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arXiv:cond-mat/0507157 · Physical Review Letters

Quantum Localization in Bilayer Heisenberg Antiferromagnets with Site Dilution

Tommaso Roscilde, Stephan Haas

Published Nov 10, 2005• 22 citations
arXivHTMLPDF

Abstract

The field-induced antiferromagnetic ordering in systems of weakly coupled S = 1/2 dimers at zero temperature can be described as a Bose-Einstein condensation of triplet quasiparticles (singlet quasiholes) in the ground state. For the case of a Heisenberg bilayer, it is here shown how the above picture is altered in the presence of site dilution of the magnetic lattice. Geometric randomness leads to quantum localization of the quasiparticles or quasiholes and to an extended Bose-glass phase in a realistic disordered model. This localization phenomenon drives the system towards a quantum-disordered phase well before the classical geometric percolation threshold is reached.

DOI
10.1103/physrevlett.95.207206

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The field-induced antiferromagnetic ordering in systems of weakly coupled S = 1/2 dimers at zero temperature can be described as a Bose-Einstein condensation of triplet quasiparticles (singlet quasiholes) in the ground state. For the case of a Heisenberg bilayer, it is here shown how the above picture is altered in the presence of site dilution of the magnetic lattice. Geometric randomness leads to quantum localization of the quasiparticles or quasiholes and to an extended Bose-glass phase in a realistic disordered model. This localization phenomenon drives the system towards a quantum-disordered phase well before the classical geometric percolation threshold is reached.
We numerically investigate the phase diagram of two-dimensional site-diluted coupled dimer systems in an external magnetic field. We show that this phase diagram is characterized by the presence of an extended Bose glass, not accessible to mean-field approximation, and stemming from the localization of two distinct species of bosonic quasiparticles appearing in the ground state. On the one hand, nonmagnetic impurities doped into the dimer-singlet phase of a weakly coupled dimer system are known to free up local magnetic moments. The deviations of these local moments from full polarization along the field can be mapped onto a gas of bosonic quasiparticles, which undergo condensation in zero and very weak magnetic fields, corresponding to transverse long-range antiferromagnetic order. An increasing magnetic field lowers the density of such quasiparticles to a critical value at which a quantum phase transition occurs, corresponding to the quasiparticle localization on clusters of local magnets (dimers, trimers, etc.) and to the onset of a Bose glass. Strong finite-size quantum fluctuations hinder further depletion of quasiparticles from such clusters, and thus lead to the appearance of pseudoplateaus in the magnetization curve of the system. On the other hand, site dilution hinders the field-induced Bose-Einstein condensation of triplet quasiparticles on the intact dimers, and it introduces instead a Bose glass of triplets. A thorough numerical investigation of the phase diagram for a planar system of coupled dimers shows that the two above-mentioned Bose glass phases are continuously connected, and they overlap in a finite region of parameter space, thus featuring a two-species Bose glass. The quantum phase transition from Bose glass to magnetically ordered phases in two dimensions is marked by novel universal exponents ($z\ensuremath{\approx}2$, $\ensuremath{\beta}\ensuremath{\approx}0.9$, and $\ensuremath{\nu}\ensuremath{\approx}1$). Hence we conclude that doped quantum antiferromagnets in a field represent an ideal setting for the study of fundamental dirty-boson physics.
Site dilution of spin-gapped antiferromagnets leads to localized free moments, which can order antiferromagnetically in two and higher dimensions. Here we show how a weak magnetic field drives this order-by-disorder state into a novel disordered-local-moment (DLM) phase, characterized by the formation of local singlets between neighboring moments and by localized moments aligned antiparallel to the field. This disordered phase is characterized by the absence of a gap, as is the case in a Bose glass. The associated field-driven quantum phase transition is consistent with the universality of a superfluid-to-Bose-glass transition. The robustness of the DLM phase and its prominent features, in particular a series of pseudo-plateaus in the magnetization curve, makes it accessible and relevant to experiments.
Using a numerical implementation of a strong-disorder renormalization group, we study the low-energy, long-distance properties of layers and bilayers of S=1∕2S=1∕2S=1∕2 Heisenberg antiferromagnets with different types of disorder: bond randomness, site dilution, and dimer dilution. Generally the systems exhibit an ordered and a disordered phase separated by a phase boundary on which the static critical exponents appear to be independent of bond randomness in the strong-disorder regime, while the dynamical exponent is a continuous function of the bond disorder strength. The low-energy fixed points of the off-critical phases are affected by the actual form of the disorder, and the disorder-induced dynamical exponent depends on the disorder strength. As the strength of the bond disorder is increased, there is a set of crossovers in the properties of the low-energy singularities. For weak disorder quantum fluctuations play the dominant role. For intermediate disorder nonlocalized disorder fluctuations are relevant, which become localized for even stronger bond disorder. We also present some quantum Monte Carlo simulation results to support the strong-disorder renormalization approach.
We use quantum Monte Carlo simulations to study a dimer-diluted S = 1/2 Heisenberg model on a bilayer square lattice with intralayer interaction J 1 and interlayer interaction J 2 . Below the classical percolation threshold p c , the system has three phases reachable by tuning the interaction ratio g = J 2 / J 1 : a Néel ordered phase, a gapless quantum glass phase, and a gapped quantum paramagnetic phase. We present the ground-state phase diagram in the plane of dilution p and interaction ratio g . The quantum glass phase is certified to be of the gapless Mott glass type, having a uniform susceptibility vanishing at zero temperature T and following a stretched exponential form at T > 0; χ u exp(- b / T α ) with α < 1. At the phase transition point from Neel ordered to Mott glass, we find that the critical exponents are different from those of the clean system described by the standard O (3) universality class in 2+1 dimensions.
The nature of the superfluid-to-Bose-glass (SF-BG) quantum phase transition, occurring in systems of interacting bosons immersed in a disordered environment, remains elusive. One fundamental open question is whether or not the transition obeys conventional scaling at quantum critical points (QCPs): this scaling would lock the value of the crossover exponent $\ensuremath{\phi}$---dictating the vanishing of the superfluid critical temperature upon approaching the QCP---to the value of quantum critical exponents for the ground-state transition. Yet such a relation between exponents has been called into question by several numerical as well as experimental results on the SF-BG transition. Here we revisit this issue in the case of the S=1/2S=1/2S=1/2 Heisenberg antiferromagnet on a site-diluted cubic lattice, which lends itself to efficient quantum Monte Carlo simulations. Our results show that the model exhibits a percolation transition in zero applied field, with the correlation length exponent $\ensuremath{\nu}=0.87(8)$ and $\ensuremath{\phi}=1.1(1)$ consistent with 3d3d3d percolation. When applying a sufficiently strong magnetic field, the dilution-induced transition decouples from geometric percolation, and it becomes a SF-BG transition; nonetheless, the $\ensuremath{\nu}$ and $\ensuremath{\phi}$ exponents maintain values consistent with those of the percolation transition. These results contradict the conventional scaling, which predicts $\ensuremath{\phi}\ensuremath{\geqslant}2$; and they suggest a possible relationship between the SF-BG transition and percolation of phase coherence.