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arXiv:0704.3522 · Physical Review A

Superradiance and multiple scattering of photons in atomic gases

Aharon Gero, Éric Akkermans

Published May 25, 2007• 14 citations
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Abstract

We study the influence of cooperative effects such as superradiance and subradiance on the scattering properties of dilute atomic gases. We show that cooperative effects lead to an effective potential between two atoms that decays as $1∕r$. In the case of superradiance, this potential is attractive for close enough atoms and can be interpreted as a coherent mesoscopic effect. We consider a model of multiple scattering of a photon among superradiant pairs and calculate the elastic mean free path and the group velocity. We study first the case of a scalar wave which allows us to obtain and to understand basic features of cooperative effects and multiple scattering. We then turn to the general problem of a vector wave. In both cases, we obtain qualitatively similar results and derive, for the case of a scalar wave, analytic expressions for the elastic mean free path and for the group velocity for an arbitrary detuning (near resonance).

DOI
10.1103/physreva.75.053413

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We study the influence of cooperative effects such as superradiance and subradiance on the scattering properties of dilute atomic gases. We show that cooperative effects lead to an effective potential between two atoms that decays as 1∕r1∕r1∕r. In the case of superradiance, this potential is attractive for close enough atoms and can be interpreted as a coherent mesoscopic effect. We consider a model of multiple scattering of a photon among superradiant pairs and calculate the elastic mean free path and the group velocity. We study first the case of a scalar wave which allows us to obtain and to understand basic features of cooperative effects and multiple scattering. We then turn to the general problem of a vector wave. In both cases, we obtain qualitatively similar results and derive, for the case of a scalar wave, analytic expressions for the elastic mean free path and for the group velocity for an arbitrary detuning (near resonance).
We show that in atomic gases cooperative effects like superradiance and subradiance lead to a potential between two atoms that decays like 1/r. In the case of superradiance, this potential is attractive for close enough atoms and can be interpreted as a coherent mesoscopic effect. The contribution of superradiant pairs to multiple scattering properties of a dilute gas, such as photon elastic mean free path and group velocity, is significantly different from that of independent atoms. We discuss the conditions under which these effects may be observed and compare our results to recent experiments on photon transport in cold atomic gases.
Cooperative scattering has been the subject of intense research in the last years. In this article, we discuss the concept of cooperative scattering from a broad perspective. We briefly review the various collective effects that occur when light interacts with an ensemble of atoms. We show that some effects that have been recently discussed in the context of ‘single-photon superradiance’, or cooperative scattering in the linear-optics regime, can also be explained by ‘standard optics’, i.e. using macroscopic quantities such as the susceptibility or the diffusion coefficient. We explain why some collective effects depend on the atomic density, and others on the optical depth. In particular, we show that, for a large and dilute atomic sample driven by a far-detuned laser, the decay of the fluorescence, which exhibits superradiant and subradiant dynamics, depends only on the on-resonance optical depth. We also discuss the link between concepts that are independently studied in the quantum-optics community and in the mesoscopic-physics community. We show that the coupled-dipole model predicts a departure from Ohm’s law for the diffuse light, that incoherent multiple scattering can induce a saturation of fluorescence and we also show the similarity between the weak-localization correction to the diffusion coefficient and the inaccuracy of Lorentz local field correction to the susceptibility.
When atoms are coupled to a common electromagnetic environment, the exchange of photons through dipole-dipole interactions leads to the emergence of cooperative effects. As a particular example, superradiance arises from spontaneous emission when this exchange leads to constructive interference of the emitted photons. Here, we introduce an integrated method for studying cooperative radiation in many-body systems. This method, which allows to study extended systems with arbitrarily large number of particles, can be formulated by an effective, nonlinear, two-atom master equation that describes the dynamics using a closed form which treats single- and many-body terms on an equal footing. We apply this method to a homogeneous gas of initially inverted two-level atoms, and demonstrate the appearance of both superradiance and subradiance, identifying a many-body coherence term as the source of these cooperative effects. We describe the many-body induced broadening -- which is analytically found to scale with the optical depth of the system -- and light shifts, and distinguish spontaneous effects from induced ones. In addition, we theoretically predict the time-dependence of subradiance, and the phase change of the radiated field during the cooperative decay.
Mesoscopic interference effects in multiple scattering of photons depend crucially on the internal structure of the scatterers. In the present paper, we develop the analytical theory of multiple photon scattering by cold atoms with arbitrary internal hyperfine multiplets. For a specific application, we calculate the enhancement factor of elastic coherent backscattering as a function of detuning from an entire hyperfine multiplet of neighboring resonances that cannot be considered isolated. Our theory permits one to understand why atoms behave differently from classical Rayleigh point-dipole scatterers, and how the classical description is recovered for larger but still microscopic objects like molecules or clusters.
Superradiance and coherent atomic recoil lasing are two closely related phenomena, both resulting from the cooperative scattering of light by atoms. In ultracold atomic gases below the critical temperature for Bose-Einstein condensation these processes take place with the simultaneous amplification of the atomic matter waves. We explore these phenomena by surveying some of the experimental and theoretical developments that have emerged in this field of study since the first observation of superradiant scattering from a Bose-Einstein condensate in 1999 [1].
Cooperative scattering in cold atoms has gained renewed interest, in particular in the context of single-photon superradiance, with the recent experimental observation of super- and subradiance in dilute atomic clouds. Numerical simulations to support experimental signatures of cooperative scattering are often limited by the number of dipoles which can be treated, well below the number of atoms in the experiments. In this paper, we provide systematic numerical studies aimed at matching the regime of dilute atomic clouds. We use a scalar coupled-dipole model in the low excitation limit and an exclusion volume to avoid density-related effects. Scaling laws for super- and subradiance are obtained and the limits of numerical studies are pointed out. We also illustrate the cooperative nature of light scattering by considering an incident laser field, where half of the beam has a π phase shift. The enhanced subradiance obtained under such condition provides an additional signature of the role of coherence in the detected signal.