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arXiv:cond-mat/0601302 · Physical Review Letters

Quantum Magnetism with Multicomponent Dipolar Molecules in an Optical Lattice

Ryan Barnett, Dmitry S. Petrov, Mikhail D. Lukin, Eugene Demler

Published May 16, 2006• 208 citations
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Abstract

We consider bosonic dipolar molecules in an optical lattice prepared in a mixture of different rotational states. The 1/R(3) interaction between molecules for this system is produced by exchanging a quantum of angular momentum between two molecules. We show that the Mott states of such systems have a large variety of quantum phases characterized by dipolar orderings including a state with an ordering wave vector that can be changed by tilting the lattice. As the Mott insulating phase is melted, we also describe several exotic superfluid phases that will occur.

DOI
10.1103/physrevlett.96.190401

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We consider bosonic dipolar molecules in an optical lattice prepared in a mixture of different rotational states. The 1/R(3) interaction between molecules for this system is produced by exchanging a quantum of angular momentum between two molecules. We show that the Mott states of such systems have a large variety of quantum phases characterized by dipolar orderings including a state with an ordering wave vector that can be changed by tilting the lattice. As the Mott insulating phase is melted, we also describe several exotic superfluid phases that will occur.
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The superfluid--Mott-insulator phase transition of dipolar bosons in optical lattice is analyzed. By using the Bogoliubov approach and decoupling approximation, the energy spectrum and zero-temperature phase diagram of dipolar bosonic atoms in an optical lattice are obtained analytically. The results show that in these systems the superfluid--Mott-insulator phase transition can be induced by tuning the dipole-dipole interaction and the position of the phase boundary can be moved when the on-site interaction is varied. Corresponding to a large on-site interaction, the dipole-dipole interaction is attractive near the critical point of the superfluid--Mott-insulator phase transition.
The competition between tunneling and interactions in bosonic lattice models generates a whole variety of different quantum phases. While, in the presence of a single species interacting via on site interaction, the phase diagram presents only superfluid or Mott insulating phases, for long-range interactions or multiple species, exotic phases such as supersolid or pair-superfluid appear. In this Letter, we show for the first time that the coexistence of effective multiple species and long-range interactions leads to the formation of a novel pair-supersolid phase, namely, a supersolid of composites. We propose a possible implementation with dipolar bosons in a bilayer two-dimensional optical lattice.
We show that multichannel interactions significantly alter the phase diagram of ultracold bosonic molecules in an optical lattice. Most prominently, an unusual fluid region intervenes between the conventional superfluid and the Mott insulator. In it, number fluctuations remain but phase coherence is suppressed by a significant factor. This factor can be made arbitrarily large, at least in a two-site configuration. We calculate the phase diagram using complementary methods, including Gutzwiller mean-field and density-matrix renormalization group calculations. Although we focus on bosonic molecules without dipolar interactions, we expect multichannel interactions to remain important for dipolar interacting and fermionic molecules.
We present a theoretical analysis of the phase diagram of two-component bosons on an optical lattice. A new formalism is developed which treats the effective spin interactions in the Mott and superfluid phases on the same footing. Using this new approach we chart the phase boundaries of the broken spin symmetry states up to the Mott to superfluid transition and beyond. Near the transition point, the magnitude of spin exchange can be very large, which facilitates the experimental realization of spin-ordered states. We find that spin and quantum fluctuations have a dramatic effect on the transition, making it first order in extended regions of the phase diagram. When each species is at integer filling, an additional phase transition may occur, from a spin-ordered insulator to a Mott insulator with no broken symmetries. We determine the phase boundaries in this regime and show that this is essentially a Mott transition in the spin sector.