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arXiv:quant-ph/0107007

Comparative study of the transient evolution of Hanle EIT/EIA resonances

Paulo Valente, H. Failache, A. Lezama

Published Jul 2, 2001• 2 citations
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Abstract

The temporal evolutions of coherent resonances corresponding to electromagnetically induced transparency (EIT) and absorption (EIA) were observed in a Hanle absorption experiment carried on the $D_{2}$ lines of $% ^{87}$Rb vapor by suddenly turning the magnetic field on or off. The main features of the experimental observations are well reproduced by a theoretical model based on Bloch equation where the atomic level degeneracy has been fully accounted for. Similar (opposite phase) evolutions were observed at low optical field intensities for Hanle/EIT or Hanle/EIA resonances. Unlike the Hanle/EIA\ transients which are increasingly shorter for driving field intensities approaching saturation, the $B\neq 0$ transient of the Hanle/EIT signal at large driving field intensities present a long decay time approaching the atomic transit time. Such counterintuitive behavior is interpreted as a consequence of the Zeno effect.

DOI
10.48550/arxiv.quant-ph/0107007

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The temporal evolutions of coherent resonances corresponding to electromagnetically induced transparency (EIT) and absorption (EIA) were observed in a Hanle absorption experiment carried on the D2D_{2}D2​ lines of % ^{87}Rb vapor by suddenly turning the magnetic field on or off. The main features of the experimental observations are well reproduced by a theoretical model based on Bloch equation where the atomic level degeneracy has been fully accounted for. Similar (opposite phase) evolutions were observed at low optical field intensities for Hanle/EIT or Hanle/EIA resonances. Unlike the Hanle/EIA\ transients which are increasingly shorter for driving field intensities approaching saturation, the B≠0B\neq 0B=0 transient of the Hanle/EIT signal at large driving field intensities present a long decay time approaching the atomic transit time. Such counterintuitive behavior is interpreted as a consequence of the Zeno effect.
The temporal evolutions of electromagnetically induced transparency (EIT) and absorption (EIA) were observed in a Hanle absorption experiment carried on the D2{D}_{2}D2​ lines of 87Rb{}^{87}\mathrm{Rb}87Rb vapor by suddenly turning the magnetic field on or off. The main features of the experimental observations are well reproduced by a theoretical model based on Bloch equation where the atomic level degeneracy has been fully accounted for. Similar (opposite phase) evolutions were observed at low optical-field intensities for Hanle-EIT or Hanle-EIA resonances. Unlike the Hanle-EIA transients that are increasingly shorter for driving field intensities approaching saturation, the $B\ensuremath{\ne}0$ transient of the Hanle-EIT signal at large driving field intensities present a long decay time approaching the atomic transit time. Such counterintuitive behavior is interpreted as a consequence of the Zeno effect.
The temporal evolution of electromagnetically induced transparency (EIT) and absorption (EIA) coherence resonances in pump-probe spectroscopy of degenerate two-level atomic transition is studied for light intensities below saturation. Analytical expressions for the transient absorption spectra are given for simple model systems and a model for the calculation of the time-dependent response of realistic atomic transitions, where the Zeeman degeneracy is fully accounted for, is presented. EIT and EIA resonances have a similar (opposite sign) time-dependent line shape, however, the EIA evolution is slower and thus narrower lines are observed for long interaction time. Qualitative agreement with the theoretical predictions is obtained for the transient probe absorption on the 85Rb{}^{85}\mathrm{Rb}85Rb D2{D}_{2}D2​ line in an atomic beam experiment.
A perturbation method was used to solve optical Bloch equations (OBEs) for the transition F g =1→ F e =2, in order to describe the role of ground-level Zeeman coherences in the formation of electromagnetically induced absorption (EIA). A narrow Lorentzian peak, centered at zero value of the scanning magnetic field, appears in the analytical expression of the second-order correction of a density-matrix element for ground-level Zeeman coherences, (ρ g −1 , g +1 ) x 2 . Through analytical expressions for lower-order corrections of density-matrix elements, we were able to establish clear relations between the narrow Lorentzian in (ρ g − 1 , g +1 ) x 2 and higher-order corrections of optical coherences, i.e. EIA. We see from analytical expressions that these two resonances have opposite signs and that EIA becomes electromagnetically induced transparency (EIT) in the limit of low efficiency of spontaneous transfer of coherences from excited-level to ground-level Zeeman sublevels. The transient behavior of EIA follows the time evolution of (ρ g − 1 , g +1 ) x 2 . After the coupling laser is turned on, both the Lorentzian peak in (ρ g − 1 , g +1 ) x 2 and EIA reach steady state via over-damped oscillations.
The effect of incident light field ellipticity on the electromagnetically induced absorption (EIA) and electromagnetically induced transparency (EIT) resonances has been studied experimentally and computationally in Hanle configuration with longitudinal and transverse magnetic fields. We identify the Zeeman coherences that influence the resonance profile and study the role of coherence-transfer from excited to ground state via spontaneous emission as a function of ellipticity for the ${F}_{g}=2\ensuremath{\rightarrow}{F}_{e}=3$ transition of 87Rb^{87}\mathrm{Rb}87Rb. The EIT resonance observed with the light field locked on the ${F}_{g}=1\ensuremath{\rightarrow}{F}_{e}=2$ transition of 87Rb^{87}\mathrm{Rb}87Rb is an influence of the nearby ${F}_{g}=1\ensuremath{\rightarrow}{F}_{e}=0$ closed and ${F}_{g}=1\ensuremath{\rightarrow}{F}_{e}=1$ open transitions. With increase in ellipticity the observed EIA and EIT resonances diminish in amplitude for a longitudinal magnetic field and are enhanced for a transverse magnetic field. We computationally account for these observations and discuss the factors that influence the EIA and EIT resonance amplitudes as a function of ellipticity and show that for a transverse field scan the ellipticity dependence of the EIA resonance amplitude can be accounted for without invoking the Doppler effect unlike for a longitudinal field scan. We also show that the maximum in the EIA resonance amplitude obtained for nonzero ellipticities with a longitudinal magnetic field depends on the closedness of the atomic system.
Using a 1 --> 2 transition as an analytically tractable model, we discuss in detail magneto-optical resonances of both electromagnetically induced absorption (EIA) and electromagnetically induced transparency (EIT) types in the Hanle configuration. The analysis is made for an arbitrary rate of depolarizing collisions in the excited state and an arbitrary elliptical field polarization. The obtained results clearly show that the main reason for the EIA subnatural resonance is the spontaneous transfer of anisotropy from the excited level to the ground level. In the EIA case we predict the negative structures in the absorption resonance at large field detuning. The role of the finite atom-light interaction time is briefly discussed. In addition we study nontrivial peculiarities of the resonance line shape related to the velocity spread in a gas.
The method for observing the high-contrast and narrow-width resonances of electromagnetically induced absorption (EIA) in the Hanle configuration under counterpropagating light waves is proposed. We theoretically analyze the absorption of a probe light wave in presence of counterpropagating one with the same frequency as the function of a static magnetic field applied along the vectors of light waves, propagating in a vapour cell. Here, as an example, we study a "dark" type of atomic dipole transition Fg=1-->Fe=1 in D1 line of 87Rb, where usually the electromagnetically induced transparency (EIT) can be observed. To obtain the EIA signal one should proper chose the polarizations of light waves and intensities. In contrast of regular schemes for observing EIA signals (in a single travelling light wave in the Hanle configuration or in a bichromatic light field consisted of two travelling waves), the proposed scheme allows one to use buffer gas to significantly enhance properties of the resonance. Also the dramatic influence of atomic transition openness on contrast of the resonance is revealed, that gives great advantage in comparison with cyclic atomic transitions. The obtained results can be interesting in high-resolution spectroscopy, nonlinear and magneto-optics.