Two-photon states emitted from spontaneous parametric downconversion (SPDC) can exhibit quantum correlations in various degrees of freedom. On the other hand, plasmonic nanostructures show enhanced transmission thanks to the conversion of light into surface plasmon polaritons. It has been shown previously that polarization, time-energy and orbital angular momentum entanglement are preserved in such structures. The fact that surface plasmons are collective charge density waves, consisting of billions of electrons makes this observation remarkable. Here we show that spatial entanglement is also preserved by characterizing it after the photons interacted with gold nanopillar arrays. The detection is realized with novel single photon avalanche diode (SPAD) arrays with high spatial and temporal resolution. By measuring the spatial correlations of the photon in the near- and far-fields, we can characterize the state with respect to spatial entanglement with and without the nano-structure.
Two-photon states emitted from spontaneous parametric downconversion (SPDC) can exhibit quantum correlations in various degrees of freedom. On the other hand, plasmonic nanostructures show enhanced transmission thanks to the conversion of light into surface plasmon polaritons. It has been shown previously that polarization, time-energy and orbital angular momentum entanglement are preserved in such structures. The fact that surface plasmons are collective charge density waves, consisting of billions of electrons makes this observation remarkable. Here we show that spatial entanglement is also preserved by characterizing it after the photons interacted with gold nanopillar arrays. The detection is realized with novel single photon avalanche diode (SPAD) arrays with high spatial and temporal resolution. By measuring the spatial correlations of the photon in the near- and far-fields, we can characterize the state with respect to spatial entanglement with and without the nano-structure.
Previous experiments have shown that surface plasmon polaritons (SPPs) preserve their entangled state and do not cause measurable decoherence. However, essentially all of them were done using SPPs whose dispersion was in the linear “photon-like” regime. We report in this presentation on experiments showing how transition to “true-plasmon” non-linear dispersion regime, which occurs near SPP resonance frequency, will affect quantum coherent properties of light. To generate a polarization-entangled state we utilize type-I parametric down-conversion, occurring in a pair of non-linear crystals (BiBO), glued together and rotated by 90 degrees with respect to each other. For state projection measurements, we use a pair of polarizers and single-photon avalanche diode coincidence count detectors. We interpose a plasmonic hole array in the path of down-converted light before the polarizer. Without the hole array, we measure visibility V=99-100% and Bell’s number S=2.81±0.03. To study geometrical effects we fabricated plasmonic hole arrays (gold on optically polished glass) with elliptical holes (axes are 190nm and 240nm) using focused ion beam. When we put this sample in our system we measured the reduction of visibility V=86±5% using entangled light. However, measurement using classical light gave exactly the same visibility; hence, this reduction is caused only by the difference in transmission coefficients of different polarizations. As samples with non-linear dispersion we fabricated two-layer (a-Si - Au) and three-layer (a-Si – Au – a-Si) structures on optically polished glass with different pitches and circular holes. The results of measurements with these samples will be discussed along with the theoretical investigations.
Previous experiments have shown that surface plasmon polaritons (SPPs) preserve their entangled state and do not cause measurable decoherence. However, essentially all of them were done using SPPs whose dispersion was in the linear “photon-like” regime. We report in this presentation on experiments showing how transition to “true-plasmon” non-linear dispersion regime, which occurs near SPP resonance frequency, will affect quantum coherent properties of light. To generate a polarization-entangled state we utilize type-I parametric down-conversion, occurring in a pair of non-linear crystals (BiBO), glued together and rotated by 90 degrees with respect to each other. For state projection measurements, we use a pair of polarizers and single-photon avalanche diode coincidence count detectors. We interpose a plasmonic hole array in the path of down-converted light before the polarizer. Without the hole array, we measure visibility V=99-100% and Bell’s number S=2.81±0.03. To study geometrical effects we fabricated plasmonic hole arrays (gold on optically polished glass) with elliptical holes (axes are 190nm and 240nm) using focused ion beam. When we put this sample in our system we measured the reduction of visibility V=86±5% using entangled light. However, measurement using classical light gave exactly the same visibility; hence, this reduction is caused only by the difference in transmission coefficients of different polarizations. As samples with non-linear dispersion we fabricated two-layer (a-Si - Au) and three-layer (a-Si – Au – a-Si) structures on optically polished glass with different pitches and circular holes. The results of measurements with these samples will be discussed along with the theoretical investigations.
We present an experimental evidence that high-dimensional orbital angular-momentum entanglement of a pair of photons can be survived after a photon-plasmon-photon conversion. The information of spatial modes can be coherently transmitted by surface plasmons. This experiment primarily studies the high-dimensional entangled systems based on surface plasmon with subwavelength structures. It maybe useful in the investigation of spatial-mode properties of surface plasmon-assisted transmission through subwavelength hole arrays.
Surface plasmon polaritons (SPPs) are collective excitations of free electrons propagating along a metal-dielectric interface. Although some basic quantum properties of SPPs, such as the preservation of entanglement, the wave-particle duality of a single plasmon, the quantum interference of two plasmons, and the verification of entanglement generation, have been shown, more advanced quantum information protocols have yet to be demonstrated with SPPs. Here, we experimentally realize quantum state teleportation between single photons and SPPs. To achieve this, we use polarization-entangled photon pairs, coherent photon-plasmon-photon conversion on a metallic subwavelength hole array, complete Bell-state measurements and an active feed-forward technique. The results of both quantum state and quantum process tomography confirm the quantum nature of the SPP mediated teleportation. An average state fidelity of [Formula: see text] and a process fidelity of [Formula: see text], which are well above the classical limit, are achieved. Our work shows that SPPs may be useful for realizing complex quantum protocols in a photonic-plasmonic hybrid quantum network.
We report on experimental evidence of the preservation of the energy-time entanglement of a pair of photons after a photon-plasmon-photon conversion. This preservation is observed in two different plasmon conversion experiments, namely, extraordinary optical transmission through subwavelength metallic hole arrays and long range surface plasmon propagation in metallic waveguides. Plasmons are shown to coherently exist at two different times separated by much more than their lifetimes. This kind of entanglement involving light and matter is expected to be useful for future processing and storing of quantum information.
Surface plasmon polaritons (SPPs) result from collective oscillations of free electrons coupled to an electromagnetic field at a plane interface between a metal and a dielectric medium. As photons, SPPs can be considered either as waves or as bosonic particles [1] and they can experience striking quantum interferences such as Hong-Ou-Mandel (HOM) effect [2]. We use in this paper a plasmonic platform (Fig.1) that can convert photons into plasmons, and separate or recombine them on a plasmonic beamsplitter [3]. Single SPPs are excited using single photons created by parametric down conversion into a periodically-poled KTP crystal. The platform is placed in a Mach-Zehnder interferometer in order to vary the path difference between SPPs before impinging on the beamsplitter. The setup allows us to revisit quantum optics experiments using SPP as carriers of the quantum of energy. Using the same device, we can test the wave-particle duality, two-particle (HOM) interference and non-local control of single plasmon interference using the entanglement between a photon and a SPP [4]. In the case of the HOM experiment, we demonstrate that the losses can be used as a new degree of freedom [5]. Playing with the dephasing between transmission and reflection coefficient of the beamsplitter, we can observe a peak instead of the usually expected dip in the HOM interference (Fig.2), i.e. an anti-coalescence effect of SPP. In this talk, we will introduce the plasmonic device main features as well as the different quantum plasmonics experiments that have been performed thanks to the SPP beamsplitter. These results are essential to understand the SPP quantum behavior or to develop hybrid plasmon-photon systems for potential future applications in quantum communication mediated by SPP. [1] JM Elson and R.H. Ritchie, Phys. Rev. B 4, 4129 (1971) [2] J.S. Fakonas et al., Nat. Phot. 8, 317 (2014) [3] M.C. Dheur et al. , Sc. Advances 2, e151574 (2016) [4] M.C. Dheur et al. ArXiv 1610.07493, B. Vest et al. ArXiv 1610.07479 [5] S. Barnett et al., Phys. Rev. A 57, 2134 (1998) Fig.1: Plasmonic platform used for the quantum optics experiment (B). It consists in two SPP launchers (A), a plasmonic beamsplitter, and two slits to convert SPP to photons in the glass substrate. The plasmonic interference can thus be probed using single photon counting modules. Fig2: HOM experiment on a lossy plasmonic beamsplitter, whose complex amplitude reflection and transmission factors are denoted r and t respectively. The usual HOM dip is observed when r = it (left), a peak in the coincidence rate is shown when r = t.