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arXiv:quant-ph/0102036 · Physical Review Letters

Irreversibility in Asymptotic Manipulations of Entanglement

Guifré Vidal, J. I. Cirac

Published Jun 18, 2001• 110 citations
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Abstract

We show that the process of entanglement distillation is irreversible by showing that the entanglement cost of a bound entangled state is finite. Such irreversibility remains even if extra pure entanglement is loaned to assist the distillation process.
DOI
10.1103/physrevlett.86.5803

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The manipulation of quantum entanglement is fundamentally irreversible: some mixed entangled states require pure entanglement for their preparation, although no pure entanglement can be recovered from them by local operations and classical communication. This irreversibility is known to persist even under the maximal class of operations that do not generate entanglement, revealing a fundamental distinction between entanglement theory and thermodynamics. We construct cases for which any attempt to restore reversibility necessarily incurs an error that increases exponentially with the number of copies. Technically, we demonstrate a strict separation between the exponential strong-converse distillable entanglement and the exponential strong-converse entanglement cost. Our result resolves a conjecture posed by Lami and Regula (Nat. Phys. 19, 184-189 (2023)) and strengthens it by showing that the irreversibility of entanglement persists even at the level of polynomially (in the number of copies) growing error. We further derive a semidefinite-programming lower bound on the exponential strong-converse cost under non-entangling operations. Finally, for the class of completely PPT-preserving operations, we construct analytically solvable families of antisymmetric states exhibiting the exponential strong-converse irreversibility. Remarkably, to our knowledge, no analogous separation between exponential strong converse cost and the analogous distillable entanglement is currently known even under the more restrictive class of LOCC operations.
We investigate the irreversibility of entanglement distillation for a symmetric (d+1)(d+1)(d+1)-parameter family of mixed bipartite quantum states acting on Hilbert spaces of arbitrary dimension $d\ifmmode\times\else\texttimes\fi{}d$. We prove that in this family the entanglement cost is generically strictly larger than the distillable entanglement, so that the set of states for which the distillation process is asymptotically reversible is of measure zero. This remains true even if the distillation process is catalytically assisted by pure-state entanglement and every operation is allowed, which preserves the positivity of the partial transpose. It is shown that reversibility occurs only in cases where the state is a tagged mixture. The reversible cases are shown to be completely characterized by minimal uncertainty vectors for entropic uncertainty relations.
We demonstrate the irreversibility of asymptotic entanglement manipulation under quantum operations that completely preserve the positivity of partial transpose (PPT), resolving a major open problem in quantum information theory. Our key tool is a new efficiently computable additive lower bound for the asymptotic relative entropy of entanglement with respect to PPT states, which can be used to evaluate the entanglement cost under local operations and classical communication (LOCC). We find that for any rank-two mixed state supporting on the 3⊗3 antisymmetric subspace, the amount of distillable entanglement by PPT operations is strictly smaller than one entanglement bit (ebit) while its entanglement cost under PPT operations is exactly one ebit. As a by-product, we find that for this class of states, both the Rains's bound and its regularization are strictly less than the asymptotic relative entropy of entanglement. So, in general, there is no unique entanglement measure for the manipulation of entanglement by PPT operations. We further show a computable sufficient condition for the irreversibility of entanglement distillation by LOCC (or PPT) operations.