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arXiv:cond-mat/0603712 · Physical Review Letters

Effect of Superradiance on Transport of Diffusing Photons in Cold Atomic Gases

Aharon Gero, Éric Akkermans

Published Mar 6, 2006• 20 citations
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Abstract

We show that in atomic gases cooperative effects like superradiance and subradiance lead to a potential between two atoms that decays like 1/r. In the case of superradiance, this potential is attractive for close enough atoms and can be interpreted as a coherent mesoscopic effect. The contribution of superradiant pairs to multiple scattering properties of a dilute gas, such as photon elastic mean free path and group velocity, is significantly different from that of independent atoms. We discuss the conditions under which these effects may be observed and compare our results to recent experiments on photon transport in cold atomic gases.

DOI
10.1103/physrevlett.96.093601

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We show that in atomic gases cooperative effects like superradiance and subradiance lead to a potential between two atoms that decays like 1/r. In the case of superradiance, this potential is attractive for close enough atoms and can be interpreted as a coherent mesoscopic effect. The contribution of superradiant pairs to multiple scattering properties of a dilute gas, such as photon elastic mean free path and group velocity, is significantly different from that of independent atoms. We discuss the conditions under which these effects may be observed and compare our results to recent experiments on photon transport in cold atomic gases.
We study the influence of cooperative effects such as superradiance and subradiance on the scattering properties of dilute atomic gases. We show that cooperative effects lead to an effective potential between two atoms that decays as 1∕r1∕r1∕r. In the case of superradiance, this potential is attractive for close enough atoms and can be interpreted as a coherent mesoscopic effect. We consider a model of multiple scattering of a photon among superradiant pairs and calculate the elastic mean free path and the group velocity. We study first the case of a scalar wave which allows us to obtain and to understand basic features of cooperative effects and multiple scattering. We then turn to the general problem of a vector wave. In both cases, we obtain qualitatively similar results and derive, for the case of a scalar wave, analytic expressions for the elastic mean free path and for the group velocity for an arbitrary detuning (near resonance).
Cooperative scattering has been the subject of intense research in the last years. In this article, we discuss the concept of cooperative scattering from a broad perspective. We briefly review the various collective effects that occur when light interacts with an ensemble of atoms. We show that some effects that have been recently discussed in the context of ‘single-photon superradiance’, or cooperative scattering in the linear-optics regime, can also be explained by ‘standard optics’, i.e. using macroscopic quantities such as the susceptibility or the diffusion coefficient. We explain why some collective effects depend on the atomic density, and others on the optical depth. In particular, we show that, for a large and dilute atomic sample driven by a far-detuned laser, the decay of the fluorescence, which exhibits superradiant and subradiant dynamics, depends only on the on-resonance optical depth. We also discuss the link between concepts that are independently studied in the quantum-optics community and in the mesoscopic-physics community. We show that the coupled-dipole model predicts a departure from Ohm’s law for the diffuse light, that incoherent multiple scattering can induce a saturation of fluorescence and we also show the similarity between the weak-localization correction to the diffusion coefficient and the inaccuracy of Lorentz local field correction to the susceptibility.
The problem of the interaction of N atoms with a laser beam and vacuum modes can give rise to many interesting phenomena concerning the spontaneous emission of light and its propagation in the medium. The cooperative effects, for example, such as superadiance and subradiance, are effects related to the coherence created between the atoms when a photon is emitted spontaneously by a single excited atom. Superradiance can be defined as the enhancement of the spontaneous emission due to constructive interference of the scattered light. Its counterpart, subradiance, is the trapping of some remaining light due to destructive interference. In cold atoms, some previous theoretical works predict and characterize these two cooperative effects in a large and diluted atomic cloud, in the regime of low intensities and large detunings of the incident laser. The theoretical model is a coupled-dipole model for two-level atoms driven by a low-intensity field and in the scalar approach. The experiment consists in measuring the super- and subradiant decay rates from the temporal emitted intensity after the switch off of the incident laser in the steady state. Our experimental setup consists in a magneto-optical trap of rubidium 87 atoms at large resonant optical thicknesses. A probe beam excites the atoms close to the D2 line. The intensity emitted is detected by a single photon detector with no afterpulsing and a calibration procedure allows us to determine the resonant optical thickness of the cloud and its temperature. In this work, we report the experimental observation of super- and subradiance in a large cloud of cold atoms. For subradiance, the main result is the linear evolution of the characteristic time with the resonant optical thickness of the cloud and its independence of the detuning. For superradiance, we observe superradiance out of the forward direction. We verify the validity of our interpretations with the predictions of the coupled-dipole model. Finally, we discuss the interplay of subradiance and radiation trapping, as well as theoretical predictions for: a setup of a phased cloud, to control the subradiant amplitude emission; and temperature effects, where subradiance is shown to be robust in a large range of temperatures.
When atoms are coupled to a common electromagnetic environment, the exchange of photons through dipole-dipole interactions leads to the emergence of cooperative effects. As a particular example, superradiance arises from spontaneous emission when this exchange leads to constructive interference of the emitted photons. Here, we introduce an integrated method for studying cooperative radiation in many-body systems. This method, which allows to study extended systems with arbitrarily large number of particles, can be formulated by an effective, nonlinear, two-atom master equation that describes the dynamics using a closed form which treats single- and many-body terms on an equal footing. We apply this method to a homogeneous gas of initially inverted two-level atoms, and demonstrate the appearance of both superradiance and subradiance, identifying a many-body coherence term as the source of these cooperative effects. We describe the many-body induced broadening -- which is analytically found to scale with the optical depth of the system -- and light shifts, and distinguish spontaneous effects from induced ones. In addition, we theoretically predict the time-dependence of subradiance, and the phase change of the radiated field during the cooperative decay.
Superradiance has been extensively studied in the 1970s and 1980s in the regime of superfluorescence, where a large number of atoms are initially excited. Cooperative scattering in the linear-optics regime, or "single-photon superradiance," has been investigated much more recently, and superradiant decay has also been predicted, even for a spherical sample of large extent and low density, where the distance between atoms is much larger than the wavelength. Here, we demonstrate this effect experimentally by directly measuring the decay rate of the off-axis fluorescence of a large and dilute cloud of cold rubidium atoms after the sudden switch off of a low-intensity laser driving the atomic transition. We show that, at large detuning, the decay rate increases with the on-resonance optical depth. In contrast to forward scattering, the superradiant decay of off-axis fluorescence is suppressed near resonance due to attenuation and multiple-scattering effects.