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arXiv:1506.08029 · Physical Review B

Bose and Mott glass phases in dimerized quantum antiferromagnets

S. J. Thomson, Frank Krüger

Published Nov 4, 2015• 9 citations
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Abstract

We examine the effects of disorder on dimerized quantum antiferromagnets in a magnetic field, using the mapping to a lattice gas of hard-core bosons with finite-range interactions. Combining a strong-coupling expansion, the replica method, and a one-loop renormalization-group analysis, we investigate the nature of the glass phases formed. We find that away from the tips of the Mott lobes, the transition is from a Mott insulator to a compressible Bose glass, however the compressibility at the tips is strongly suppressed. We identify this finding with the presence of a rare Mott glass phase and demonstrate that the inclusion of replica symmetry breaking is vital to correctly describe the glassy phases. This result suggests that the formation of Bose and Mott glass phases is not simply a weak localization phenomenon but is indicative of much richer physics. We discuss our results in the context of both ultracold atomic gases and spin-dimer materials.

DOI
10.1103/physrevb.92.180201

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We examine the effects of disorder on dimerized quantum antiferromagnets in a magnetic field, using the mapping to a lattice gas of hard-core bosons with finite-range interactions. Combining a strong-coupling expansion, the replica method, and a one-loop renormalization-group analysis, we investigate the nature of the glass phases formed. We find that away from the tips of the Mott lobes, the transition is from a Mott insulator to a compressible Bose glass, however the compressibility at the tips is strongly suppressed. We identify this finding with the presence of a rare Mott glass phase and demonstrate that the inclusion of replica symmetry breaking is vital to correctly describe the glassy phases. This result suggests that the formation of Bose and Mott glass phases is not simply a weak localization phenomenon but is indicative of much richer physics. We discuss our results in the context of both ultracold atomic gases and spin-dimer materials.
We investigate the nature of the Bose glass phase of the disordered Bose-Hubbard model in d>2d>2d>2 and demonstrate the existence of a glass-like replica symmetry breaking (RSB) order parameter in terms of particle number fluctuations. Starting from a strong-coupling expansion around the atomic limit, we study the instability of the Mott insulator towards the formation of a Bose glass. We add some infinitesimal RSB, following the Parisi hierarchical approach in the most general form, and observe its flow under the momentum-shell renormalization group scheme. We find a new fixed point with one-step RSB, corresponding to the transition between the Mott insulator and a Bose glass phase with hitherto unseen RSB. The susceptibility associated to infinitesimal RSB perturbation in the Mott insulator is found to diverge at the transition with an exponent of γ=1/dγ=1/dγ=1/d. Our findings are consistent with the expectation of glassy behavior and the established breakdown of self-averaging. We discuss the possibility of measuring the glass-like order parameter in optical lattice experiments as well as in certain spin systems that are in the same universality class as the Bose-Hubbard model.
This thesis contains four studies of the effects of disorder and randomness on strongly correlated quantum phases of matter. Starting with an itinerant ferromagnet, I first use an order-by-disorder approach to show that adding quenched charged disorder to the model generates new quantum fluctuations in the vicinity of the quantum critical point which lead to the formation of a novel magnetic phase known as a helical glass. Switching to bosons, I then employ a momentum-shell renormalisation group analysis of disordered lattice gases of bosons where I show that disorder breaks ergodicity in a non-trivial way, leading to unexpected glassy freezing effects. This work was carried out in the context of ultracold atomic gases, however the same physics can be realised in dimerised quantum antiferromagnets. By mapping the antiferromagnetic model onto a hard-core lattice gas of bosons, I go on to show the importance of the non-ergodic effects to the thermodynamics of the model and find evidence for an unusual glassy phase known as a Mott glass not previously thought to exist in this model. Finally, I use a mean-field numerical approach to simulate current generation quantum gas microscopes and demonstrate the feasibility of a novel measurement scheme designed to measure the Edwards-Anderson order parameter, a quantity which describes the degree of ergodicity breaking and which has never before been experimentally measured in any strongly correlated quantum system. Together, these works show that the addition of disorder into strongly interacting quantum systems can lead to qualitatively new behaviour, triggering the formation of new phases and new physics, rather than simply leading to small quantitative changes to the physics of the clean system. They provide new insights into the underlying physics of the models and make direct connection with experimental systems which can be used to test the results presented here.
We study quantum phase transitions of Mott insulators between spin-glass and featureless paramagnetic phases. Specifically, we consider a triangular-lattice bilayer Heisenberg model with bond disorder. The clean system has two phases, a dimer quantum paramagnet and a non-collinear antiferromagnet, separated by a quantum critical point. Bond disorder destroys the antiferromagnetic phase via the interference of dipolar textures and results in spin-glass order, such that the system features a quantum phase transition between spin-glass and dimer phases. We study the vicinity of this transition using a variant of bond-operator theory and calculate thermodynamic observables as well as excitation spectra. Bond disorder leads to strong inhomogeneities near the transition which suppresses non-collinearities and leads to anomalously weak glassiness in the near-critical quantum spin glass. We characterize the low-energy excitations which have a strong tendency towards spatial localization, and we track the behavior of the amplitude (i.e. Higgs) mode across the glass phase whose spectral weight we find to be strongly suppressed due to interference effects.
We investigate the instabilities of the Mott-insulating phase of the weakly disordered Bose-Hubbard model within a renormalization group analysis of the replica field theory obtained by a strong-coupling expansion around the atomic limit. We identify an order parameter and associated correlation length scale that are capable of capturing the transition from a state with zero compressibility, the Mott insulator, to one in which the compressibility is finite, the Bose glass. The order parameter is the relative variance of the disorder-induced mass distribution. In the Mott insulator, the relative variance renormalizes to zero, whereas it diverges in the Bose glass. The divergence of the relative variance signals the breakdown of self-averaging. The length scale governing the breakdown of self-averaging is the distance between rare regions. This length scale is finite in the Bose glass but diverges at the transition to the Mott insulator with an exponent of $\ensuremath{\nu}=1/D$ for incommensurate fillings. Likewise, the compressibility vanishes with an exponent of $\ensuremath{\gamma}=4/D\ensuremath{-}1$ at the transition. At commensurate fillings, the transition is controlled by a different fixed point at which both the disorder and interaction vertices are relevant.
Quantum phases of ultracold bosons with repulsive interactions in lattices in the presence of quenched disorder are investigated. The disorder is assumed to be caused by the interaction of the bosons with impurity atoms having a large effective mass. The system is described by the Bose-Hubbard Hamiltonian with random on-site energies which have a discrete binary probability distribution. The phase diagram at zero temperature is calculated using several methods like a strong-coupling expansion, an exact numerical diagonalization, and a Bose-Fermi mapping valid in the hard-core limit. It is shown that the Mott-insulator phase exists for any strength of disorder in contrast to the case of continuous probability distribution. We find that the compressibility of the Bose glass phase varies in a wide range and can be extremely low. Furthermore, we evaluate experimentally accessible quantities like the momentum distribution, the static and dynamic structure factors, and the density of excited states. The influence of finite temperature is discussed as well.