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arXiv:cond-mat/0601652

Trapping of cold atoms by the quadrupole force

Nimrod Moiseyev, Milan Šindelka, Lorenz S. Cederbaum

Published Jan 29, 2006• 0 citations
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Abstract

Cold atoms are traditionally trapped by the dipole force in periodically spaced potential wells induced by the standing laser field. We derive here a theory beyond the conventional dipole approximation which provides field/atom coupling potential terms that so far have not been taken into consideration in theoretical or experimental studies. We show that for some atoms for specific laser parameters despite the absence of dipole transition laser trapping is still possible due to the quadrupole force. Illustrative numerical calculations for Ca and Na trapped by the quadrupole force are given.

DOI
10.48550/arxiv.cond-mat/0601652

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Cold atoms are traditionally trapped by the dipole force in periodically spaced potential wells induced by the standing laser field. We derive here a theory beyond the conventional dipole approximation which provides field/atom coupling potential terms that so far have not been taken into consideration in theoretical or experimental studies. We show that for some atoms for specific laser parameters despite the absence of dipole transition laser trapping is still possible due to the quadrupole force. Illustrative numerical calculations for Ca and Na trapped by the quadrupole force are given.
Manipulation of cold atoms by lasers has so far been studied solely within the framework of the conventional dipole approximation, and the atom-light interaction has been treated using low order perturbation theory. Laser control of atomic motions has been ascribed exclusively to the corresponding light-induced dipole forces. In this work, we present a general theory to derive the potential experienced by an atom in a monochromatic laser field in a context analogous to the Born-Oppenheimer approximation for molecules in the field-free case. The formulation goes beyond the dipole approximation and gives rise to the field-atom coupling potential terms which so far have not been taken into consideration in theoretical or experimental studies. Contrary to conventional approaches, our method is based upon the many electron Floquet theory and remains valid also for high intensity laser fields (i.e., for a strongly nonperturbative atom-light interaction). As an illustration of the developed theory, we investigate the trapping of cold atoms in optical lattices. We find that for some atoms for specific laser parameters, despite the absence of the dipole force, the laser trapping is still possible due to the electric quadrupole forces. Namely, we show that by using realistic laser parameters one can form a quadrupole optical lattice which is sufficiently strong to trap Ca and Na atoms.
We have observed rectified dipole forces acting on three-level atoms in the cascade configuration. Laser cooled and trapped rubidium atoms are illuminated with an intense bichromatic standing wave (780 and 776 nm) tuned near resonance with the 5S1/2{\mathit{S}}_{1/2}S1/2​\ensuremath{\rightarrow}5P3/2{\mathit{P}}_{3/2}P3/2​\ensuremath{\rightarrow}5D5/2{\mathit{D}}_{5/2}D5/2​ transitions. The resulting rectified forces produce periodic potential wells (71-\ensuremath{\mu}m period), which localize the cold atoms. Experimental results are in reasonable agreement with theoretical predictions. These forces may be useful in atom optics and laser traps.
This review describes the methods of trapping cold atoms in electromagnetic fields and in the combined electromagnetic and gravity fields. We discuss first the basic types of the dipole radiation forces used for cooling and trapping atoms in the laser fields. We outline next the fundamentals of the laser cooling of atoms and classify the temperature limits for basic laser cooling processes. The main body of the review is devoted to discussion of atom traps based on the dipole radiation forces, dipole magnetic forces, combined dipole radiation-magnetic forces, and the forces combined of the dipole radiation-magnetic and gravity forces. Physical fundamentals of atom traps operating as waveguides and cavities for cold atoms are also considered. The review ends with the applications of cold and trapped atoms in atomic, molecular and optical physics.
Recent studies have confirmed the coupling of optical vortices, such as Laguerre-Gaussian and Bessel-Gaussian modes, to quadrupole-active atomic transitions. This interaction has been shown to be enhanced considerably in the case of Laguerre-Gaussian beams due to the gradient coupling, particularly, in the case of a relatively large winding number. Here, we consider the trapping and the dynamics of atoms in the optical quadrupole potential generated by two coaxial counterpropagating optical vortex beams. We focus on the atomic transition $6{\phantom{\rule{0.16em}{0ex}}}^{2}{S}_{1/2}\ensuremath{\rightarrow}5{\phantom{\rule{0.16em}{0ex}}}^{2}{D}_{5/2}$ in Cs which is a dipole-forbidden but a quadrupole-allowed transition. We show how this atomic transition engages with the optical vortex fields at near resonance, leading to atom trapping in the optical quadrupole potential well accompanied by translational motion. We show how the optical forces generate the motion of the atoms trapped within the quadrupole potential, illustrating the results using typical experimentally accessible parameters.
The theory of an atom dipole trap composed of a focused, far red-detuned, trapping laser beam, and a pair of red-detuned, counterpropagating, cooling beams is developed for the simplest realistic multilevel dipole interaction scheme based on a model of a (3+5)-level atom. The description of atomic motion in the trap is based on the quantum kinetic equations for the atomic density matrix and the reduced quasiclassical kinetic equation for atomic distribution function. It is shown that when the detuning of the trapping field is much larger than the detuning of the cooling field, and with low saturation, the one-photon absorption (emission) processes responsible for the trapping potential can be well separated from the two-photon processes responsible for sub-Doppler cooling atoms in the trap. Two conditions are derived that are necessary and sufficient for stable atomic trapping. The conditions show that stable atomic trapping in the optical dipole trap can be achieved when the trapping field has no effect on the two-photon cooling process and when the cooling field does not change the structure of the trapping potential but changes only the numerical value of the trapping potential well. It is concluded that the separation of the trapping and cooling processes in a pure optical dipole trap allows one to cool trapped atoms down to a minimum temperature close to the recoil temperature, keeping simultaneously a deep potential well.
A cold atomic gas with an inverted population on a transition coupled to a field mode of an optical resonator constitutes a generic model of a laser. For quasi-continuous operation, external pumping, trapping and cooling of the atoms is required to confine them in order to achieve enough gain inside the resonator. As inverted atoms are high-field seekers in blue detuned light fields, tuning the cavity mode to the blue side of the atomic gain transition allows for combining lasing with stimulated cavity cooling and dipole trapping of the atoms at the antinodes of the laser field. We study such a configuration using a semiclassical description of particle motion along the cavity axis. In extension of earlier work we include free space atomic and cavity decay as well as atomic dipole-dipole interactions and their corresponding forces. We show that for a proper choice of parameters even in the bad cavity limit the atoms can create a sufficiently strong field inside the resonator such that they are trapped and cooled via the superradiant lasing action with less than one photon on average inside the cavity.