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arXiv:1606.09421 · Physical Review Letters

Irreversibility of Asymptotic Entanglement Manipulation Under Quantum Operations Completely Preserving Positivity of Partial Transpose

Xin Wang, Runyao Duan

Published Nov 3, 2017• 32 citations
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Abstract

We demonstrate the irreversibility of asymptotic entanglement manipulation under quantum operations that completely preserve the positivity of partial transpose (PPT), resolving a major open problem in quantum information theory. Our key tool is a new efficiently computable additive lower bound for the asymptotic relative entropy of entanglement with respect to PPT states, which can be used to evaluate the entanglement cost under local operations and classical communication (LOCC). We find that for any rank-two mixed state supporting on the 3⊗3 antisymmetric subspace, the amount of distillable entanglement by PPT operations is strictly smaller than one entanglement bit (ebit) while its entanglement cost under PPT operations is exactly one ebit. As a by-product, we find that for this class of states, both the Rains's bound and its regularization are strictly less than the asymptotic relative entropy of entanglement. So, in general, there is no unique entanglement measure for the manipulation of entanglement by PPT operations. We further show a computable sufficient condition for the irreversibility of entanglement distillation by LOCC (or PPT) operations.

DOI
10.1103/physrevlett.119.180506

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We demonstrate the irreversibility of asymptotic entanglement manipulation under quantum operations that completely preserve the positivity of partial transpose (PPT), resolving a major open problem in quantum information theory. Our key tool is a new efficiently computable additive lower bound for the asymptotic relative entropy of entanglement with respect to PPT states, which can be used to evaluate the entanglement cost under local operations and classical communication (LOCC). We find that for any rank-two mixed state supporting on the 3⊗3 antisymmetric subspace, the amount of distillable entanglement by PPT operations is strictly smaller than one entanglement bit (ebit) while its entanglement cost under PPT operations is exactly one ebit. As a by-product, we find that for this class of states, both the Rains's bound and its regularization are strictly less than the asymptotic relative entropy of entanglement. So, in general, there is no unique entanglement measure for the manipulation of entanglement by PPT operations. We further show a computable sufficient condition for the irreversibility of entanglement distillation by LOCC (or PPT) operations.
We study entanglement distillation under operations that remain completely positive under partial-transpose conjugation, a.k.a. PPT channels, in the standard quantum Shannon theory regime of asymptotically vanishing but non-zero error. Our main results are: (a) a regularised formula for the PPT distillable entanglement in terms of a measured-relative-entropy-like quantity; and (b) two different single-letter converses, one based on operator quadratic forms and the other on Hirschman's strengthening of the Hadamard three-line theorem. As an immediate application of (b), we show that the PPT distillable entanglement can be strictly smaller than the regularised Rains bound, thereby resolving an open problem in the theory of entanglement manipulation [Regula et al., NJP 21:103017, 2019]. A gap appears already for 3×33\times 33×3 Werner states: at antisymmetric weight 25/2625/2625/26, a certified upper bound of 0.621070.621070.62107 ebits lies below the (regularised) Rains bound, which equals 2526log⁡25−log⁡23≈0.64766\frac{25}{26} \log_2 5 - \log_2 3 \approx 0.647662625​log2​5−log2​3≈0.64766 ebits. On a different note, (a) implies a faithful lower bound on the PPT distillable entanglement in terms of the entanglement negativity, which provides a quantitative counterpart to the qualitatively known fact that any NPT state is PPT distillable [Eggeling et al., PRL 87:257902, 2001].
We first study the reversibility for a class of states under the operations which completely preserve the positivity of partial transpose (PPT) and show that the entanglement cost is equal to the distillable entanglement for a rank-two mixed state on the 4⊗4 antisymmetric subspace under PPT operations. By using a similar method in finding the irreversibility, we also find that the value of a new efficiently computable additive lower bound E η ( ρ ) for the asymptotic PPT-relative entropy of entanglement presented in [ Phys. Rev. Lett. 119 , 180506 (2017)] is equal to the regularized Rains’ bound and an upper bound E N ( ρ ) for distillable entanglement for these states. Furthermore, we find states on the symmetric subspace satisfying the relation mentioned above, generalize the antisymmetric states and symmetric states in higher dimensions, and give a specific value for distillable entanglement and entanglement cost for these states under the PPT operations.
Quantum catalysts can overcome otherwise impossible quantum state transformations without being consumed, and allowing them to become correlated with the output makes this assistance substantially more powerful. This raises a fundamental question for entanglement theory: which limitations on state manipulation remain when such correlated catalysts are freely available? We answer this question in the positive-partial-transpose (PPT) resource theory, which allows a substantially broader class of operations than local operations and classical communication (LOCC). We identify general conditions under which regularized relative-entropy measures become strongly superadditive, and use them to construct monotones that constrain correlated catalytic PPT transformations without any knowledge of the catalyst. In particular, we prove that the regularized PPT relative entropy is fully additive and strongly superadditive, resolving an open problem in entanglement theory. Most importantly, these constraints show that even arbitrary correlated catalysts cannot restore asymptotic reversibility: for an explicit state, the optimal entanglement distillation rate remains strictly smaller than the entanglement cost. Thus, substantial catalytic assistance does not remove some of the fundamental limitations of mixed-state entanglement manipulation.
The manipulation of quantum entanglement is fundamentally irreversible: some mixed entangled states require pure entanglement for their preparation, although no pure entanglement can be recovered from them by local operations and classical communication. This irreversibility is known to persist even under the maximal class of operations that do not generate entanglement, revealing a fundamental distinction between entanglement theory and thermodynamics. We construct cases for which any attempt to restore reversibility necessarily incurs an error that increases exponentially with the number of copies. Technically, we demonstrate a strict separation between the exponential strong-converse distillable entanglement and the exponential strong-converse entanglement cost. Our result resolves a conjecture posed by Lami and Regula (Nat. Phys. 19, 184-189 (2023)) and strengthens it by showing that the irreversibility of entanglement persists even at the level of polynomially (in the number of copies) growing error. We further derive a semidefinite-programming lower bound on the exponential strong-converse cost under non-entangling operations. Finally, for the class of completely PPT-preserving operations, we construct analytically solvable families of antisymmetric states exhibiting the exponential strong-converse irreversibility. Remarkably, to our knowledge, no analogous separation between exponential strong converse cost and the analogous distillable entanglement is currently known even under the more restrictive class of LOCC operations.
Quantifying the minimum entanglement needed to prepare quantum states and implement quantum processes is a key challenge in quantum information theory. In this Letter, we develop computable and faithful lower bounds on the entanglement cost under quantum operations that completely preserve the positivity of partial transpose (PPT operations), by introducing the generalized divergence of k-negativity, a generalization of logarithmic negativity. Our bounds are efficiently computable via semidefinite programming and provide nontrivial values for all states that are non-PPT (NPT), establishing their faithfulness for the resource theory of NPT entanglement. Notably, we find and affirm the irreversibility of asymptotic entanglement manipulation under PPT operations for full-rank entangled states. Furthermore, we extend our methodology to derive lower bounds on the entanglement cost of both point-to-point and bipartite quantum channels. Our bound demonstrates improvements over previously known computable bounds for a wide range of quantum states and channels. These findings push the boundaries of understanding the structure of entanglement and the fundamental limits of entanglement manipulation.
Exact entanglement distillation converts a noisy bipartite state into a maximally entangled state with zero error. Under completely PPT-preserving operations, the additive min-Rains relative entropy provides a single-letter upper bound on the regularized distillation rate. An interesting problem in entanglement theory dating back to 2016 has been whether this bound is always tight. Here we resolve this question in the negative. The key is a tensor-stable rigidity absent from the min-Rains relaxation: every feasible exact-distillation effect must act as the identity on the support of the input state. We convert this constraint into a new single-letter upper bound using a generally non-Hermitian, range-supported witness. For a rank-three subspace, we show this upper bound lies strictly below the min-Rains relative entropy for every state with that support. Thus, the constraint discarded by the min-Rains relaxation remains relevant under arbitrary tensor powers. Our result rules out the min-Rains relative entropy as a closed-form formula for exact PPT distillable entanglement and reveals the subtle asymptotic structure of exact entanglement manipulation under PPT operations.