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Physical Review A

Dipole and quadrupole forces exerted on atoms in laser fields: The nonperturbative approach

Milan Šindelka, Nimrod Moiseyev, Lorenz S. Cederbaum

Published Nov 29, 2006• 13 citations
Publisher

Abstract

Manipulation of cold atoms by lasers has so far been studied solely within the framework of the conventional dipole approximation, and the atom-light interaction has been treated using low order perturbation theory. Laser control of atomic motions has been ascribed exclusively to the corresponding light-induced dipole forces. In this work, we present a general theory to derive the potential experienced by an atom in a monochromatic laser field in a context analogous to the Born-Oppenheimer approximation for molecules in the field-free case. The formulation goes beyond the dipole approximation and gives rise to the field-atom coupling potential terms which so far have not been taken into consideration in theoretical or experimental studies. Contrary to conventional approaches, our method is based upon the many electron Floquet theory and remains valid also for high intensity laser fields (i.e., for a strongly nonperturbative atom-light interaction). As an illustration of the developed theory, we investigate the trapping of cold atoms in optical lattices. We find that for some atoms for specific laser parameters, despite the absence of the dipole force, the laser trapping is still possible due to the electric quadrupole forces. Namely, we show that by using realistic laser parameters one can form a quadrupole optical lattice which is sufficiently strong to trap Ca and Na atoms.

DOI
10.1103/physreva.74.053420

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Manipulation of cold atoms by lasers has so far been studied solely within the framework of the conventional dipole approximation, and the atom-light interaction has been treated using low order perturbation theory. Laser control of atomic motions has been ascribed exclusively to the corresponding light-induced dipole forces. In this work, we present a general theory to derive the potential experienced by an atom in a monochromatic laser field in a context analogous to the Born-Oppenheimer approximation for molecules in the field-free case. The formulation goes beyond the dipole approximation and gives rise to the field-atom coupling potential terms which so far have not been taken into consideration in theoretical or experimental studies. Contrary to conventional approaches, our method is based upon the many electron Floquet theory and remains valid also for high intensity laser fields (i.e., for a strongly nonperturbative atom-light interaction). As an illustration of the developed theory, we investigate the trapping of cold atoms in optical lattices. We find that for some atoms for specific laser parameters, despite the absence of the dipole force, the laser trapping is still possible due to the electric quadrupole forces. Namely, we show that by using realistic laser parameters one can form a quadrupole optical lattice which is sufficiently strong to trap Ca and Na atoms.
Cold atoms are traditionally trapped by the dipole force in periodically spaced potential wells induced by the standing laser field. We derive here a theory beyond the conventional dipole approximation which provides field/atom coupling potential terms that so far have not been taken into consideration in theoretical or experimental studies. We show that for some atoms for specific laser parameters despite the absence of dipole transition laser trapping is still possible due to the quadrupole force. Illustrative numerical calculations for Ca and Na trapped by the quadrupole force are given.
The usual form of electromagnetic forces is given by but for neutral atoms q = 0. The next order of force is the dipole term, but this also vanishes because neutral atoms have no inherent dipole moment. However, a dipole moment can be induced by a field, and this is most efficient if the field is alternating near the atomic resonance frequency. Since these frequencies are typically in the optical range, dipole moments are efficiently induced by shining nearly resonant light on the atoms. Laser cooling and trapping rely on the interaction between laser light and atoms to exert a controllable force on the atoms, and many sophisticated schemes have been developed using the special properties of the interaction. This chapter begins with the simplest schemes for exerting optical forces on atoms, namely a single-frequency light field interacting with a two-level atom. Although this is the simplest possible scheme, it is pedagogically valuable because it shows many of the features that will be encountered further on. The ultimate temperature using such a scheme is limited, but lower temperatures can be achieved with multilevel atoms. This topic is addressed later in the chapter. Two kinds of optical forces When an atom absorbs nearly resonant light, it makes a transition to the excited state, and its subsequent return to the ground state can be either by spontaneous or by stimulated emission. The nature of the optical force that arises from these two different processes is quite different, and will be described separately [1]. The spontaneous emission case is different from the familiar quantum mechanical calculations using state vectors to describe the state of the system, because spontaneous emission causes the state of the system to evolve from a pure state into a mixed state (see Exercise 6.9). Spontaneous emission is an essential ingredient for the dissipative nature of the optical forces in monochromatic light, and the density matrix is needed to describe it (see Chap. 6). When an atom absorbs light, its energy excites the atom and its angular momentum changes the electron's orbit. Both of these are internal atomic properties. However, the linear momentum of the light, can change only the external, translational motion of the atom.
Recent years have witnessed considerable interest in simulating the dynamics of complex many-body systems by well-controlled cold atom model systems. Among others, magnetic ordering phenomena draw a lot of attention. We demonstrated an unconventional approach to light mediated atomic interactions using laser light undergoing diffraction [1]. Diffractive propagation of periodically modulated light fields leads to an exchange between phase and amplitude modulated planes (Talbot effect) which can be used to couple atomic degrees of freedom. In a feedback scheme this can lead to the spontaneous formation of coupled lattices in the light field and the atomic degrees of freedom. After adiabatic elimination of the dynamics of the light field, one is left with light mediated atomic interactions. The coupling can occur via optomechanical nonlinearities [1] or via optical pumping [2]. In the latter case, the result is a spontaneous magnetic ordering in the atomic cloud, a spin or a magnetic dipole pattern [2]. We will provide further details on the latter as well as evidence for novel alignment patterns, corresponding to quadrupole states.
The theory of an atom dipole trap composed of a focused, far red-detuned, trapping laser beam, and a pair of red-detuned, counterpropagating, cooling beams is developed for the simplest realistic multilevel dipole interaction scheme based on a model of a (3+5)-level atom. The description of atomic motion in the trap is based on the quantum kinetic equations for the atomic density matrix and the reduced quasiclassical kinetic equation for atomic distribution function. It is shown that when the detuning of the trapping field is much larger than the detuning of the cooling field, and with low saturation, the one-photon absorption (emission) processes responsible for the trapping potential can be well separated from the two-photon processes responsible for sub-Doppler cooling atoms in the trap. Two conditions are derived that are necessary and sufficient for stable atomic trapping. The conditions show that stable atomic trapping in the optical dipole trap can be achieved when the trapping field has no effect on the two-photon cooling process and when the cooling field does not change the structure of the trapping potential but changes only the numerical value of the trapping potential well. It is concluded that the separation of the trapping and cooling processes in a pure optical dipole trap allows one to cool trapped atoms down to a minimum temperature close to the recoil temperature, keeping simultaneously a deep potential well.
A cold atomic gas with an inverted population on a transition coupled to a field mode of an optical resonator constitutes a generic model of a laser. For quasi-continuous operation, external pumping, trapping and cooling of the atoms is required to confine them in order to achieve enough gain inside the resonator. As inverted atoms are high-field seekers in blue detuned light fields, tuning the cavity mode to the blue side of the atomic gain transition allows for combining lasing with stimulated cavity cooling and dipole trapping of the atoms at the antinodes of the laser field. We study such a configuration using a semiclassical description of particle motion along the cavity axis. In extension of earlier work we include free space atomic and cavity decay as well as atomic dipole-dipole interactions and their corresponding forces. We show that for a proper choice of parameters even in the bad cavity limit the atoms can create a sufficiently strong field inside the resonator such that they are trapped and cooled via the superradiant lasing action with less than one photon on average inside the cavity.
A cold atomic gas with an inverted population on a transition coupled to a field mode of an optical resonator constitutes a generic model of a laser. For quasi-continuous operation, external pumping, trapping and cooling of the atoms is required to confine them in order to achieve enough gain inside the resonator. As inverted atoms are high-field seekers in blue detuned light fields, tuning the cavity mode to the blue side of the atomic gain transition allows for combining lasing with stimulated cavity cooling and dipole trapping of the atoms at the antinodes of the laser field. We study such a configuration using a semiclassical description of particle motion along the cavity axis. In extension of earlier work we include free space atomic and cavity decay as well as atomic dipole-dipole interactions and their corresponding forces. We show that for a proper choice of parameters even in the bad cavity limit the atoms can create a sufficiently strong field inside the resonator such that they are trapped and cooled via the superradiant lasing action with less than one photon on average inside the cavity.