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arXiv:quant-ph/0410064 · Physical Review Letters

Energy-Time Entanglement Preservation in Plasmon-Assisted Light Transmission

Sylvain Fasel, F. Robin, Esteban Moreno, Daniel Erni, Nicolas Gisin, Hugo Zbinden

Published Mar 21, 2005• 171 citations
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Abstract

We report on experimental evidence of the preservation of the energy-time entanglement of a pair of photons after a photon-plasmon-photon conversion. This preservation is observed in two different plasmon conversion experiments, namely, extraordinary optical transmission through subwavelength metallic hole arrays and long range surface plasmon propagation in metallic waveguides. Plasmons are shown to coherently exist at two different times separated by much more than their lifetimes. This kind of entanglement involving light and matter is expected to be useful for future processing and storing of quantum information.

DOI
10.1103/physrevlett.94.110501

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We report on experimental evidence of the preservation of the energy-time entanglement of a pair of photons after a photon-plasmon-photon conversion. This preservation is observed in two different plasmon conversion experiments, namely, extraordinary optical transmission through subwavelength metallic hole arrays and long range surface plasmon propagation in metallic waveguides. Plasmons are shown to coherently exist at two different times separated by much more than their lifetimes. This kind of entanglement involving light and matter is expected to be useful for future processing and storing of quantum information.
We experimentally study two-photon coherence in plasmon-assisted transmission with a two-photon Mach-Zehnder (MZ) interferometer. Two collinear photons of identical or orthogonal polarization are simultaneously incident on one optically thick metal film, perforated with a periodic array of subwavelength holes. The de Broglie wavelength of plasmon-assisted transmitted photons is measured, which shows that two photons are re-eradiated by the plasmons and the quantum coherence of biphoton is preserved in the conversion process of transforming biphoton to plasmons and then back to biphoton.
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Two-photon states emitted from spontaneous parametric downconversion (SPDC) can exhibit quantum correlations in various degrees of freedom. On the other hand, plasmonic nanostructures show enhanced transmission thanks to the conversion of light into surface plasmon polaritons. It has been shown previously that polarization, time-energy and orbital angular momentum entanglement are preserved in such structures. The fact that surface plasmons are collective charge density waves, consisting of billions of electrons makes this observation remarkable. Here we show that spatial entanglement is also preserved by characterizing it after the photons interacted with gold nanopillar arrays. The detection is realized with novel single photon avalanche diode (SPAD) arrays with high spatial and temporal resolution. By measuring the spatial correlations of the photon in the near- and far-fields, we can characterize the state with respect to spatial entanglement with and without the nano-structure.
We experimentally demonstrated preservation of indistinguishability between two photons via mode conversions, namely, photon-to-plasmon and plasmon-to-photon conversions. A two-photon interference experiment was carried out using a broadband photon pair generated through a spontaneous parametric downconversion process. We observed the so-called Hong-Ou-Mandel dip with an interferometer including a 1-mm-long surface-plasmon-polariton (SPP) waveguide. The photon indistinguishability of 92.4% was retained after propagation in the SPP waveguide.
In the past decades, quantum plasmonics has become an active area due to its potential applications in on-chip plasmonic devices for quantum information processing. However, the fundamental physical process, i.e., how a quantum state of light evolves in the photon-plasmon conversion process, has not been described by a detailed microscopic quantum model. Here, we report a complete characterization of the plasmon-assisted extraordinary optical transmission process through quantum process tomography. By inputting various coherent states to interact with the plasmonic structure and detecting the output states with a homodyne detector, we reconstruct the process tensor of the photon-plasmon conversion process. Both the amplitude and phase information of the process are extracted, which explain the evolution of the quantum-optical state after the coupling with plasmons. Our experimental demonstration constitutes a fundamental block for future on-chip applications of quantum plasmonic circuits.
Quantum superpositions and entanglement are at the heart of the quantum information science. There have been only a few investigations of these phenomena at the mesoscopic level, despite the fact that these systems are promising for quantum state storage and processing. Here, we present two novel experiments with surface plasmons propagating on cm-long metallic stripe waveguides. We demonstrate that two plasmons can be entangled at remote places. In addition, we create a single plasmon in a temporal superposition state: it exists in a superposition of two widely separated moments. These quantum states, created using photons at telecom wavelength, are collectively held by a mesoscopic number of electrons coding a single-quantum bit of information; they are shown to be very robust against decoherence.