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arXiv:cond-mat/9905415 · Journal of the Physical Society of Japan

Spin Transport Properties of the Quantum One-Dimensional Non-Linear Sigma Model: an Application to Haldane Gap Systems

Satoshi Fujimoto

Published Aug 15, 1999• 42 citations
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Abstract

Spin transport properties of the quantum one-dimensional non-linear sigma model are studied based upon the Bethe ansatz exact solution for the O(3) sigma model and the 1/N-expansion approach for the O(N) sigma model. It is shown that the spin transport at finite temperatures is ballistic and there is no spin diffusion in this system. A possible mechanism for the spin diffusion observed in the NMR experiment of the Haldane gap system AgVP_2S_6 by Takigawa et al. [Phys. Rev. Lett.{\bf 76}, 2173 (1996)] is also discussed. The inclusion of the spin-phonon interaction accounts for the experimental results qualitatively.

DOI
10.1143/jpsj.68.2810

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Spin transport properties of the quantum one-dimensional non-linear sigma model are studied based upon the Bethe ansatz exact solution for the O(3) sigma model and the 1/N-expansion approach for the O(N) sigma model. It is shown that the spin transport at finite temperatures is ballistic and there is no spin diffusion in this system. A possible mechanism for the spin diffusion observed in the NMR experiment of the Haldane gap system AgVP_2S_6 by Takigawa et al. [Phys. Rev. Lett.{\bf 76}, 2173 (1996)] is also discussed. The inclusion of the spin-phonon interaction accounts for the experimental results qualitatively.
In a recent preprint (cond-mat/9905415), Fujimoto has used the Bethe ansatz to compute the finite temperature, zero frequency Drude weight of spin transport in the quantum O(3) non-linear sigma model in a magnetic field H≠0H \neq 0H=0. We show here that, contrary to his claims, the results are in accord with earlier semiclassical results (Sachdev and Damle, cond-mat/9610115). We also comment on his 1/N expansion, and show that it does not properly describe the long-time correlations.
We study both the static and dynamic properties of gapped, one-dimensional, Heisenberg, antiferromagnetic, spin chains at finite temperature through an analysis of the O(3) nonlinear sigma model. Exploiting the integrability of this theory, we are able to compute an exact low-temperature expansion of the finite temperature correlators. We do so using a truncated ``form-factor'' expansion and so provide evidence that this technique can be successfully extended to finite temperature. As a direct test, we compute the static zero-field susceptibility and obtain an exact match to the susceptibility derived from the low-temperature expansion of the exact free energy. We also study transport properties, computing both the spin conductance and the NMR-relaxation rate, 1/T1.{1/T}_{1}.1/T1​. We find these quantities to show ballistic behavior. In particular, the computed spin conductance exhibits a nonzero Drude weight at finite temperature and zero applied field. The physics thus described differs from the spin diffusion reported by Takigawa et al. [Phys. Rev. Lett. 76, 2173 (1996)] from experiments on the Haldane gap material, AgVP2S6.{\mathrm{AgVP}}_{2}{S}_{6}.AgVP2​S6​.
An effective, low temperature, classical model for spin transport in the one-dimensional, gapped, quantum O(3)\mathrm{O}(3)O(3) nonlinear $\ensuremath{\sigma}$ model is developed. Its correlators are obtained by a mapping to a model solved earlier by Jepsen. We obtain universal functions for the ballistic-to-diffusive crossover and the value of the spin diffusion constant, and these are claimed to be exact at low temperatures. Implications for experiments on one-dimensional insulators with a spin gap are noted.
We discuss the theory of the nonzero temperature (T)(T)(T) spin dynamics and transport in one-dimensional Heisenberg antiferromagnets with a gap $\ensuremath{\Delta}$. For $T\ensuremath{\ll}\ensuremath{\Delta}$, we develop a semiclassical picture of thermally excited particles. Multiple inelastic collisions between the particles are crucial, and are described by a two-particle S\mathcal{S}S matrix which is shown to have a superuniversal form at low momenta. This is established by computations on the O(3)O(3)O(3) $\ensuremath{\sigma}$ model, and strong- and weak-coupling expansions (the latter using a Majorana fermion representation) for the two-leg S=1/2S=1/2S=1/2 Heisenberg antiferromagnetic ladder. As an aside, we note that the strong-coupling calculation reveals an S=1S=1S=1, two-particle bound state which leads to the presence of a second peak in the T=0T=0T=0 inelastic neutron-scattering (INS) cross section for a range of values of momentum transfer. We obtain exact, or numerically exact, universal expressions for the thermal broadening of the quasiparticle peak in the INS cross section, the spin diffusivity, and for the field dependence of the NMR relaxation rate 1/T1{1/T}_{1}1/T1​ of the effective semiclassical model; these are expected to be asymptotically exact for the quantum antiferromagnets in the limit $T\ensuremath{\ll}\ensuremath{\Delta}$. The results for 1/T1{1/T}_{1}1/T1​ are compared with the experimental findings of Takigawa et al. [Phys. Rev. Lett. 76, 2173 (1996)] and the agreement is quite good. In the regime $\ensuremath{\Delta}<T<$(a typical microscopic exchange) and we argue that a complementary description in terms of semiclassical waves applies, and give some exact results for the thermodynamics and dynamics.
The transport properties of quantum systems are one of the most interesting current topics in statistical physics. Heat transport can directly be observed through thermal conductivity measurements, while spin transport can be extracted from nuclear spin–lattice relaxation-time measurements. Numerous experiments have indeed been performed in an attempt to settle the argument about whether finite-temperature energy transport should be diffusive or ballistic. From the theoretical point of view, there is an argument that integrable Hamiltonians exhibit ballistic transport, whereas nonintegrable ones are diffusive or insulators. Since nonintegrable systems have much less been studied in this context so far, we investigate spin-½ ferromagnetic-antiferromagnetic bond-alternating chains, which exhibit common features of Haldane-gap antiferromagnets. Employing the Jordan–Wigner spinless-fermion representation, their level statistics is investigated by the exact-diagonalization method. We argue a possibility of the diffusive transport occurring in the system.
We use a quantum O(N) nonlinear \ensuremath{\sigma} model to describe one-dimensional quantum Heisenberg antiferromagnets with integer spin S. A large-N analytical treatment of this effective theory leads to definite predictions for thermodynamic quantities in the low-temperature regime. We obtain the Haldane gap as a function of the temperature and note a trend similar to that found in the compound NENP. The specific heat and magnetic susceptibility are also obtained and comparison with exact numerical results for the S=1 spin chain allows us to determine the domain of validity of our approximation. By a calculation at subleading 1/N order we compute the quasiparticle lifetime. Results are given on-shell, for the width observed at the quasiparticle pole as seen in neutron-scattering experiments, and also off-shell, for the NMR relaxation rate ${\mathit{T}}_{1}^{\mathrm{\ensuremath{-}}1}$. The phenomenological interacting boson model is compared with our approach. We discuss the effects of anisotropy and compare our results with present experiments on NENP.