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arXiv:cond-mat/0603609 · Physical Review B

Condensation of magnons and spinons in a frustrated ladder

J.-B. Fouet, Frédéric Mila, D. Clarke, Hyun Youk, Oleg Tchernyshyov, Paul Fendley, R. M. Noack

Published Jun 6, 2006• 51 citations
arXivHTMLPDF

Abstract

Motivated by the ever-increasing experimental effort devoted to the properties of frustrated quantum magnets in a magnetic field, we present a careful and detailed theoretical analysis of a one-dimensional version of this problem, a frustrated ladder with a magnetization plateau at $m=1∕2$. We show that even for purely isotropic Heisenberg interactions, the magnetization curve exhibits a rather complex behavior that can be fully accounted for in terms of simple elementary excitations. The introduction of anisotropic interactions (e.g., Dzyaloshinskii-Moriya interactions) modifies significantly the picture and reveals an essential difference between integer and fractional plateaus. In particular, anisotropic interactions generically open a gap in the region between the plateaus, but we show that this gap closes upon entering fractional plateaus. All of these conclusions, based on analytical arguments, are supported by extensive density matrix renormalization group calculations.

DOI
10.1103/physrevb.73.214405

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Motivated by the ever-increasing experimental effort devoted to the properties of frustrated quantum magnets in a magnetic field, we present a careful and detailed theoretical analysis of a one-dimensional version of this problem, a frustrated ladder with a magnetization plateau at m=1∕2m=1∕2m=1∕2. We show that even for purely isotropic Heisenberg interactions, the magnetization curve exhibits a rather complex behavior that can be fully accounted for in terms of simple elementary excitations. The introduction of anisotropic interactions (e.g., Dzyaloshinskii-Moriya interactions) modifies significantly the picture and reveals an essential difference between integer and fractional plateaus. In particular, anisotropic interactions generically open a gap in the region between the plateaus, but we show that this gap closes upon entering fractional plateaus. All of these conclusions, based on analytical arguments, are supported by extensive density matrix renormalization group calculations.
We study the T=0T=0T=0 magnetization of frustrated two-leg spin ladders with arbitrary value of the spin SSS. In the strong-rung limit, we use degenerate perturbation theory to prove that frustration leads to magnetization plateaus at fractional values of the magnetization for all spins SSS and to determine the critical ratios of parallel to diagonal inter-rung couplings for the appearance of these plateaus. These ratios depend both on the plateau and on the spin. To confirm these results and to investigate the properties of these ladders away from the strong-coupling limit, we have performed extensive density-matrix renormalization-group calculations for $S\ensuremath{\le}2$. For large enough inter-rung couplings, all plateaus simply disappear, leading to a magnetization curve typical of integer-spin chains in a magnetic field. The intermediate region turns out to be surprisingly rich however, with, upon increasing the inter-rung couplings, the development of magnetization jumps and, in some cases, the appearance of one or more phase transitions inside a given plateau.
We present a solvable ladder model which displays magnetization plateaus at fractional values of the total magnetization. Plateau signatures are also shown to exist along special lines. The model has isotropic Heisenberg interactions with additional many-body terms. The phase diagram can be calculated exactly for all values of the rung coupling and the magnetic field. We also derive the anomalous behavior of the susceptibility near the plateau boundaries. There is good agreement with the phase diagram obtained recently for the pure Heisenberg ladders by numerical and perturbative techniques.
The quantum phase transitions induced by a magnetic field are theoretically studied in a frustrated two-leg spin ladder. Using the density-matrix renormalization-group method, we find some magnetic phase transitions and plateaus in two different cases of strong and weak rung couplings. With the strong rung coupling, the three magnetization plateaus are found at 1/3, 1/2, and 2/3 due to the frustration. Those can be understood in terms of a quasispinon reconstructed from the singlet and the triplets of spins on a rung. The plateau at 1/2 corresponds to the valence bond solid of the quasispinons, while the plateaus at 1/3 and 2/3 can be associated with the array of quasispinons such as the soliton lattice. This is different from the usual Bose-Einstein-condensation picture of triplons. Our results will be useful in understanding magnetization curves in BiCu2PO6{\mathrm{BiCu}}_{2}{\mathrm{PO}}_{6}BiCu2​PO6​.
The quantum phase transitions induced by a magnetic field are theoretically studied in a frustrated two-leg spin ladder. Using the density-matrix renormalization-group method, we find some magnetic phase transitions and plateaux in two different cases of strong and weak rung couplings. With the strong rung coupling, the three magnetization plateaux are found at 1/3, 1/2, and 2/3 due to the frustration. Those can be understood in terms of a quasi-spinon reconstructed from the singlet and the triplets of spins on a rung. The plateau at 1/2 corresponds to the valence bond solid of the quasispinons, while the plateaux at 1/3 and 2/3 can be associated with the array of quasi-spinons such as soliton lattice. This is different from the usual Bose-Einstein-condensation picture of triplons. Our results will be useful to understand magnetization curves in BiCu2PO6.
Magnetization plateaus emerging in quantum spin systems due to spontaneously breaking of translational symmetry have been reported both theoretically and experimentally. The broken symmetry can induce reconstruction of elementary excitations such as Goldstone and Higgs modes, whereas its microscopic mechanism and reconstructed quasiparticle in magnetization-plateau phases have remained unclear so far. Here we theoretically study magnetic excitations in the magnetization-plateau phases of a frustrated spin ladder by using the dynamical density-matrix renormalization-group method. Additionally, analytical approaches with the perturbation theory are performed to obtain an intuitive view of magnetic excitations. A comparison between numerical and analytical results indicates the presence of a reconstructed quasiparticle originating from spontaneously broken translational symmetry, which is realized as a collective mode of the spin trimer called a trimeron.
We show that Dzyaloshinskii-Moriya (DM) interactions can substantially modify the phase diagram of spin-1/2 Heisenberg ladders in a magnetic field provided they compete with exchange. For nonfrustrated ladders, they induce a local magnetization along the DM vector that turns the gapless intermediate phase into an Ising phase with broken translational symmetry, while for frustrated ladders, they extend the Ising order of the half-integer plateau to the surrounding gapless phases of the purely Heisenberg case. Implications for experimental ladder and dimer systems are discussed.