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arXiv:quant-ph/0309074 · Journal of Physics B Atomic Molecular and Optical Physics

Adiabatic creation of coherent superposition states via multiple intermediate states

A. Karpati, Z. Kis

Published Feb 19, 2003• 24 citations
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Abstract

We consider an adiabatic population transfer process that resembles the well-established stimulated Raman adiabatic passage. In our system, the states have nonzero angular momentums J , therefore, the coupling laser fields induce transitions between the magnetic sublevels of the states. In particular, we discuss the possibility of creating coherent superposition states in a system with coupling pattern J = 0 ⇔ 1 and 1 ⇔ 2. Initially, the system is in the J = 0 state. We show that by, applying two delayed overlapping laser pulses, it is possible to create any final superposition state of the magnetic sublevels |2, −2⟩, |2, 0⟩, |2, +2⟩. Moreover, we find that the relative phases of the applied pulses influence not only the phases of the final superposition state but also the probability amplitudes. We show that if we fix the shape and the time delay between the pulses, the final state space can be entirely covered by varying the polarizations and relative phases of the two pulses. Performing numerical simulations we find that our transfer process is nearly adiabatic for the whole parameter set.

DOI
10.1088/0953-4075/36/5/310

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We consider an adiabatic population transfer process that resembles the well-established stimulated Raman adiabatic passage. In our system, the states have nonzero angular momentums J , therefore, the coupling laser fields induce transitions between the magnetic sublevels of the states. In particular, we discuss the possibility of creating coherent superposition states in a system with coupling pattern J = 0 ⇔ 1 and 1 ⇔ 2. Initially, the system is in the J = 0 state. We show that by, applying two delayed overlapping laser pulses, it is possible to create any final superposition state of the magnetic sublevels |2, −2⟩, |2, 0⟩, |2, +2⟩. Moreover, we find that the relative phases of the applied pulses influence not only the phases of the final superposition state but also the probability amplitudes. We show that if we fix the shape and the time delay between the pulses, the final state space can be entirely covered by varying the polarizations and relative phases of the two pulses. Performing numerical simulations we find that our transfer process is nearly adiabatic for the whole parameter set.
A technique for creation of well-defined preselected coherent superpositions of multiple quantum states is proposed. It is based on an extension of the technique of stimulated Raman adiabatic passage (STIRAP) to degenerate levels. As an example, the nine-state system composed of the magnetic sublevels of three levels with angular momenta Jg=0{J}_{g}=0Jg​=0, Je=1{J}_{e}=1Je​=1, and Jf=2{J}_{f}=2Jf​=2 is studied in detail. Starting from the $\ensuremath{\mid}{J}_{g}=0,{M}_{g}=0⟩$ state, STIRAP can create an arbitrary preselected coherent superposition between the five Mf{M}_{f}Mf​ sublevels $({M}_{f}=\ensuremath{-}2,\ensuremath{-}1,0,+1,+2)$ of the Jf=2{J}_{f}=2Jf​=2 level with 100% efficiency in the adiabatic limit. The populations and the phases of the Mf{M}_{f}Mf​ states in this superposition are determined entirely by the polarizations of the two laser fields. It is shown that this technique allows one to create any superposition of the five Mf{M}_{f}Mf​ states, that is, to reach any point in the Hilbert space of the Jf=2{J}_{f}=2Jf​=2 manifold, and the corresponding recipes for choosing the laser polarizations are presented.
The technique of stimulated Raman adiabatic passage (STIRAP) has become an established procedure for producing complete population inversion in atoms or molecules via application of Stokes and pump pulses in a counterintuitive sequence. Previously we reported on numerical and analytical investigations showing some of the additional and important phenomena that arise when some of the levels involved have nonzero angular momentum, the field polarization directions have no simplifying symmetries, and Zeeman splitting lifts the magnetic sublevel degeneracy. Here we verify our theoretical findings using the metastable neon system: 3^{3}3P0{\mathit{P}}_{0}P0​?3{\mathrm{?}}^{3}?3P1{\mathit{P}}_{1}P1​?3{\mathrm{?}}^{3}?3P2{\mathit{P}}_{2}P2​ with the corresponding angular momentum sequence J=0?J=1?J=2. In particular, we demonstrate that it is possible to transfer all population from the single initial state to any single selectable final magnetic sublevel M. Selectivity can be achieved either by choosing special laser polarization angles or, for fixed polarizations, by tuning the two lasers into two-photon resonance between the initial and desired final state. The complete control of magnetic sublevel population enabled by this procedure extends the customary experimental methods for producing oriented or aligned beams of atoms. In addition, we demonstrate very clearly the previous prediction that population transfer may fail for certain sets of parameters (detunings, Rabi frequencies, and polarization angles). \textcopyright{} 1996 The American Physical Society.
The technique of stimulated Raman adiabatic passage has become an established procedure for producing complete population inversion in atoms or molecules via application of Stokes and pump pulses in a counterintuitive sequence. We discuss here some of the new and important phenomena that arise when some of the states involved have nonzero angular momentum, the field polarization directions have no simplifying symmetries, and Zeeman splitting lifts the magnetic sublevel degeneracy. We consider the effects of the linkage structure of the Hamiltonian, the effects of various polarization directions, and the effects of various choices for carrier frequencies, as expressed by detunings from single-photon resonance. In particular, we consider an example with angular momentum J=0\ensuremath{\leftrightarrows}J=1\ensuremath{\leftrightarrows}J=2 in which nine magnetic sublevels occur. We show that under suitable conditions it is possible, simply through the appropriate tuning of pump and Stokes carrier frequencies, to place the entire population into any specified single magnetic sublevel.
We present the theory for a technique, based on multistate variants of the stimulated Raman adiabatic passage (STIRAP) process, that allows efficient and robust preparation of a preselected superposition of two or three degenerate states (magnetic sublevels of an atom) and the measurement of their relative amplitudes and phases. Because the preparation utilizes adiabatic passage it is robust against small fluctuations of the Rabi frequencies and temporal shapes of the coupling fields. We here describe and, in the following companion paper we demonstrate, an approach to the experimental characterization of the superposition state, i.e., the measurement of the relative phases and the ratios of amplitudes of the components. That technique, termed phase-to-population mapping, is applicable to the characterization of a stream of identically prepared atoms and is based on laser-induced fluorescence after the atoms have undergone optical pumping cycles induced by an additional laser. The optical pumping process maps the phase into populations of a subset of levels by means of a filtering laser field, and is robust against variations in the intensity and detuning of that field. We describe four linkage patterns appropriate to the creation of superpositions of two or three degenerate states of angular momentum J=2J=2J=2, starting from J=0J=0J=0. We offer an interpretation, from three different perspectives, of the subsequent characterization procedure.
We discuss the properties of a simple and robust scheme for preparing atoms and molecules in an arbitrary preselected coherent superposition of quantum states - fractional stimulated Raman adiabatic passage (fractional STIRAP) - first proposed by Marte et al (1991 Phys. Rev. A 44 R4118). As in STIRAP, the Stokes pulse arrives before the pump pulse, but unlike STIRAP, here the two pulses terminate simultaneously, while maintaining a constant ratio of amplitudes. We extend earlier research and suggest a realization of this scheme with two smoothly varying delayed laser pulses (which can be derived from a single laser), the parameters of the created superposition being controlled by the polarization of the delayed pulse. Furthermore, we provide simple analytic estimates of the robustness of this process against variations in the laser intensity, laser frequency and pulse delay. Finally, we discuss an extension to multistate systems which provides a possibility for creating coherent superpositions of more than two states.
The manipulation of population transfer and the creation of an arbitrary superposition between two atomic states in the framework of a closed inverse Y-type four-level system driven by a series of pulse pairs and an external control field is reported. It is shown that when the laser fields are tuned to resonance with respective transitions, the non-adiabatic coupling between two degenerate adiabatic states can be reduced tremendously and complete population transfer from the initial state to the target state can be achieved in a piecewise manner. Moreover, an arbitrary superposition between the initial state and target state can be created by suitably tuning the Rabi frequency of the control laser field, inter-pair time delay, pulse number or intra-pair time delay between the pump and Stokes pulses. This scheme combines stimulated Raman adiabatic passage and temporal coherent control, and may be useful for quantum information processing and control of chemical reactions.