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arXiv:2205.15255

Superradiance and Subradiance in Dense Atomic Gases: An Integrated Method

H. Ma, Oriol Rubies-Bigordà, Susanne F. Yelin

Published May 30, 2022• 4 citations
arXivHTMLPDF

Abstract

When atoms are coupled to a common electromagnetic environment, the exchange of photons through dipole-dipole interactions leads to the emergence of cooperative effects. As a particular example, superradiance arises from spontaneous emission when this exchange leads to constructive interference of the emitted photons. Here, we introduce an integrated method for studying cooperative radiation in many-body systems. This method, which allows to study extended systems with arbitrarily large number of particles, can be formulated by an effective, nonlinear, two-atom master equation that describes the dynamics using a closed form which treats single- and many-body terms on an equal footing. We apply this method to a homogeneous gas of initially inverted two-level atoms, and demonstrate the appearance of both superradiance and subradiance, identifying a many-body coherence term as the source of these cooperative effects. We describe the many-body induced broadening -- which is analytically found to scale with the optical depth of the system -- and light shifts, and distinguish spontaneous effects from induced ones. In addition, we theoretically predict the time-dependence of subradiance, and the phase change of the radiated field during the cooperative decay.

DOI
10.48550/arxiv.2205.15255

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When atoms are coupled to a common electromagnetic environment, the exchange of photons through dipole-dipole interactions leads to the emergence of cooperative effects. As a particular example, superradiance arises from spontaneous emission when this exchange leads to constructive interference of the emitted photons. Here, we introduce an integrated method for studying cooperative radiation in many-body systems. This method, which allows to study extended systems with arbitrarily large number of particles, can be formulated by an effective, nonlinear, two-atom master equation that describes the dynamics using a closed form which treats single- and many-body terms on an equal footing. We apply this method to a homogeneous gas of initially inverted two-level atoms, and demonstrate the appearance of both superradiance and subradiance, identifying a many-body coherence term as the source of these cooperative effects. We describe the many-body induced broadening -- which is analytically found to scale with the optical depth of the system -- and light shifts, and distinguish spontaneous effects from induced ones. In addition, we theoretically predict the time-dependence of subradiance, and the phase change of the radiated field during the cooperative decay.
The problem of the interaction of N atoms with a laser beam and vacuum modes can give rise to many interesting phenomena concerning the spontaneous emission of light and its propagation in the medium. The cooperative effects, for example, such as superadiance and subradiance, are effects related to the coherence created between the atoms when a photon is emitted spontaneously by a single excited atom. Superradiance can be defined as the enhancement of the spontaneous emission due to constructive interference of the scattered light. Its counterpart, subradiance, is the trapping of some remaining light due to destructive interference. In cold atoms, some previous theoretical works predict and characterize these two cooperative effects in a large and diluted atomic cloud, in the regime of low intensities and large detunings of the incident laser. The theoretical model is a coupled-dipole model for two-level atoms driven by a low-intensity field and in the scalar approach. The experiment consists in measuring the super- and subradiant decay rates from the temporal emitted intensity after the switch off of the incident laser in the steady state. Our experimental setup consists in a magneto-optical trap of rubidium 87 atoms at large resonant optical thicknesses. A probe beam excites the atoms close to the D2 line. The intensity emitted is detected by a single photon detector with no afterpulsing and a calibration procedure allows us to determine the resonant optical thickness of the cloud and its temperature. In this work, we report the experimental observation of super- and subradiance in a large cloud of cold atoms. For subradiance, the main result is the linear evolution of the characteristic time with the resonant optical thickness of the cloud and its independence of the detuning. For superradiance, we observe superradiance out of the forward direction. We verify the validity of our interpretations with the predictions of the coupled-dipole model. Finally, we discuss the interplay of subradiance and radiation trapping, as well as theoretical predictions for: a setup of a phased cloud, to control the subradiant amplitude emission; and temperature effects, where subradiance is shown to be robust in a large range of temperatures.
Superradiance and subradiance are collective effects that emerge from coherent interactions between quantum emitters. Due to their many-body nature, theoretical studies of extended samples with length larger than the atomic transition wavelength are usually restricted to their early-time behavior or to the few-excitation limit. We use herein a mean-field approach to reduce the complex many-body system to an effective two-atom master equation that includes all correlations up to second order and that can be numerically propagated in time. We find that three-dimensional and two-dimensional inverted atomic arrays sustain superradiance below a critical lattice spacing and quantify the scaling of the superradiant peak for both dimensionalities. Finally, we study the late-time dynamics of the system and demonstrate that a subradiant phase appears before the system finally relaxes.
Recent advances in optical studies of condensed matter systems have led to the emergence of a variety of phenomena that have conventionally been studied in the realm of quantum optics. These studies have not only deepened our understanding of light–matter interactions but have also introduced aspects of many-body correlations inherent in optical processes in condensed matter systems. This paper is concerned with the phenomenon of superradiance (SR), a profound quantum optical process originally predicted by Dicke in 1954. The basic concept of SR applies to a general N body system, where constituent oscillating dipoles couple together through interaction with a common light field and accelerate the radiative decay of the whole system. Hence, the term SR ubiquitously appears in order to describe radiative coupling of an arbitrary number of oscillators in many situations in modern science of both classical and quantum description. In the most fascinating manifestation of SR, known as superfluorescence (SF), an incoherently prepared system of N inverted atoms spontaneously develops macroscopic coherence from vacuum fluctuations and produces a delayed pulse of coherent light whose peak intensity ∝N2. Such SF pulses have been observed in atomic and molecular gases, and their intriguing quantum nature has been unambiguously demonstrated. In this review, we focus on the rapidly developing field of research on SR phenomena in solids, where not only photon-mediated coupling (as in atoms) but also strong Coulomb interactions and ultrafast scattering processes exist. We describe SR and SF in molecular centers in solids, molecular aggregates and crystals, quantum dots, and quantum wells. In particular, we will summarize a series of studies we have recently performed on semiconductor quantum wells in the presence of a strong magnetic field. In one type of experiment, electron-hole pairs were incoherently prepared, but a macroscopic polarization spontaneously emerged and cooperatively decayed, emitting an intense SF burst. In another type of experiment, we observed the SR decay of coherent cyclotron resonance of ultrahigh-mobility 2D electron gases, leading to a decay rate that is proportional to the electron density. These results show that cooperative effects in solid-state systems are not merely small corrections that require exotic conditions to be observed; rather, they can dominate the nonequilibrium dynamics and light emission processes of the entire system of interacting electrons.
Recent advances in generating well controlled dense arrangements of individual atoms in free space have generated interest in understanding how the extended nature of these systems influences superradiance phenomena. Here, we provide an in-depth analysis on how space-dependent light shifts and decay rates induced by dipole-dipole interactions modify the steady-state properties of coherently driven arrays of quantum emitters. We characterize the steady-state phase diagram, with particular focus on the radiative properties in the steady state. Interestingly, we find that diverging from the well-established Dicke paradigm of equal all-to-all interactions significantly modifies the emission properties. In particular, the prominent quadratic scaling of the radiated light intensity with particle number in the steady state—a hallmark of steady-state Dicke superradiance—is entirely suppressed, resulting in only linear scaling with particle number. We show that this breakdown of steady-state superradiance occurs due to the emergence of additional dissipation channels that populate not only superradiant states but also subradiant ones. The additional contribution of subradiant dark states in the dynamics leads to a divergence in the time scales needed to achieve steady states. Building on this, we further show that measurements taken at finite times for extended atom ensembles reveal properties closely mirroring the idealized Dicke scenario. Published by the American Physical Society 2024
Quantum cooperativity is evident in light-matter platforms where quantum emitter ensembles are interfaced with confined optical modes and are coupled via the ubiquitous electromagnetic quantum vacuum. Cooperative aspects such as dipole-dipole interactions and subradiance find applications in the design of nanoscale coherent light sources and highly-reflective quantum metasurfaces made up of hundreds of optically trapped atoms, in the implementation of topological quantum optics on subwavelength arrays of emitters, in quantum metrology and quantum information. The quick bursts of radiation from a collection of quasi-indistiguishable emitters provides an alternative approach to standard lasers by introducing superradiant lasers operating at extremely low intracavity power. This tutorial provides a set of theoretical tools to tackle the behavior responsible for the onset of cooperativity in light-matter systems by extending open quantum system dynamics methods, such as the master equation and quantum Langevin equations, to electron-photon interactions in strongly coupled and correlated quantum emitters ensembles. These analytical approaches are then also extended to frequency disordered or vibronically coupled quantum emitter ensembles with wide relevance ranging from atoms in optical lattices, quantum dots in solid state environments or molecular quantum systems.
Ordered atomic arrays with subwavelength lattice spacing emit light collectively. For fully inverted atomic arrays, this results in an initial burst of radiation and a fast buildup of coherences between the atoms at initial times. Based on a cumulant expansion of the equations of motion, we derive exact analytical expressions for the emission properties and numerically analyze the full many-body problem resulting in the collective decay process for unprecedented system sizes of up to a few hundred atoms. We benchmark the cumulant expansion approach and show that it correctly captures the cooperative dynamics resulting in superradiance. For fully inverted arrays, this allows us to extract the scaling of the superradiant peak with particle number. For partially excited arrays where no coherences are shared among atoms, we also determine the critical number of excitations required for the emergence of superradiance in one- and two-dimensional geometries. In addition, we study the robustness of superradiance in the case of non-unit filling and position disorder.