 .
We report an experimental observation of the variation in linewidth of the electromagnetically induced transparency (EIT) resonance in a three-level ?-type system for several laser bandwidths in a Rb vapor cell, with and without a buffer gas. It is found, using narrow bandwidth (about 20 kHz) diode laser for both coupling and probe beams, that the linewidth of the EIT resonance can be significantly narrowed in the Rb vapor cell with the buffer gas. The results are in good qualitative agreement with a simple theoretical calculation.
We experimentally studied the effects of laser beam diameter on electromagnetically induced transparency (EIT) due to Zeeman coherences induced by a laser resonant with the hyperfine transition Fg = 2 → Fe = 1 of 87Rb in a rubidium buffer gas cell. We use two laser beams of Gaussian intensity radial profile for laser beam diameters of 6.5 and 1.3 mm, laser intensities in the range of 0.1–35 mW cm−2 and cell temperatures between 60 and 82 °C. The results show that the amplitude of the normalized EIT resonance has a maximum at a laser intensity which depends on laser beam diameter and cell temperature. The laser intensity corresponding to the maximum EIT amplitude is higher for a smaller laser beam and higher cell temperature. The linewidth of Zeeman EIT resonance varies nearly linearly with laser intensity, almost independent of cell temperature and laser beam diameter.