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arXiv:cond-mat/0505492 · Physical Review Letters

Coherent Collisional Spin Dynamics in Optical Lattices

Artur Widera, Fabrice Gerbier, Simon Fölling, Tatjana Gericke, Olaf Mandel, Immanuel Bloch

Published Nov 3, 2005• 158 citations
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Abstract

We report on the observation of coherent, purely collisionally driven spin dynamics of neutral atoms in an optical lattice. For high lattice depths, atom pairs confined to the same lattice site show weakly damped Rabi-type oscillations between two-particle Zeeman states of equal magnetization, induced by spin-changing collisions. Moreover, measurement of the oscillation frequency allows for precise determination of the spin-changing collisional coupling strengths, which are directly related to fundamental scattering lengths describing interatomic collisions at ultracold temperatures.

DOI
10.1103/physrevlett.95.190405

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We report on the observation of coherent, purely collisionally driven spin dynamics of neutral atoms in an optical lattice. For high lattice depths, atom pairs confined to the same lattice site show weakly damped Rabi-type oscillations between two-particle Zeeman states of equal magnetization, induced by spin-changing collisions. Moreover, measurement of the oscillation frequency allows for precise determination of the spin-changing collisional coupling strengths, which are directly related to fundamental scattering lengths describing interatomic collisions at ultracold temperatures.
This thesis reports on the experimental investigation of controlled spin dependent interactions in a sample of ultracold Rubidium atoms trapped in a periodic optical potential. In such a situation, the most basic interaction between only two atoms at one common potential well, forming a micro laboratory for this atom pair, can be investigated. Spin dependent interactions between the atoms can lead to an intriguing time evolution of the system. In this work, we present two examples of such spin interaction induced dynamics. First, we have been able to observe and control a coherent spin changing interaction. Second, we have \nachieved to examine and manipulate an interaction\ninduced time evolution of the relative phase of a spin 1/2-system, both in the case of particle pairs and in the more general case of N interacting particles. The first part of this thesis elucidates the spin-changing interaction mechanism underlying many fascinating effects resulting from interacting spins at ultracold temperatures. This process changes the spin states of two colliding particles, while preserving total magnetization. If initial and final states have almost equal energy, this process is resonant and leads to large amplitude\noscillations between different spin states. The measured coupling parameters of such a process allow to precisely infer atomic scattering length differences, that e.g. determine the nature of the magnetic ground state of the hyperfine states in Rubidium.\nMoreover, a method to tune the spin oscillations at will based on the AC-Zeeman effect has been implemented. This allowed us to use resonant spin changing \ncollisions as a quantitative and non-destructive particle pair probe in the optical lattice. This led to a series of experiments shedding light on the Bosonic superfluid to Mott insulator transition.\nIn a second series of experiments we have been able to coherently manipulate the interaction induced time evolution of the relative phase in an ensemble of spin 1/2-systems. For two particles, interactions can lead to an entanglement oscillation of the particle pair. For the general case of N interacting particles, the ideal time evolution leads to the creation of spin squeezed states and even Schrödinger cat states. In the experiment we have been able to control the underlying\ninteractions by a Feshbach resonance. For particle pairs we could directly observe the entanglement oscillations. For the many particle case we have been able to observe and reverse the interaction induced dispersion of the relative phase.\nThe presented results demonstrate how correlated spin states can be engineered through \ncontrol of atomic interactions. Moreover, the results point towards the possibility to simulate quantum\nmagnetism phenomena with ultracold atoms in optical traps, and to realize and analyze many novel quantum spin states which have not been experimentally realized so far.
Quantum beat phenomenon presence in coherent spin dynamics of spin-2 87^{87}87Rb atoms in a deep optical lattice
Motivated by the recent experimental work (A. Widera, \textit{et al}, Phys. Rev. Lett. 95, 19045), we study the collisional spin dynamics of two spin-2 % ^{87}Rb atoms confined in a deep optical lattice. When the system is initialized as ∣0,0>|0,0>∣0,0>, three different two-particle Zeeman states are involved in the time evolution due to the conservation of magnetization. For a large magnetic field B>0.8B>0.8B>0.8 Guass, the spin coherent dynamics reduces to a Rabi-like oscillation between the states ∣0,0>|0,0>∣0,0> and % |1,-1>. However, under a small magnetic field, a general three-level coherent oscillation displays. In particular, around a critical magnetic field Bc≃0.48B_{c}\simeq 0.48Bc​≃0.48 Guass, the probability in the Zeeman states $% |2,-2> $ exhibits a novel quantum beat phenomenon, ready to be confirmed in future experiments.
We report on precision measurements of spin-dependent interaction-strengths in the 87 Rb spin-1 and spin-2 hyperfine ground states. Our method is based on the recent observation of coherence in the collisionally driven spin-dynamics of ultracold atom pairs trapped in optical lattices. Analysis of the Rabi-type oscillations between two spin states of an atom pair allows a direct determination of the coupling parameters in the interaction Hamiltonian. We deduce differences in scattering lengths from our data that can directly be compared to theoretical predictions in order to test interatomic potentials. Our measurements agree with the predictions within 20%. The knowledge of these coupling parameters allows one to determine the nature of the magnetic ground state. Our data imply a ferromagnetic ground state for 87 Rb in the f = 1 manifold, in agreement with earlier experiments performed without the optical lattice. For 87 Rb in the f = 2 manifold, the data point towards an antiferromagnetic ground state; however our error bars do not exclude a possible cyclic phase.
Quantum gases in optical lattices allow for fundamental studies in atomic and condensed-matter physics and the exploration of novel effects. After a brief introduction to the fundamentals of quantum gas experiments in optical lattices, we discuss two recent experiments focusing on driven matter waves in a one-dimensional optical lattice. The first experiment uses a tilted bichromatic optical lattice to investigate the interplay of disorder and collisional interactions in the accelerated transport of a Bose-Einstein condensate. Here, a screening effect is observed, in which the interactions effectively cancel the damping of Bloch oscillations induced by a (quasi-)disordered potential. This effect can be understood through a modification of the underlying band structure by the interactions. The second experiment studies the dynamics of a weakly trapped condensate resonantly coupled to the orbitals of a strongly confining state-selective lattice. We observe momentum distributions that correspond to matter wave diffraction from a periodic structure; however, the diffractive dynamics remain strongly linked to the internal-state Rabi oscillations. In the regime investigated, which we call the nonadiabatic regime, no diffracting potential can be defined. We show how only for much stronger coupling, the internal and external dynamics decouple, transitioning from nonadiabatic diffraction to the well-studied Kapitza-Dirac diffraction. We further investigate prospects for realizing dissipative spin models in our ultracold atomic gas experiment. To this end, we develop and test in the laboratory several possible implementations of effective spins with differential coupling to a superfluid background and examine their viability for a realization of the spin-boson model. | 94 pages
We report on high-resolution optical spectroscopy of interacting bosonic 174 Yb atoms in deep optical lattices with negligible tunneling. We prepare Mott insulator phases with singly- and doubly-occupied isolated sites and probe the atoms using an ultra-narrow 'clock' transition. Atoms in singly-occupied sites undergo long-lived Rabi oscillations. Atoms in doubly-occupied sites are strongly affected by interatomic interactions, and we measure their inelastic decay rates and energy shifts. We deduce from these measurements all relevant collisional parameters involving both clock states, in particular the intra- and inter-state scattering lengths.
Temporal evolution of a macroscopic condensate of ultracold atoms is usually driven by mean-field potentials, either due to scattering between atoms or due to coupling to external fields; and coherent quantum dynamics of this type have been observed in various cold atom experiments. In this paper, we report results of studies of a class of quantum spin dynamics which are purely driven by zero point quantum fluctuations of spin collective coordinates. Unlike the usual mean-field coherent dynamics, quantum-fluctuation-controlled spin dynamics (or QFCSD) studied here are very sensitive to variation of quantum fluctuations and the corresponding driving potentials induced by zero point motions can be tuned by four to five orders of magnitude using optical lattices. These dynamics have unique dependence on optical lattice potential depths and quadratic Zeeman fields. We also find that thermal fluctuations generally can further enhance the induced potentials although the enhancement in deep optical lattices is much less substantial than in traps or shallow lattices. QFCSD can be potentially used to calibrate quantum fluctuations and investigate correlated fluctuations and various universal scaling properties near quantum critical points.