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arXiv:cond-mat/0505603 · Physical Review Letters

Bose-Glass Phases in Disordered Quantum Magnets

Omid Nohadani, Stefan Weßel, Stephan Haas

Published Nov 21, 2005• 50 citations
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Abstract

In disordered spin systems with antiferromagnetic Heisenberg exchange, transitions into and out of a magnetic-field-induced ordered phase pass through unique regimes. Using quantum Monte Carlo simulations to study the zero-temperature behavior, these intermediate regions are determined to be Bose-glass phases. The localization of field-induced triplons causes a finite compressibility and, hence, glassiness in the disordered phase.

DOI
10.1103/physrevlett.95.227201

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In disordered spin systems with antiferromagnetic Heisenberg exchange, transitions into and out of a magnetic-field-induced ordered phase pass through unique regimes. Using quantum Monte Carlo simulations to study the zero-temperature behavior, these intermediate regions are determined to be Bose-glass phases. The localization of field-induced triplons causes a finite compressibility and, hence, glassiness in the disordered phase.
The phase diagram of the Bose-Hubbard model in the presence of off-diagonal disorder is determined using quantum Monte Carlo simulations. A sequence of quantum glass phases intervene at the interface between the Mott insulating and the superfluid phases of the clean system. In addition to the standard Bose glass phase, the coexistence of gapless and gapped regions close to the Mott insulating phase leads to a novel Mott glass regime which is incompressible yet gapless. Numerical evidence for the properties of these phases is given in terms of global (compressibility, superfluid stiffness) and local (compressibility, momentum distribution) observables.
We examine the effects of disorder on dimerized quantum antiferromagnets in a magnetic field, using the mapping to a lattice gas of hard-core bosons with finite-range interactions. Combining a strong-coupling expansion, the replica method, and a one-loop renormalization-group analysis, we investigate the nature of the glass phases formed. We find that away from the tips of the Mott lobes, the transition is from a Mott insulator to a compressible Bose glass, however the compressibility at the tips is strongly suppressed. We identify this finding with the presence of a rare Mott glass phase and demonstrate that the inclusion of replica symmetry breaking is vital to correctly describe the glassy phases. This result suggests that the formation of Bose and Mott glass phases is not simply a weak localization phenomenon but is indicative of much richer physics. We discuss our results in the context of both ultracold atomic gases and spin-dimer materials.
We discuss a magnetically ordered (``superfluid'') phase near quantum transition to the Bose-glass phase in a simple modeling system, a Heisenberg antiferromagnet with spatial dimension d>2d>2d>2 in an external magnetic field with disorder in exchange coupling constants. Our analytical consideration is based on hydrodynamic description of long-wavelength excitations. Results obtained are valid in the entire critical region near the quantum critical point (QCP), allowing us to describe a possible crossover from one critical behavior to another. We demonstrate that the system behaves in full agreement with predictions by M. P. Fisher et al. [Phys. Rev. B 40, 546 (1989)] in close vicinity to the QCP. We find as an extension to that analysis that the anomalous dimension $\ensuremath{\eta}=2\ensuremath{-}d$ and $\ensuremath{\beta}=\ensuremath{\nu}d/2$, where $\ensuremath{\beta}$ and $\ensuremath{\nu}$ are critical exponents of the order parameter and the correlation length, respectively. The density of states per spin of low-energy localized excitations is found to be independent of ddd (``superuniversal''). We show that many recent experimental and numerical results obtained in various three-dimensional (3D) systems can be described by our formulas using percolation critical exponents. Then, it is a possibility that a percolation critical regime arises in the ordered phase in some 3D systems not very close to the QCP.
Bosonic excitations within long-range ordered, but strongly inhomogeneous phases have been studied in quite some detail. My thesis focuses instead on understanding the insulating, localized phase of disordered bosonic systems. In particular I study localization properties of strongly interacting bosons and spin systems in a disorder potential at zero temperature. I focus on simple, prototypical spin models (Ising model and XY model) in random fields on a Cayley tree with large connectivity. Regarding the nature of the quantum phase transition in strong disorder I find the following results: i) With a uniformly distributed disorder non-extensive excitations in the disordered phase are all localized. ii)Moreover, I find that the order arises due to a collective condensation, which is qualitatively distinct from a Bose Einstein condensation of single particle excitations into a delocalized state. In particular, in non-frustrated Bose glasses, I do not find evidence for a boson mobility edge in the Bose glass. These results are qualitatively different from claims in the recent literatures . Considering that (many body) localization of bosons is a kind of quantum glass transition, it is an interesting question to ask what phenomena occur, if the ingredients for more conventional (classical) glassy physics are added to a disordered bosons system, namely: random, frustrated interactions between the bosons. One can still think about such a system as bosons in a disordered potential, where the disordered potential is, at least partly, self-generated by random frustrated interactions between the bosons. This question takes us to the study of another type of disordered systems: glassy systems. Those are typically characterized by low temperature phases with an inhomogeneous density or magnetization pattern, which is extremely long-lived due to the occurrence of non-trivial ergodicity breaking. I study a solvable model of hard core bosons (pseudospins) subject to disorder and frustrating interactions. This solvable model provides insight into the possibility of coexistence of super uidity and glassy density order, as well as into the nature of the coexistence phase (the superglass). In particular, for the considered mean field model I prove the existence of a superglass phase. This complements the numerical evidence for such phases provided by quantum Monte Carlo investigations in finite dimensions and on random graphs. Those were, however, limited to finite temperature, and could thus not fully elucidate the structure of the phases at T = 0. In contrast, my analytical approach allows one to understand the quantum phase transition between glassy superfluid and insulator, and the non-trivial role played by glassy correlations. When the frustrated interactions are strong enough, the superfluid order may be destroyed. As I will show in a mean field model, this happens within the glass phase of the system, where a disorder induced superfluid-insulator phase transition takes place to give way to a frustrated Bose glass. The glassy background on top of which this happens leads to many interesting phenomena which seem not to have been noticed before. To understand the nature of the glassy superfluid-insulator quantum phase transition at zero temperature and the transport properties on the insulating, Bose glass side of the transition is the goal of the third part of my thesis. To address the above questions, I studied an exactly solvable model of a glassy superfluid-insulator quantum phase transition on a Bethe lattice geometry with high connectivity. My main results can be summarized as follows: i) I found that the superfluid-insulator transition is shifted to stronger hopping. This is a result of the pseudo gap in the density of states of the glass state, which tends to strongly disfavor the onset of superfluidity. ii) In the glassy insulator, the discrete local energy levels become broadened due to the quantum fluctuations.The level-broadening process appears as a phase transition which has strong similarities with an Anderson localization transition, and has implications on many body localization. By using the locator expansion for bosons I found that, the glassy insulator has a finite mobility edge for the bosonic excitations, which, however, does not close upon approaching the SI quantum phase transition point. This finding helps to understand the nature of the superfluid-to-frustrated Bose glass transition: the superfluid emerges as a collective phase ordering phenomenon at zero temperature, and not as a condensation in to a single particle delocalized state, in contrast to opposite predictions in the recent literatures. The existence of a mobility edge in the insulator suggests the possibility of phononless, activated transport in the bosonic insulator, which might be a candidate explanation for the experimentally seen activated transport, which has remained a mystery for a long time.
The field-induced antiferromagnetic ordering in systems of weakly coupled S = 1/2 dimers at zero temperature can be described as a Bose-Einstein condensation of triplet quasiparticles (singlet quasiholes) in the ground state. For the case of a Heisenberg bilayer, it is here shown how the above picture is altered in the presence of site dilution of the magnetic lattice. Geometric randomness leads to quantum localization of the quasiparticles or quasiholes and to an extended Bose-glass phase in a realistic disordered model. This localization phenomenon drives the system towards a quantum-disordered phase well before the classical geometric percolation threshold is reached.
Site dilution of spin-gapped antiferromagnets leads to localized free moments, which can order antiferromagnetically in two and higher dimensions. Here we show how a weak magnetic field drives this order-by-disorder state into a novel disordered-local-moment (DLM) phase, characterized by the formation of local singlets between neighboring moments and by localized moments aligned antiparallel to the field. This disordered phase is characterized by the absence of a gap, as is the case in a Bose glass. The associated field-driven quantum phase transition is consistent with the universality of a superfluid-to-Bose-glass transition. The robustness of the DLM phase and its prominent features, in particular a series of pseudo-plateaus in the magnetization curve, makes it accessible and relevant to experiments.