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arXiv:cond-mat/0605148 · Journal of Physics Condensed Matter

Bose–Einstein condensation and entanglement in magnetic systems

M. A. Contínentino

Published Aug 18, 2006• 6 citations
arXivHTMLPDF

Abstract

We present a study of magnetic field induced quantum phase transitions in insulating systems. A generalized scaling theory is used to obtain the temperature dependence of several physical quantities along the quantum critical trajectory ($H=H_{C}$, $T\to0$) where $H$ is a longitudinal external magnetic field and $H_{C}$ the critical value at which the transition occurs. We consider transitions from a spin liquid at a critical field $H_{C1}$ and from a fully polarized paramagnet, at $H_{C2}$, into phases with long range order in the transverse components. The transitions at $H_{C1}$ and $H_{C2}$ can be viewed as Bose-Einstein condensations of magnons which however belong to different universality classes since they have different values of the dynamic critical exponent $z$. Finally, we use that the magnetic susceptibility is an entanglement witness to discuss how this type of correlation sets in as the system approaches the quantum critical point along the critical trajectory, $H=H_{C2}$, $T\to0$.

DOI
10.1088/0953-8984/18/35/023

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We present a study of magnetic field induced quantum phase transitions in insulating systems. A generalized scaling theory is used to obtain the temperature dependence of several physical quantities along the quantum critical trajectory (H=HCH=H_{C}H=HC​, T→0T\to0T→0) where HHH is a longitudinal external magnetic field and HCH_{C}HC​ the critical value at which the transition occurs. We consider transitions from a spin liquid at a critical field HC1H_{C1}HC1​ and from a fully polarized paramagnet, at HC2H_{C2}HC2​, into phases with long range order in the transverse components. The transitions at HC1H_{C1}HC1​ and HC2H_{C2}HC2​ can be viewed as Bose-Einstein condensations of magnons which however belong to different universality classes since they have different values of the dynamic critical exponent zzz. Finally, we use that the magnetic susceptibility is an entanglement witness to discuss how this type of correlation sets in as the system approaches the quantum critical point along the critical trajectory, H=HC2H=H_{C2}H=HC2​, T→0T\to0T→0.
We study field-induced magnetic order in cubic lattices of dimers with antiferromagnetic Heisenberg interactions. The thermal critical exponents at the quantum phase transition from a spin liquid to a magnetically ordered phase are determined from stochastic series expansion quantum Monte Carlo simulations. These exponents are independent of the interdimer coupling ratios, and converge to the value obtained by considering the transition as a Bose-Einstein condensation of magnons, ${\ensuremath{\alpha}}_{\mathrm{BEC}}=\frac{3}{2}.$ The scaling results are of direct relevance to the spin-dimer systems TlCuCl3{\mathrm{TlCuCl}}_{3}TlCuCl3​ and KCuCl3,{\mathrm{KCuCl}}_{3},KCuCl3​, and explain the broad range of exponents reported for field-induced ordering transitions.
We study magnetic-field-induced three-dimensional ordering transitions in low-dimensional quantum spin liquids, such as weakly coupled, antiferromagnetic spin- 1/2 Heisenberg dimers and ladders. Using stochastic series expansion quantum Monte Carlo simulations, we obtain the critical scaling exponents which dictate the power-law dependence of the transition temperature on the magnetic field. These are compared with recent experiments on candidate materials and with predictions for the Bose-Einstein condensation of magnons. The critical exponents deviate from isotropic mean-field theory and exhibit different scaling behavior at the lower and upper critical magnetic fields.
Over the past decade, significant progress has been achieved to create Bose-Einstein condensates (BECs) of magnetic excitations, i.e., magnons, at room temperature, which is a novel quantum many-body system with a strong spin-spin correlation, and contains potential applications in magnonic spintronics. For quantum information science, the magnonic condensates can become an attractive source of quantum entanglement, which plays a central role in most of the quantum information processing tasks. Here we theoretically study the entanglement properties of a magnon gas above and below the condensation temperature. We show that the thermodynamic entanglement of the spins is a manifestation of the off-diagonal long-range order; the entanglement of the condensate does not vanish, even if the spins are separated by an infinitely long distance, which is fundamentally distinct from the normal magnetic ordering below the Curie temperature. In addition, the phase-transition point occurs when the derivative of the entanglement changes abruptly. These results provide a theoretical foundation for a future investigation of the magnon BEC in terms of quantum entanglement.
The recent experimental advances in the field of quantum spin materials have led to well-controlled systems which can be used in order to simulate complex quantum models in a clean fashion. Here we discuss how fascinating effects normally known from bosonic systems such as the Bose-Einstein condensation can be investigated with the help of such materials. We discuss as an example how a crossover between an effectively one-dimensional geometry described by a Luttinger liquid to a three-dimensional Bose-Einstein condensation can be induced. Additionally, we point out how more complex phases as the Bose-glass phase could be realized in these quantum magnets. Introduction Although it can seem paradoxical, the quantum magnetic states found in insulators offer an interesting route to study Bose-Einstein condensation (BEC) and more generally phenomena related to itinerant, interacting bosonic systems. In many materials, the repulsion between the electrons causes the ground state to be a Mott insulator with one electron localized per site. In such a case, the charge degrees of freedom are completely locked by large charge gaps (usually of the order of tens of electron volts). However, one can study the fascinating physics of the spin degrees of freedom. As was shown a long time ago, the localized spins are coupled by a so-called superexchange which may be ferro- or antiferromagnetic. The properties of the exchange coupling between the spins depend mainly on the underlying atomic structure of the material. The resulting physics is extremely rich and such materials can have a host of phases ranging from ordered magnetic phases to so-called spin-liquid phases in which spin–spin correlations decay extremely fast with distance. The field of research concerning these materials, dubbed quantum magnetism, is thus an extremely active field in its own right [1]. Additionally, one can exploit the formal mapping that exists between spin operators and bosonic ones, as will be described in the next section, to connect the magnetic materials to itinerant bosonic systems with interactions between the bosons. This opens the way to use such quantum spin systems as quantum simulators. A quantum simulator means that the experimental system can be employed in order to “solve” in a controlled way a problem/Hamiltonian known from a different less controlled physical realization, e.g., inspired by fundamental many-body physics, quantum information or computational applications.
Classical and quantum criticality In most cases the phases of quantum field theories, in particular those of interest in condensed matter physics, can be described in terms of the behavior of local observables, such as order parameters or currents that transform properly under the symmetries of the theory. Quantum and thermal phase transitions are characterized by the behavior of these observables as a function of temperature and of the coupling constants of the theory. The phase transitions themselves, quantum or thermal, are classified into universality classes, which are represented by the critical exponents which specify the scaling laws of the expectation values of the observables. Historically, the development of this approach to critical behavior goes back to the Landau theory of critical behavior. It acquired its most complete form with the development of the renormalization group (RG) in the late 1960s and early 1970s. It is the centerpiece of Wilson’s approach to quantum field theory, in which all local quantum field theories are defined by the scaling regime of a physical system near a continuous phase transition. From this point of view there is no fundamental difference between classical (or thermal) phase transitions, which are described by the theory of classical critical behavior, and quantum phase transitions. For example, the expectation value of a local order parameter M as the thermal phase transition is approached from below behaves as M ~ (Tc − T) β . Here T c is the critical temperature and β is a critical exponent that depends on the universality class of the thermal phase transition and on the dimensionality of space. While quantum mechanics can play a key role in the existence of the ordered phase, e.g. superfluidity and superconductivity are macroscopic manifestations of essentially quantum-mechanical phenomena, the thermal transition itself is governed entirely by classical statistical mechanics, and quantum mechanics plays a role in setting the value of non-universal quantities such as the critical temperature, etc. On the other hand, in the case of a quantum phase transition, the order parameter M has a similar scaling behavior as a function of the coupling constant, M~(gc−g)β˜, where g is the coupling constant, g c is the critical coupling constant, and β˜ is a critical exponent that depends on the universality class of the quantum phase transition. Here we assume that M has a non-vanishing expectation value only for g < g c .
Spinor Bose-Einstein condensates under external magnetic fields exhibit well-characterized spin domains of its ground state due to spin-dependent interactions. At low temperatures, collision-induced spin-mixing instabilities may promote the condensate to dwell into metastable states occurring near the phase boundaries. In this paper, we study theoretically the metastable spin-phase diagram of a spin-1 antiferromagnetic Bose-Einstein condensate at zero and finite temperatures. The approach makes use of Hartree-Fock theory and exploits the symmetry of the Hamiltonian and of the order parameters yielding a closed system of transcendental equations for the free energy, fully avoiding the use of self-consistency methods. Our results are consistent with recent experiments and allow us to explain qualitatively the different types of observed quench dynamics. In addition, we found that similar phenomena should occur in antiferromagnetic spinor condensates with a sudden change in the temperature. It is shown also that the increase in temperature induces a traceable shift of the ferromagnetic-polar transition boundary, behavior previously not noted by self-consistent mean-field calculations.