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arXiv:1711.04394 · Physical review. B./Physical review. B

Thermodynamic entanglement of magnonic condensates

H. Y. Yuan, Man‐Hong Yung

Published Feb 20, 2018• 16 citations
arXivHTMLPDF

Abstract

Over the past decade, significant progress has been achieved to create Bose-Einstein condensates (BECs) of magnetic excitations, i.e., magnons, at room temperature, which is a novel quantum many-body system with a strong spin-spin correlation, and contains potential applications in magnonic spintronics. For quantum information science, the magnonic condensates can become an attractive source of quantum entanglement, which plays a central role in most of the quantum information processing tasks. Here we theoretically study the entanglement properties of a magnon gas above and below the condensation temperature. We show that the thermodynamic entanglement of the spins is a manifestation of the off-diagonal long-range order; the entanglement of the condensate does not vanish, even if the spins are separated by an infinitely long distance, which is fundamentally distinct from the normal magnetic ordering below the Curie temperature. In addition, the phase-transition point occurs when the derivative of the entanglement changes abruptly. These results provide a theoretical foundation for a future investigation of the magnon BEC in terms of quantum entanglement.

DOI
10.1103/physrevb.97.060405

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•Mar 2, 2015•1 citation
Over the past decade, significant progress has been achieved to create Bose-Einstein condensates (BECs) of magnetic excitations, i.e., magnons, at room temperature, which is a novel quantum many-body system with a strong spin-spin correlation, and contains potential applications in magnonic spintronics. For quantum information science, the magnonic condensates can become an attractive source of quantum entanglement, which plays a central role in most of the quantum information processing tasks. Here we theoretically study the entanglement properties of a magnon gas above and below the condensation temperature. We show that the thermodynamic entanglement of the spins is a manifestation of the off-diagonal long-range order; the entanglement of the condensate does not vanish, even if the spins are separated by an infinitely long distance, which is fundamentally distinct from the normal magnetic ordering below the Curie temperature. In addition, the phase-transition point occurs when the derivative of the entanglement changes abruptly. These results provide a theoretical foundation for a future investigation of the magnon BEC in terms of quantum entanglement.
A quantised spin wave – magnon – in magnetic films can undergo Bose-Einstein condensation (BEC) into two energetically degenerate lowest-energy quantum states with nonzero wave vectors ±k BEC . This corresponds to two interfering condensates forming spontaneously in momentum space. Brillouin Light Scattering studies for a microwavepumped film with submicrometer spatial resolution experimentally confirm the existence of the two wavefunctions and show that their interference results in a nonuniform ground state of the condensate with the density oscillating in space. Moreover, fork dislocations in the density fringes provide direct experimental evidence for the formation of pinned half-quantum vortices in the magnon condensate. The measured amplitude of the density oscillation implies the formation of a nonsymmetric state that corresponds to nonequal occupation of two energy minima. We discuss the experimental findings and consider the theory of magnon condensates, which includes, to leading order, the contribution from the noncondensed magnons. The effect of the noncondensed magnon cloud is to increase the contrast of the asymmetric state and to bring about the experimental measurements. Introduction Magnons are quasiparticles corresponding to quantised spin waves that describe the collective motion of spins [1]. In recent years, it has become possible to realise a BEC of magnons in two remarkably different systems: in superfluid phases of an isotope of helium – Helium-3 at ultralow temperatures [2, 3] and in ferrimagnetic insulators [4, 5, 6, 7]. In the normal, noncondensed state, these magnetic materials exhibit a magnetically ordered state with a gas of magnons whose phases are not correlated. However, once condensation occurs, spins develop phase coherence resulting in a common global frequency and phase of precession. At room temperature, ferrimagnetic insulators, such as yttrium-iron garnet (YIG) films, together with a combination of an in-plane magnetic field and microwave radiation, are required for the magnon condensation [4, 5, 6, 7]. Therefore, in analogy with exciton– polariton condensates, this provides yet another example of a BEC of quasiparticle excitations in a solid-state system. Experimental Realisation of a Bose-Einstein Condensate of Magnons in an Epitaxial YIG-film A room-temperature Bose-Einstein condensate of magnons was created in an epitaxial YIG-film using an experimental setup shown in Fig. 25.1a, which, in general, is similar to that used in our previous studies [4, 5]. Given that magnons are quasiparticle excitations, their number is not conserved and, therefore, the chemical potential is zero.
Bose-Einstein condensation (BEC) is a quantum phenomenon of formation of a collective quantum state in which a macroscopic number of particles occupy the lowest energy state and thus is governed by a single wavefunction. Here we highlight the BEC in a magnetic subsystem--the BEC of magnons, elementary magnetic excitations. The magnon BEC is manifested as the spontaneously emerging state of the precessing spins, in which all spins precess with the same frequency and phase even in an inhomogeneous magnetic field. The coherent spin precession was observed first in superfluid (3)He-B and this domain was called the homogeneously precessing domain (HPD). The main feature of the HPD is the induction decay signal, which ranges over many orders of magnitude longer than is prescribed by the inhomogeneity of magnetic field. This means that spins precess not with a local Larmor frequency, but coherently with a common frequency and phase. This BEC can also be created and stabilized by continuous NMR pumping. In this case the NMR frequency plays the role of a magnon chemical potential, which determines the density of the magnon condensate. The interference between two condensates has also been demonstrated. It was shown that HPD exhibits all the properties of spin superfluidity. The main property is the existence of a spin supercurrent. This spin supercurrent flows separately from the mass current. Transfer of magnetization by the spin supercurrent by a distance of more than 1 cm has been observed. Also related phenomena have been observed: the spin current Josephson effect; the phase-slip processes at the critical current; and the spin current vortex--a topological defect which is the analog of a quantized vortex in superfluids and of an Abrikosov vortex in superconductors; and so on. It is important to mention that the spin supercurrent is a magnetic phenomenon, which is not directly related to the mass superfluidity of (3)He: it is the consequence of a specific antiferromagnetic ordering in superfluid (3)He. Several different states of coherent precession have been observed in (3)He-B: the homogeneously precessing domain (HPD); a persistent signal formed by Q-balls at very low temperatures; coherent precession with fractional magnetization; and two new modes of coherent precession in compressed aerogel. In compressed aerogel the coherent precession has been also found in (3)He-A. We demonstrate that the coherent precession of magnetization is a true BEC of magnons, with the magnon interaction term in the Gross-Pitaevskii equation being provided by spin-orbit coupling which is different for different states of the magnon BEC.
We present a study of magnetic field induced quantum phase transitions in insulating systems. A generalized scaling theory is used to obtain the temperature dependence of several physical quantities along the quantum critical trajectory (H=HCH=H_{C}H=HC​, T→0T\to0T→0) where HHH is a longitudinal external magnetic field and HCH_{C}HC​ the critical value at which the transition occurs. We consider transitions from a spin liquid at a critical field HC1H_{C1}HC1​ and from a fully polarized paramagnet, at HC2H_{C2}HC2​, into phases with long range order in the transverse components. The transitions at HC1H_{C1}HC1​ and HC2H_{C2}HC2​ can be viewed as Bose-Einstein condensations of magnons which however belong to different universality classes since they have different values of the dynamic critical exponent zzz. Finally, we use that the magnetic susceptibility is an entanglement witness to discuss how this type of correlation sets in as the system approaches the quantum critical point along the critical trajectory, H=HC2H=H_{C2}H=HC2​, T→0T\to0T→0.
Under suitable experimental conditions, collective spin-wave excitations, magnons, form a Bose–Einstein condensate (BEC), where the spins precess with a globally coherent phase. Bose–Einstein condensation of magnons has been reported in a few systems, including superfluid phases of 3He, solid state systems, such as yttrium-iron-garnet films, and cold atomic gases. The superfluid phases of 3He provide a nearly ideal test bench for coherent magnon physics owing to experimentally proven spin superfluidity, the long lifetime of the magnon condensate, and the versatility of the accessible phenomena. We first briefly recap the properties of the different magnon BEC systems, with focus on superfluid 3He. The main body of this review summarizes recent advances in the application of magnon BEC as a laboratory to study basic physical phenomena connecting to diverse areas from particle physics and cosmology to vortex dynamics and new phases of condensed matter. This line of research complements the ongoing efforts to utilize magnon BECs as probes and components for potentially room-temperature quantum devices. In conclusion, we provide a roadmap for future directions in the field of applications of magnon BEC to fundamental research.
Bose-Einstein condensation occurs at an appropriate density of bosonic particles, depending on their mass and temperature. The transition from the semiclassical paradigm of spin waves to the magnon Bose-Einstein condensed state (mBEC) was obtained experimentally with increasing magnon density. We used the Faraday rotation effect to study the spatial distribution of the magnon density and phase far from their excitation region. A coherent magnetization precession was observed throughout the sample, which indicates the formation of a magnon BEC. It is shown that this result under experimental conditions goes beyond the applicability of the Landau-Lifshitz-Gilbert semiclassical theory.
We report evidence for the existence of a supercurrent of magnons in a magnon Bose-Einstein condensate (BEC) prepared in a room temperature yttrium-iron-garnet (YIG) magnetic film. The magnon BEC is formed in a parametrically populated magnon gas, and its temporal evolution is studied by time-resolved Brillouin light scattering (BLS) spectroscopy in the area of the BLS laser focus. It has been found that local laser heating in the center of the condensate decreases the density of the magnon BEC in the steady-state pump regime and it enhances the temporal decrease of the freely evolving magnon condensate after the termination of the pumping pulse, but it does not alter the relaxation dynamics of the gaseous magnon phase. This phenomenon is understood as the appearance of a magnon supercurrent within the condensate due to a temperature-gradient induced phase gradient in the condensate. Bose-Einstein condensation [1] can be achieved either by decreasing the temperature of a boson gas [2] or by increasing its density. The latter method is especially applicable to g ases of weakly interacting quasi-particles such as excitons [3] , polaritons [4, 5], photons [6], and magnons [7, 8]. When a spin system is pumped, and when the injected magnons thermalize through scattering processes conserving both their number and the total energy, a Bose-Einstein condensate (BEC) may be formed at the lowest energy state of the energy-momentum spectrum even at room temperature conditions of the magnetic film carrying the magnons [8, 9]. As the condensed magnon phase is localized in the global energy minimum, its group velocity is exactly zero and no energy transport can be associated with the magnon BEC. The situation can change, when a magnon supercurrent driven by a gradient in the phase of the wavefunction of a magnon condensate can be excited. Such a phase gradient can be induced by, e.g., a potential gradient or a temperature gradient. However, the dynamics of magnon condensates in such a gradient is still terra incognita. Here we provide experimental insight into the evolution of a magnon BEC in a thermal gradient generated by local laser heating. We show that such a heating influences both the steady-state characteristics and the transitional behavior of the magno n BEC, which can be understood using the concept of a magnon supercurrent. We study the temporal evolution of a magnon BEC in a single-crystal yttrium iron garnet (YIG, Y3Fe5O12) film by